Quantum memories are indispensable for quantum communication and quantum computation, which are able to realize the storage and retrieval of a quantum state such as a single photon, entanglement, or a squeezed state on demand. Among those memories realized by different protocols, the Raman quantum memory has advantages in its broadband and high-speed properties, resulting in huge potential applications in quantum network and quantum computation. However, the realization of Raman quantum memory for a true single photon and photonic entanglement is a challenging job. In this review, after briefly introducing the main benchmarks for quantum memories, showing the state of the art, we focus on the review of the experimental progress recently achieved in storing the quantum state by Raman scheme in our group. We believe that all achievements reviewed are very hopeful in building up a high-speed quantum network.
Constructing a quantum memory for a photonic entanglement is vital for realizing quantum communication and network. Because of the inherent infinite dimension of orbital angular momentum (OAM), the photon's OAM has the potential for encoding a photon in a high-dimensional space, enabling the realization of high channel capacity communication. Photons entangled in orthogonal polarizations or optical paths had been stored in a different system, but there have been no reports on the storage of a photon pair entangled in OAM space. Here, we report the first experimental realization of storing an entangled OAM state through the Raman protocol in a cold atomic ensemble. We reconstruct the density matrix of an OAM entangled state with a fidelity of 90.3%±0.8% and obtain the Clauser-Horne-Shimony-Holt inequality parameter S of 2.41±0.06 after a programed storage time. All results clearly show the preservation of entanglement during the storage.
A quantum memory for photonic entanglement is the basic component in quantum networks. Photons entangled in multiple degrees of freedom enable the mutual transformation of Hilbert spaces for the same particle and different particles, thereby connecting heterogeneous nodes in the quantum network. So far, the quantum storage for photonic entanglement is limited to two degrees of freedom. Here, we demonstrate the heralded storage of single-photon hybrid entanglement involving three degrees of freedom (polarization, orbital angular momentum, and path) using a solid-state medium. The fidelity of the output state with the ideal maximum entangled state is $94.0\ifmmode\pm\else\textpm\fi{}0.8%$. The quantum property of the retrieved state is verified by testing the hypothesis of noncontextual hidden-variable theories. These results demonstrate the entanglement interface between light and matter involving multiple degrees of freedom, paving the way for the construction of hybrid quantum networks.
Abstract Quantum entanglement recognized by Einstein, Podolsky, Rosen and Schrodinger is the essence of quantum physics, and has become a real available resource in the laboratory over recent years. The observation of quantum entanglement in macroscopic matters has implications in the fundamental studies of quantum mechanics, as well as the implementations of quantum information technologies, such as quantum communication, enhanced sensing and distributed quantum computing. Here, we report the creation and storage of the heralded entanglement between two different types of broadband quantum memories located on separated platforms at room temperature: a single-photon entangled state delocalized between billions of motional atoms as a collective excitation and an all-optical loop as a flying qubit. The stored entangled state is subsequently retrieved after a programmable storage time, and is verified by measuring the nonclassical correlations, quantum interference, and concurrence of the mapped-out Raman-scattered photons. Our results show that quantum entanglement can be sustained in macroscopic matters at ambient condition, which pushes the fundamental researches of the transition boundary between quantum and classical worlds. Also, the two quantum memories constitute a hybrid memory-built-in quantum network, which highlights the potential of the cooperation between an stationary atomic ensemble and an all-optical loop as quantum nodes at ambient condition, and brings a significant step towards practical quantum networks.
Quantum memories are key components in quantum information networks. Their ability to store and retrieve information on demand makes repeat-until-success strategies scalable. Warm alkali-metal vapours are interesting candidates for the implementation of such memories, thanks to their long storage times and experimental simplicity. Operation with the Raman protocol enables high time-bandwidth products, which allows for multiple synchronisation trials of probabilistically operating quantum gates via memory-based temporal multiplexing. This makes the Raman memory a promising tool, whose broad spectral bandwidth facilitates direct interfacing with other photonic primitives, such as single photon sources. Here, such a light-matter interface is implemented in a warm caesium vapour. Firstly, we study the storage of polarisation-encoded information in the memory. High quality polarisation preservation for bright coherent state input signals can be achieved, when operating the Raman memory in a dual-rail configuration inside a polarisation interferometer. Secondly, heralded single photons are stored in the memory. To this end, the memory is operated on-demand by feed-forward of source heralding events, which is a key technological capability. Prior to storage, single photons are produced in a spontaneous parametric down conversion source, whose bespoke design spectrally tailors the photons to the memory acceptance line. The faithful retrieval of stored single photons is found to be currently limited by noise in the memory, with a signal-to-noise ratio of 0.3 in the memory output. Nevertheless, a clear influence of the input's quantum nature is observed in the retrieved light by measuring signal's photon statistics. Finally, the memory noise processes are examined in detail. Four-wave-mixing noise is determined as the sole important noise source for the Raman memory.
