Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and it has become a highly successful method for experiments in chemical physics. Current quantum optical experiments approach system sizes and levels of complexity that require the development of efficient techniques to assess spectral and dynamical features with scalable experimental overhead. However, established methods from optical spectroscopy of macroscopic ensembles cannot be applied straightforwardly to few-atom systems. Based on the ideas proposed in M. Gessner et al., (arXiv:1312.3365), we develop a diagrammatic approach to construct nonlinear measurement protocols for controlled quantum systems, and we discuss experimental implementations with trapped ion technology in detail. These methods, in combination with distinct features of ultracold-matter systems, allow us to monitor and analyze excitation dynamics in both the electronic and vibrational degrees of freedom. They are independent of system size, and they can therefore reliably probe systems in which, e.g., quantum state tomography becomes prohibitively expensive. We propose signals that can probe steady-state currents, detect the influence of anharmonicities on phonon transport, and identify signatures of chaotic dynamics near a quantum phase transition in an Ising-type spin chain.
Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and it has become a highly successful method for experiments in chemical physics. Current quantum optical experiments approach system sizes and levels of complexity that require the development of efficient techniques to assess spectral and dynamical features with scalable experimental overhead. However, established methods from optical spectroscopy of macroscopic ensembles cannot be applied straightforwardly to few-atom systems. Based on the ideas proposed in M. Gessner et al., (arXiv:1312.3365), we develop a diagrammatic approach to construct nonlinear measurement protocols for controlled quantum systems, and we discuss experimental implementations with trapped ion technology in detail. These methods, in combination with distinct features of ultracold-matter systems, allow us to monitor and analyze excitation dynamics in both the electronic and vibrational degrees of freedom. They are independent of system size, and they can therefore reliably probe systems in which, e.g., quantum state tomography becomes prohibitively expensive. We propose signals that can probe steady-state currents, detect the influence of anharmonicities on phonon transport, and identify signatures of chaotic dynamics near a quantum phase transition in an Ising-type spin chain.
Certain classes of quantum many-body systems, including those supporting phenomena like high-Tc superconductivity and spin liquids, are believed to be fundamentally intractable to classical modeling. Quantum simulations, in which synthetic materials are engineered by inducing well-controlled quantum systems like ultracold atoms to obey many-body Hamiltonians of interest, are a promising new approach to study this type of physics. In this work, I present several advances toward this ultimate goal of large-scale, highly controllable quantum simulations of many-body spin physics. We simulate long-range Ising and XY spin models in the presence of transverse and longitudinal magnetic fields using chains of up to 18 ultracold 171Yb+ ions held in a linear Paul trap, where two hyperfine levels in each ion encode spin-1/2 states. The tunable spin-spin interactions and effective magnetic fields are engineered using laser fields, and the individual spin states are directly imaged with state-dependent fluorescence. The results in this thesis address several of the ongoing challenges in the development of synthetic quantum matter platforms. One such challenge is establishing more flexible capabilities in the sorts of Hamiltonians we can model. By observing suppression of the ground state spin ordering, we have demonstrated our ability to continuously tune the interaction range in a power-law interaction pattern, and hence the amount of frustration present in the spin system. We have additionally begun developing tools to study particles of higher spin, which could eventually be used to create and study topological phases of matter. Another challenge is the necessity of identifying problems that the next generation of experiments, with flexible (but not arbitrary) controls and classically intractable (but not infinitely large) system sizes, can feasibly shed new light on. We have made measurements of how the range of interaction affects dynamics of spin correlations propagating through the chain, and the excellent agreement between our observations and numerical simulations indicate that at larger sizes, our experiment can meaningfully contribute to the open question of the fundamental speed limit on the transfer of information through such a spin chain. Finally, for classically intractable system sizes, it will be crucial to have multiple techniques at our disposal for validating our understanding of the exact microscopic model being implemented. We have developed and demonstrated an MRI-like spectroscopic technique for probing the energies of the many-body Hamiltonian, which serves as a new method for validating quantum simulations of the transverse Ising model. Our experiments can potentially be scaled up in the near future to study fully connected lattice spin models with several tens of spins, where classical computation begins to fail, and the results described in this thesis contribute to the effort to build experiments that can break new ground in the study of quantum many-body physics.
Scaling trapped-ion quantum sensors from single ions to large ensembles is a key challenge for next-generation precision measurements. At the same time, many ion species of interest for optical clocks and tests of fundamental physics lack closed cycling transitions required for direct laser cooling and state detection. Collective quantum logic spectroscopy addresses both limitations by coupling an ensemble of sensor, or spectroscopy, ions to one or more logic ions that provide sympathetic cooling and state readout. Here, we establish the fundamental performance limits and operating regimes of this protocol, identifying how the interaction strength, interrogation time, and logic-ensemble size govern sensitivity, dynamic range, and robustness to experimental imperfections. We show that quantum-limited sensitivity can be retained even with a single logic ion, while increasing the number of logic ions substantially improves readout efficiency and robustness. Beyond precision metrology, the same collective interface enables many-body measurements relevant to quantum information processing, including parity measurements and stabilizer-like syndrome extraction. Our results establish collective quantum logic spectroscopy as a scalable framework for optical clocks, quantum-enhanced sensing, and trapped-ion quantum information processing.
