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arXiv:1410.7110 · Physical Review A

Generation and quantum control of giant plasmon pulses by transient quantum coherence

Weiguang Huo, Dmitri V. Voronine, Marlan O. Scully

Published Apr 30, 2015• 2 citations
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Abstract

Amplified ultrashort laser pulses are useful in many fields of science and engineering. We propose a quantum approach to ultrashort pulse generation using transient quantum coherence that predicts order of magnitude stronger pulses generated with lower input energy than in the steady-state regime. This femtosecond quantum-coherent analog of nanosecond $Q$ switching is not limited by the pulse duration constraints of the latter and, in principle, may be used for a variety of lasers including plasmon nanolasers. This approach, applied to the generation of giant plasmon pulses, could achieve quantum control of plasmon relaxation dynamics by varying the drive-pulse delay, amplitude, and duration. This holds promise for a new control mechanism. We discuss implementations and applications of this source of ultrashort nano-optical studies.

DOI
10.1103/physreva.91.043844

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Amplified ultrashort laser pulses are useful in many fields of science and engineering. We propose a quantum approach to ultrashort pulse generation using transient quantum coherence that predicts order of magnitude stronger pulses generated with lower input energy than in the steady-state regime. This femtosecond quantum-coherent analog of nanosecond QQQ switching is not limited by the pulse duration constraints of the latter and, in principle, may be used for a variety of lasers including plasmon nanolasers. This approach, applied to the generation of giant plasmon pulses, could achieve quantum control of plasmon relaxation dynamics by varying the drive-pulse delay, amplitude, and duration. This holds promise for a new control mechanism. We discuss implementations and applications of this source of ultrashort nano-optical studies.
Abstract Quantum coherence and interference offer novel pathways to control light–matter interaction at the atomic scale, with enticing prospects in both fundamental and applied science. Here, we demonstrate coherent control over transient excitation of localized surface plasmon modes of a silver nanosphere adjacent to a quantum coherence medium composed of three-level quantum emitters, using a theoretical approach. We show that quantum interference enables more than two orders of magnitude enhancement in the surface plasmon field generated when the quantum emitters are driven coherently, in comparison to incoherent pumping. Furthermore, under optimal conditions, intense surface plasmon lasing can be induced without population inversion on the spasing transition. Our results open up the possibility of overcoming dissipative losses in plasmonic modes in the transient regime when steady-state population inversion is difficult to achieve due to fast relaxation rates and impractical pumping requirements.
Nanoscale pulsed light is highly desirable in nano-integrated optics. In this paper, we obtained femtosecond pulses with THz repetition frequency via the coupling between quantum emitters (QEs) and plasmonic resonators. Our structure consists of a V\mathsf{V}V-groove (VG) plasmonic resonator and a nanowire embedded with two-level QEs. The influences of the incident light intensity and QE number density on the transmission response for this hybrid system are investigated through semiclassical theory and simulation. The results show that the transmission response can be modulated to the pulse form. And the repetition frequency and extinction ratio of the pulses can be controlled by the incident light intensity and QE number density. The reason is that the coupling causes the output power of nanowire to behave as an oscillating form, the oscillating output power in turn causes the field amplitude in the resonator to oscillate over time. A feedback system is formed between the plasmonic resonator and the QEs in the nanowire. This provides a method for generating narrow pulsed lasers with ultrahigh repetition frequencies in plasmonic systems using a continuous wave input, which has potential applications in generating optical clock signals at the nanoscale.
The four-wave mixing produced with two ultrashort phase-locked !-3! laser pulses propagating coherently in a two-level system in the infrared spectral region is shown to depend on the pulses relative phase. The Maxwell-Bloch equations are solved beyond the rotating-wave approximation to account for field frequencies which are largely detuned from the atomic resonance. The relative phase dominating the efficiency of the coupling to the 5! anti-Stokes Raman component is determined by sign of the total ac Stark shift induced in the system, in such a way that the phase influence disappears precisely where the ac Stark effect due to both pulses is compensated. This fundamental quantum interference effect can be the basis for nonlinear ultrafast optical spectroscopy techniques. Phenomena arising from the coherent control of nonlinear interactions are of importance in fields as diverse as optoelectronics and materials research, in high harmonic generation, in photoionization or molecular dissociation, and in biological applications such as spectroscopy and imaging, among others [1, 2, 3, 4, 5, 6, 7]. Optical quantum coherent control is based on