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arXiv:1502.02773 · Journal of Optics

Where are photons created in parametric down-conversion? On the control of the spatio–temporal properties of biphoton states

A Büse, Nora Tischler, Mathieu L. Juan, Gabriel Molina‐Terriza

Published May 1, 2015• 8 citations
arXivHTMLPDF

Abstract

In spontaneous parametric down-conversion, pairs of photons are known to be created coherently and with equal probability over the entire length of the crystal. Then, there is no particular position in the crystal where a photon pair is created. We make the seemingly contradictory observation that the time delay between the photons in the pair depends on the distance from the crystal to the collection lens, as if the photons were actually collected preferentially from a particular position in the crystal. We resolve this contradiction by showing that the spatio–temporal correlations critically affect the temporal properties of the pair of photons. The theoretical model we present matches all our experimental results. We expect this to have important implications for experiments that require indistinguishable photons.

DOI
10.1088/2040-8978/17/6/065201

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In spontaneous parametric down-conversion, pairs of photons are known to be created coherently and with equal probability over the entire length of the crystal. Then, there is no particular position in the crystal where a photon pair is created. We make the seemingly contradictory observation that the time delay between the photons in the pair depends on the distance from the crystal to the collection lens, as if the photons were actually collected preferentially from a particular position in the crystal. We resolve this contradiction by showing that the spatio–temporal correlations critically affect the temporal properties of the pair of photons. The theoretical model we present matches all our experimental results. We expect this to have important implications for experiments that require indistinguishable photons.
Abstract Spontaneous parametric down-conversion (SPDC) is a widely used process to prepare entangled photon pairs. In SPDC, a second-order nonlinear crystal is pumped by a coherent laser beam to generate photon pairs. The photon pairs are usually detected by single-mode fibers (SMF), where only photons in a Gaussian mode can be collected. The collection modes possess typical Gaussian parameters, namely a beam waist and a focal plane position. The collection efficiency of photons highly depends on the choice of both parameters. The exact focal plane position of the pump beam relative to those of the detection modes is difficult to determine in a real experiment. Usually, theoretical and experimental studies assume that the focal plane positions of the pump and the generated beams are positioned in the center of the crystal. The displacement of beam focal planes can lead to deviations from expected results and the coupling efficiency into SMF can decrease. In this study, we theoretically examine variable positions of focal planes in the Laguerre–Gaussian basis, a popular experimental modal decomposition of the spatial biphoton state. We explore how the choice of focal plane positions affects the spatial and temporal properties and the purity of the photon pairs. We present SPDC setups where precise knowledge of the focal plane position is essential and scenarios where focal plane displacements have negligible impact on experimental outcomes. Graphical Abstract
In the process of spontaneous parametric down-conversion, photons from a pump field are converted to signal and idler photon pairs in a nonlinear crystal. The reversed process, or up-conversion of these pairs back to single photons in a second crystal, is also possible. Here, we present experimental measurements of the up-conversion rate with a controlled time delay introduced between the signal and idler photons. As a function of delay, this rate presents a full width at half maximum of 27.9 fs under our experimental conditions, and we further demonstrate that group delay dispersion of the photon pairs broadens this width. These observations are in close agreement with our calculations, thus demonstrating an ultrafast, nonclassical correlation between the signal and idler waves.
The entangled photon pairs (biphotons) produced from parametric down-conversion (PDC) in a χ(2)crystal are the key element for several quantum information and communication schemes. Recent theoretical investigations [1–2] have revealed the peculiar structure of the biphotonic correlation characterizing the entanglement of twin beams in the space-time domain. The biphotonic correlation in type I PDC is characterized in the near field by a X-shaped geometry, which turns out to be non-factorable in space and time, offering thus the relevant possibility of manipulating the temporal bandwidth of biphoton entanglement by acting on their spatial degrees of freedom. The name “X-entanglement” was coined to describe this geometry [1]. An other key feature which emerged is the extreme spatial and temporal localization of the biphotonic correlation, on the micrometer and femtosecond range, respectively.
Spontaneous parametric down-conversion (SPDC) is a widely used process to prepare entangled photon pairs. In SPDC, a second-order nonlinear crystal is pumped by a coherent laser beam to generate photon pairs. The photon pairs are usually detected by single-mode fibers (SMF), where only photons in a Gaussian mode can be collected. The collection modes possess typical Gaussian parameters, namely a beam waist and a focal plane position. The collection efficiency of photons highly depends on the choice of both parameters. The exact focal plane position of the pump beam relative to those of the detection modes is difficult to determine in a real experiment. Usually, theoretical and experimental studies assume that the focal plane positions of the pump and the generated beams are positioned in the center of the crystal. The displacement of beam focal planes can lead to deviations from expected results and the coupling efficiency into SMF can increase or decrease. In this work, we consider variable positions of focal planes and investigate how shifts of these focal planes influence the spatial and temporal properties of photon pairs. We present SPDC arrangements, in which the knowledge of the exact position of the focal planes is essential, as well as scenarios, where focal plane displacements do not contribute significantly to experimental outcomes. These findings are of particular interest for achieving higher efficiency in SPDC experiments.
Image resolution of quantum imaging with undetected photons is governed by the spatial correlations existing between the photons of a photon pair that has been generated in a nonlinear process. These correlations allow for obtaining an image of an object with light that never interacted with that object. Depending on the imaging configuration, either position or momentum correlations are exploited. We hereby experimentally analyse how the crystal length and pump waist affect the image resolution when using position correlations of photons that have been generated via spontaneous parametric down conversion in a nonlinear interferometer. Our results support existing theoretical models for the dependency of the resolution on the crystal length. In addition, we probe the resolution of our quantum imaging scheme for varying pump waists over one order of magnitude. This analysis reveals the intricate dependency of the resolution on the strength of the correlations within the biphoton states for parameter combinations in which the crystal lengths are much larger than the involved photon wavelengths. We extend the existing models in this parameter regime to properly take nontrivial effects of finite pump waists into account and demonstrate that they match the experimental results.
We investigate the spatio-temporal structure of the biphoton entanglement in Parametric Down Conversion (PDC). In particular we study the biphoton amplitude at the output face of the nonlinear crystal (near-field) and we demonstrate its X-shaped geometry in the space-time dimensions, i.e. the non-factorability of the state with respect to spatial and temporal variables. Our analysis provides a precise and quantitative characterization of this structure in various regimes and types of phase matching of PDC. The key elements of novelty emerging from our analysis are the non-factorability of the state with respect to spatial and temporal variables, and the extreme relative localization of the entangled photons, both in space (few microns) and time (few femtoseconds). This extreme localization is connected to our ability to resolve the photon positions in the source near-field. The non factorability opens the possibility of tailoring the temporal entanglement by acting on the spatial degrees of freedom of twin photons.