We present experimental results of using trapped ions for the study of energy transport and quantum correlations in many-body systems. We investigate energy propagation by locally exciting one end of an ion chain and then observing the subsequent dynamics. The experimental results agree with the presented normal mode model of ion motion, and signify the first steps towards realizing theoretical proposals of studying many-body physics with the motional degree of freedom of trapped ions. Additionally, we present a method for detecting correlations between an open quantum system and its environment by acting only locally on the open system. We implement this method using a single trapped ion and discuss our current work towards extending the results to larger systems. Lastly, we demonstrate how the presented method for local detection of quantum correlations can be used for detection of quantum phase transitions.
Single trapped ions trapped in Paul traps correspond to ideal candidates for realization of extremely accurate optical atomic clocks and practical studies of the light–atom interactions and nonlinear mechanical dynamics. These systems benefit from both, the superb isolation of the ion from surrounding environment and excellent control of its external and internal\ndegrees of freedom, at the same time, which makes them exquisite platforms for experimental studies and applications of light matter interaction at its most fundamental level. The exceptional degree of control of single or few ion's state enabled in past decade number of major advancements in the applications from the fields of experimental quantum information\nprocessing and frequency metrology, including recent realization of scalable Shor's\nalgorithm, fractional uncertainties of the frequency measurements close to 10-18 level, or simulations of complex quantum many-body effects. These results, together with the rapid advancements in the production of low-noise segmented micro-traps, promise prompt access to long-desired regimes of quantum optomechanics and further development and applications\nof optical atomic clocks.
Many outstanding problems in quantum physics, such as high-Tc superconductivity or quark confinement, are still - after decades of research - awaiting commonly accepted explanations. One reason is that such systems are often difficult to control, show an intermingling of several effects, or are not easily accessible to measurement. To arrive at a deeper understanding of the physics at work, researchers typically derive simplified models designed to capture the most striking phenomena of the system under consideration. However, due to the exponential complexity of Hilbert space, even some of the simplest of such models pose formidable challenges to analytical and numerical calculations. In 1982, Feynman proposed to solve such quantum models with experimental simulation on a physically distinct, specifically engineered quantum system [Int. J. Theor.Phys. 21, 467]. Designed to be governed by the same underlying equations as the original model, it is hoped that direct measurements on these so called quantum simulators (QSs) will allow to gather deep insights into outstanding problems of physics and beyond. In this thesis, we identify four requirements that a useful QS has to fulfill, relevance, control, reliability, and efficiency. Focusing on these, we review the state of the art of two popular approaches, digital QSs (i.e., special purpose quantum computers) and analog QSs (devices with always-on interactions). Further, focusing on possibilities to increase control over QSs, we discuss a scheme to engineer quantum correlations between mesoscopic numbers of spinful particles in optical lattices. This technique, based on quantum polarization spectroscopy, may be useful for state preparation and quantum information protocols. Additionally, employing several analytical and numerical methods for the calculation of many-body ground states, we demonstrate the variety of condensed-matter problems that can be attacked with QSs consisting of ultracold ions or neutral atoms in optical lattices. The chosen examples, some of which have already been realized in experiment, include such diverse settings as frustrated antiferromagnetism, quantum phase transitions in exotic lattice geometries, topological insulators, non-Abelian gauge-fields, orbital order of ultracold Fermions, and systems with long-range interactions. The experimental realization of all of these models requires techniques which go beyond standard optical lattices, e.g., time-periodic driving of lattices with exotic geometry, loading ultracold atoms into higher bands, or immersing trapped ions into an optical lattice. The chosen models, motivated by important open questions of quantum physics, pose difficult problems for classical computers, but they may be amenable in the near future to quantum simulation with ultracold atoms or ions. While the experimental control over relevant models has increased dramatically in the last years, the reliability and efficiency of QSs has received considerably less attention. As a second important part of this thesis, we emphasize the need to consider these aspects under realistic experimental conditions. We discuss specific situations where terms that have typically been neglected in the description of the QS introduce systematic errors and even lead to novel physics. Further, we characterize in a generic example the influence of quenched disorder on an analog QS. Its performance for simulating universal behavior near a quantum phase transition seems satisfactory for low disorder. Moreover, our results suggest a connection between the reliability and efficiency of a QS: it works less reliable exactly in those interesting regimes where classical calculations are less efficient. If QSs fulfill all of our four requirements, they may revolutionize our approach to quantum-mechanical problems, allowing to solve the behavior of complex Hamiltonians, and to design nano-scale materials and chemical compounds from the ground up.
Direct experimental access to some of the most intriguing quantum phenomena is not granted due to the lack of precise control of the relevant parameters in their naturally intricate environment. Their simulation on conventional computers is impossible, since quantum behaviour arising with superposition states or entanglement is not efficiently translatable into the classical language. However, one could gain deeper insight into complex quantum dynamics by experimentally simulating the quantum behaviour of interest in another quantum system, where the relevant parameters and interactions can be controlled and robust effects detected sufficiently well. Systems of trapped ions provide unique control of both the internal (electronic) and external (motional) degrees of freedom. The mutual Coulomb interaction between the ions allows for large interaction strengths at comparatively large mutual ion distances enabling individual control and readout. Systems of trapped ions therefore exhibit a prominent system in several physical disciplines, for example, quantum information processing or metrology. Here, we will give an overview of different trapping techniques of ions as well as implementations for coherent manipulation of their quantum states and discuss the related theoretical basics. We then report on the experimental and theoretical progress in simulating quantum many-body physics with trapped ions and present current approaches for scaling up to more ions and more-dimensional systems.