Quantum memory is a key component of quantum networks. A successful development in enabling the distribution of quantum information requires the storage of single-photon light. Usually quantum information is encoded using a 2D space, spanned, for example, by the orthogonal polarization states of a photon. In this case, each photon carries a quantum bit of information. If the photon could be encoded in a high-dimensional space instead, the information carried by each photon could be increased from a bit to |
log2d| bits, where d is the dimension of the Hilbert space in which the photon is described. The channel capacity of the network and the transmission efficiency would then be greatly enlarged [1]. Moreover, storing high-dimensional states in quantum memory can reduce its sensitivity to memory coherence time [2], leading to significant improvements in storage capacity [3]. It is thus no surprise that many research groups are actively working on different physical systems for storing light encoded using a high-dimensional space. The degrees of freedom for position, linear momentum, time-bin or orbital angular momentum (OAM) of a photon can all be considered as a high-dimensional space for encoding. The photon's OAM has the most potential for encoding [4]. Electromagnetic waves have both spin and OAM. Spin angular momentum produces polarization. Photons with OAM can be regarded as helices with left and right handedness twisted to varying degrees (Fig. 1). Information is encoded using this handedness and the amount of twist. Because of the inherent infinite degrees of freedom for OAM, a photon can in principle carry an arbitrarily large amount of information, and hence the eagerness to store light encoded in OAM space. Although some work on this has been reported for different physical systems, what is lacking is a way of storing and releasing at some later time a true single photon, including its shape and structure [5–7]. Constructing this basic element of quantum memory has been a major challenge. The wavefront of an OAM light is a helical structure (left and center), with an optical vortex at its center in the intensity distribution of light (right). The vortex of light can carry non-zero OAM of any order m. OAM states of a different order are orthogonal. A group at the Key Laboratory of Quantum Information, Chinese Academy of Science, at the University of Science and Technology of China finally resolved this problem [8]. They reported on the first experimental realization of a true single-photon-carrying OAM stored via electromagnetically induced transparency (EIT) in a cold atomic ensemble (Fig. 2). With such a suitable candidate, this work indicates a means of constructing high-dimensional quantum memory. After this, similar results were reported by Laurat's group at Laboratoire Kastler Brossel, at Université Pierre et Marie Curie in France [9], where an extremely weak laser at single-photon level carrying OAM was also stored via EIT in a cold atomic ensemble. Ding et al. [8] first prepared two cold 85Rb atomic clouds in two magnetic-optical traps (MOT) using laser cooling and trapping techniques. They generated non-classical correlated photon pairs using spontaneous four-wave mixing in an atomic cloud. One photon of each pair was used as a trigger; the other mapped and stored in a second atomic cloud via EIT. Each photon to be stored carried one OAM unit. After a programed storage time, the photon was retrieved. What they achieved during storage included (1) proof that the non-classical correlation between the trigger photon and the retrieved photon is retained by demonstrating a strong violation of the Cauchy–Schwarz inequality, (2) a demonstration that the single-photon property of the signal photon is maintained by performing the Hanbury–Brown and Twiss experiment on the trigger photon, (3) proof that the spatial structure of the photon is also very well preserved by showing a high similarity between input and output, and (4) evidence, gathered by Sagnac interferometry, that the coherence of a single photon is also preserved. A heralded single photon is generated through spontaneous four-wave mixing in MOT 1 (a); this single photon carrying OAM is then stored through EIT in MOT 2 (b); (c) shows an image of the photon carrying OAM. Experimental measurements in the transverse position of the image carried by the photon before and after storage are presented in (d) and (e), respectively; (f) shows the simplified experimental setup for storage of a superposition of OAM. Interference patterns taken at different angle settings of the half-wave plate are shown in (g). The left column represents the experimental angle settings of the half-wave and the quarter-wave plates, the middle column gives the experimental results, and the right column gives results from theoretical simulations; (h) and (i) present the interference patterns of the input signal photon and the retrieved signal with plate angle, respectively. This is a significant breakthrough towards the realization of a quantum internet and, potentially, quantum computing. This work addresses the ability to generate, store, retrieve on demand an arbitrary single-photon-level photonic state encoded in OAM space. It signifies an important step in the development of practical quantum-enabled technologies, opens up the possibility for realizing high-dimensional quantum memories based on this degree of freedom of light, and will have a large impact in a broad physical community, especially in the quantum information and quantum optics communities. The Technology Review website of MIT comments on their work very positively with an article entitled ‘First Quantum Memory That Records the Shape of a Single Photon Unveiled in China’. Further, Nature Photonics selected this work as a research highlight. Clearly, memory that can preserve the spatial structure of photons will make the internet far more flexible and capable. Of course, there are still many basic problems remaining that need to be solved to build the future quantum internet, one of which is the construction of quantum memory exploiting entanglement. This derives from the fact that a quantum network needs the distribution of quantum-entangled photons over channels between different nodes [10]. A high-dimensional quantum internet needs to store OAM-entangled states and perform entanglement swapping to efficiently extend the achievable communication distances. While Ding et al. [8] reported the storage of light with OAM at the single-photon level, the photon was, however, still encoded in a 2D space. Therefore, whether it is possible to construct a high-dimensional quantum memory remains an open issue that needs to be investigated further.