Propagation of a two-photon pulse in a waveguide coupled to a two-level system (TLS) is studied. The pulse is formed by two spatially separated identical wave packets. A set of equations governing the dynamics of the photon distribution in the configuration-momentum space is derived and solved. It is shown that the distribution function can be negative, which manifests its quasiprobability nature. A spectrum of the reflected light is found to be narrower than that of the transmitted light that features a pronounced filtering effect. Average numbers of the transmitted and reflected photons and their variances are shown to be dependent not only on the pulse widths and the light-TLS interaction but also on the pulse separation that can serve as an effective controlling parameter. Our approach is generalized for the case of an $n$-photon Fock state.
Propagation of a two-photon pulse in a waveguide coupled to a two-level system (TLS) is studied. The pulse is formed by two spatially separated identical wave packets. A set of equations governing the dynamics of the photon distribution in the configuration-momentum space is derived and solved. It is shown that the distribution function can be negative, which manifests its quasiprobability nature. A spectrum of the reflected light is found to be narrower than that of the transmitted light that features a pronounced filtering effect. Average numbers of the transmitted and reflected photons and their variances are shown to be dependent not only on the pulse widths and the light-TLS interaction but also on the pulse separation that can serve as an effective controlling parameter. Our approach is generalized for the case of an n-photon Fock state.
We investigate propagation of few-photon pulses in waveguides coupled to a two-level system by means of the method of distribution functions in coordinate-momentum space that provides a detailed description of photon systems. We find that the distribution function of the transmitted pulse can be negative for the nonclassical input (i.e., single-photon Fock state). This reveals the quasiprobability nature of photon distribution. Analytical expressions for photon densities in the momentum space as well as in the coordinate space are obtained for the mentioned single-photon Gaussian input. We also study the evolution of the multimode coherent-state input for an arbitrary photon number. Time-dependent differential equations describing average densities and fluctuations of outgoing photons are derived and solved. The influence of the number of input photons, pulse width, and radiation-atom interaction strength on the statistical properties of the fluctuations is investigated.
We present a time-dependent quantum calculation of the scattering of a few-photon pulse on a single atom. The photon wave packet is assumed to propagate in a transversely strongly confined geometry, which ensures strong atom-light coupling and allows a quasi-one-dimensional treatment. The amplitude and phase of the transmitted, reflected, and transversely scattered part of the wave packet strongly depend on the pulse length (bandwidth) and energy. For a transverse mode size of the order of ${\ensuremath{\lambda}}^{2},$ we find nonlinear behavior for a few photons already, or even for a single photon. In a second step we study the collision of two such wave packets at the atomic site and find striking differences between the Fock state and coherent state wave packets of the same photon number.
We present a detailed quantum theory and simulations of few-photon Fock state pulses interacting with a two-level system (TLS) in an open waveguide-QED system. For a rectangular pulse shape, we present an exact temporal scattering theory to derive analytical expressions for the TLS population, using one-photon and two-photon pulses, for both chiral and symmetric emitters. We also derive the stationary (long-time) and time-dependent spectra for one-photon excitation, and show how these differ at a fundamental level when considering TLS population effects. Numerically, we also present matrix product state (MPS) simulations, which allow us to compute more general photon correlation functions for arbitrary quantum pulses, and we use this approach to also show results for Gaussian quantum pulses and to confirm the accuracy of our analytical solutions. In the case of a chiral TLS, we show how a one-photon pulse, of any temporal shape, yields a transmitted long-time spectrum that is identical to the input pulse, despite significant TLS population effects. However, the dynamical spectra and spectral intensity show rich population effects, allowing for their detection in spectroscopic experiments. We also show the striking differences between one-photon and two-photon excitation, where the latter shows clear signatures of nonlinear saturation effects. In addition, we demonstrate how significant population TLS dynamics also occur for pulses that are relatively long compared to the radiative decay time (showing that a weak excitation approximation, which neglects finite TLS population effects, cannot be made) and investigate the population signatures, nonlinear features and dynamical behavior as a function of quantum pulse length.
We present a quantum dynamical study of pulsed few-photon scattering from a single artificial atom, consisting of a two-level system (TLS) or qubit, in a waveguide QED system, directly comparing and contrasting two different quantum theoretical simulation methods: (i) an input-output scattering approach that uses frequency-dependent scattering matrices, and (ii) a matrix product states (MPS) approach, which uses quantum noise operators in time bins and a tensor network technique to solve the time-dependent waveguide function for the entire system. Beginning with pulsed excitation using one-photon and two-photon Fock state pulses, we first show how to compute time-dependent observables with the scattering matrix approach, in terms of frequency integrals that encode the pulse spectrum, including how to extract the population dynamics of the excited quantum emitter, as well as the linear and nonlinear contributions. We present solutions for both symmetric and chiral TLS coupling. We then show how to compute the qubit and field observables in a more direct way using MPS, and obtain the characteristic bird-like shape for the two-photon correlation function at two times, which has been observed in recent experiments. We compare and contrast both of these methods, for one and two-photon excitation pulses, and show excellent agreement. We also present a study of the linear and nonlinear contributions, which can easily be calculated using scattering theory, and show the important role of pulse duration. Finally, we demonstrate the clear advantages of MPS by easily going to higher N-photon excitations, and show selected example population dynamics of up to eight-photon Fock-state pulses, manifesting in clear nonlinear population oscillations during the pulse interaction, similar to classical Rabi oscillations, but with quantum input fields that have a vanishing electric field expectation value.
In the paper, we employ a wave-function approach to investigate the evolution of a two-photon wave packet propagating in a one-dimensional waveguide coupled to the Jaynes-Cummings (JC) system. We derive and solve, both analytically and numerically, a set of equations of motion governing the quantum state of the system. That allows us to provide real-time analysis of the evolution of the wave packet two-photon joint spectrum (2PJS) and the excitation dynamics of the JC system in the course of its interaction with the two-photon pulse. We demonstrate that the 2PJS and the spectrum of the wave packet scattered from the JC system experience transformation for nonzero atom-cavity couplings. Moreover, using Schmidt decomposition, we show that the scattered photons feature frequency entanglement contrary to the incident ones which are not entangled.
We study the dynamics of a single-photon pulse travelling through a linear qubit chain coupled to continuum modes in a one-dimensional (1D) photonic waveguide. We derive a time-dependent dynamical theory for qubit amplitudes and for transmitted and reflected spectra. We show that the requirement for the photon-qubit coupling to exist only for positive frequencies can significantly change the dynamics of the system. First, it leads to an additional photon-mediated dipole-dipole interaction between qubits which results in the violation of the phase coherence between them. Second, the spectral lines of transmitted and reflected spectra crucially depend on the shape of the incident pulse and the initial distance between the pulse center and the first qubit in the chain. We apply our theory to one-qubit and two-qubit systems. For these two cases, we obtain the explicit expressions for the qubits' amplitudes and the photon radiation spectra as time tends to infinity. For the incident Gaussian wave packet we calculate the line shapes of transmitted and reflected photons.