the fact that the phases of interfering transition amplitudes in light-matter interactions can be controlled through the optical phase of coherent light sources that drive the interaction, in such a way that the transition rates to final states and the dynamics at various stages of the process can be modified [1]. In a recent paper [8], a theoretical investigation on the quantum coherent control of the optical transient four-wave mixing of two intense phase-locked femtosecond laser pulses of central angular frequencies ω and 3ω propagating in a two-level atom (TLA) was reported. It was shown how the nonlinear (χ (3) ) coupling to the antiStokes Raman field at frequency 5ω depends critically on the initial relative phase φ of the propagating pulses. In Ref. [8], the study was centered to intense pulses in the visible and ultraviolet spectral regions, with frequencies at resonance or lower than the atomic transition. The phenomena observed in [8], however, can be scaled to various laser and material parameters. In the infrared spectral range, for instance, experiments on ultrafast molecular dynamics are frequently performed by help of twocolor pump probe nonlinear spectroscopy techniques. In this type of studies, due to the high intensities inherent to ultrashort (subpicosecond) pulses, nonlinear effects such as stimulated Raman processes may become important and are often utilized as a complementary tool to gain information [9]. In this Letter, we address the conditions for quantum coherent control of transient four-wave mixing interactions with two phase-locked ω-3ω femtosecond laser pulses in the mid-IR spectral region. Our purpose is to reveal the basic physics for a strict two-level medium and to this end the Maxwell-Bloch TLA will be considered. We will study pulses with a duration of 300 fs (with a w 5w
Electronic flying qubits offer an interesting alternative to photonic qubits: electrons propagate slower, hence easier to control in real time, and Coulomb interaction enables direct entanglement between different qubits. Although their coherence time is limited, flying electrons in the form of picosecond plasmonic pulses could be competitive in terms of the number of achievable coherent operations. The key challenge in achieving this critical milestone is the development of a new technology capable of injecting ‘on-demand’ single-electron wavepackets into quantum devices, with temporal durations comparable to or shorter than the device dimensions. Here, we take a significant step towards achieving this regime in a quantum nanoelectronic system by injecting ultrashort single-electron plasmonic pulses into a 14-micrometer-long Mach-Zehnder interferometer. Our results establish that quantum coherence is robust under the on-demand injection of ultrashort plasmonic pulses, as evidenced by the observation of coherent oscillations in the single-electron regime. Building on this, our results demonstrate the existence of a “non-adiabatic" regime that is prominent at high frequencies. This result highlights the potential of flying qubits as a promising alternative to localised qubit architectures, offering advantages such as a reduced hardware footprint, enhanced connectivity, and scalability for quantum information processing. The development of electronic flying qubits requires the ability to generate and control single-electron excitations. Here the authors demonstrate quantum coherence of ultrashort single-electron plasmonic pulses in an electronic Mach-Zehnder interferometer, revealing a non-adiabatic regime at high frequencies.
Our recent studies of methods for obtaining ultrashort light pulses and analysis of the impact of ultrashort optical pulses on classical and quantum micro-objects with the identification of the determining role of the degree of unipolarity of pulses (maximum for strictly unipolar pulses) in the efficiency of direct laser acceleration of charged particles and excitation of atoms and molecules have been reviewed. Special attention has been paid to the coherent mode locking regime in lasers, which is implemented when the laser pulse duration is less than the relaxation time of the working transition in media with resonance amplification and absorption (laser analog of the phenomenon of self-induced transparency). Experimental data on coherent mode locking in a titanium-sapphire laser with a cell with rubidium vapor at self-induced transparency in rubidium have been presented. The interaction of ultrashort pulses in resonant media has also been analyzed.
Ultra-short pulses with high repetition frequency have great application prospects in the field of nano-optics. Here, in the case of continuous wave incidence, the femtosecond pulses with THz repetition frequency are achieved in the transmission system consisting of quantum emitters (QEs) and plasmonic resonators. The generation mechanism of the ultra-short pulses with high repetition frequency is elucidated by semi-classical model. Attribute to the presence of the two-level QEs, the field amplitude in plasmonic resonator is oscillating with time, resulting in the transmittance of the system behave as the form of pulse oscillation. Moreover, the pulse repetition frequency and extinction ratio can be freely controlled by the incident light intensity and QEs number density to obtain the required ultra-short pulses at nanoscale. This also has potential applications in high-speed signal processing fields and generating optical clock signals that can be used in optical computing.