We investigate propagation of few-photon pulses in waveguides coupled to a two-level system by means of the method of distribution functions in coordinate-momentum space that provides a detailed description of photon systems. We find that the distribution function of the transmitted pulse can be negative for the nonclassical input (i.e., single-photon Fock state). This reveals the quasiprobability nature of photon distribution. Analytical expressions for photon densities in the momentum space as well as in the coordinate space are obtained for the mentioned single-photon Gaussian input. We also study the evolution of the multimode coherent-state input for an arbitrary photon number. Time-dependent differential equations describing average densities and fluctuations of outgoing photons are derived and solved. The influence of the number of input photons, pulse width, and radiation-atom interaction strength on the statistical properties of the fluctuations is investigated.
We investigate propagation of few-photon pulses in waveguides coupled to a two-level system by means of the method of distribution functions in coordinate-momentum space that provides a detailed description of photon systems. We find that the distribution function of the transmitted pulse can be negative for the nonclassical input (i.e., single-photon Fock state). This reveals the quasiprobability nature of photon distribution. Analytical expressions for photon densities in the momentum space as well as in the coordinate space are obtained for the mentioned single-photon Gaussian input. We also study the evolution of the multimode coherent-state input for an arbitrary photon number. Time-dependent differential equations describing average densities and fluctuations of outgoing photons are derived and solved. The influence of the number of input photons, pulse width, and radiation-atom interaction strength on the statistical properties of the fluctuations is investigated.
Propagation of a two-photon pulse in a waveguide coupled to a two-level system (TLS) is studied. The pulse is formed by two spatially separated identical wave packets. A set of equations governing the dynamics of the photon distribution in the configuration-momentum space is derived and solved. It is shown that the distribution function can be negative, which manifests its quasiprobability nature. A spectrum of the reflected light is found to be narrower than that of the transmitted light that features a pronounced filtering effect. Average numbers of the transmitted and reflected photons and their variances are shown to be dependent not only on the pulse widths and the light-TLS interaction but also on the pulse separation that can serve as an effective controlling parameter. Our approach is generalized for the case of an n-photon Fock state.
We present a detailed quantum theory and simulations of few-photon Fock state pulses interacting with a two-level system (TLS) in an open waveguide-QED system. For a rectangular pulse shape, we present an exact temporal scattering theory to derive analytical expressions for the TLS population, using one-photon and two-photon pulses, for both chiral and symmetric emitters. We also derive the stationary (long-time) and time-dependent spectra for one-photon excitation, and show how these differ at a fundamental level when considering TLS population effects. Numerically, we also present matrix product state (MPS) simulations, which allow us to compute more general photon correlation functions for arbitrary quantum pulses, and we use this approach to also show results for Gaussian quantum pulses and to confirm the accuracy of our analytical solutions. In the case of a chiral TLS, we show how a one-photon pulse, of any temporal shape, yields a transmitted long-time spectrum that is identical to the input pulse, despite significant TLS population effects. However, the dynamical spectra and spectral intensity show rich population effects, allowing for their detection in spectroscopic experiments. We also show the striking differences between one-photon and two-photon excitation, where the latter shows clear signatures of nonlinear saturation effects. In addition, we demonstrate how significant population TLS dynamics also occur for pulses that are relatively long compared to the radiative decay time (showing that a weak excitation approximation, which neglects finite TLS population effects, cannot be made) and investigate the population signatures, nonlinear features and dynamical behavior as a function of quantum pulse length.
We present a quantum dynamical study of pulsed few-photon scattering from a single artificial atom, consisting of a two-level system (TLS) or qubit, in a waveguide QED system, directly comparing and contrasting two different quantum theoretical simulation methods: (i) an input-output scattering approach that uses frequency-dependent scattering matrices, and (ii) a matrix product states (MPS) approach, which uses quantum noise operators in time bins and a tensor network technique to solve the time-dependent waveguide function for the entire system. Beginning with pulsed excitation using one-photon and two-photon Fock state pulses, we first show how to compute time-dependent observables with the scattering matrix approach, in terms of frequency integrals that encode the pulse spectrum, including how to extract the population dynamics of the excited quantum emitter, as well as the linear and nonlinear contributions. We present solutions for both symmetric and chiral TLS coupling. We then show how to compute the qubit and field observables in a more direct way using MPS, and obtain the characteristic bird-like shape for the two-photon correlation function at two times, which has been observed in recent experiments. We compare and contrast both of these methods, for one and two-photon excitation pulses, and show excellent agreement. We also present a study of the linear and nonlinear contributions, which can easily be calculated using scattering theory, and show the important role of pulse duration. Finally, we demonstrate the clear advantages of MPS by easily going to higher N-photon excitations, and show selected example population dynamics of up to eight-photon Fock-state pulses, manifesting in clear nonlinear population oscillations during the pulse interaction, similar to classical Rabi oscillations, but with quantum input fields that have a vanishing electric field expectation value.
We present a full multimode treatment of the interaction of the quantized radiation field with a single two-level atom in a one-dimensional waveguide configuration. Starting with an incident pulse consisting of an arbitrary (finite) number of photons in a general initial state, we derive the equations of motion and a closed-form expression for the shape of the pulse after its interaction with the atom. We then specialize our results to the two-photon case where a number of analytical results can be derived, for both unidirectional and bidirectional systems. We study the effects of different pulse shapes, the manifestations of the entangled, so-called bound state of the two photons, single- and two-photon detection probabilities, and provide simple approximate results for the strong-coupling (or adiabatic, or long-pulse) regime. We also discuss the requirements for a true unidirectional setup, and the application of such a setup to photon sorting proposed by Witthaut, Lukin, and S\o{}rensen [Europhys. Lett. 97, 50007 (2012)].
In the paper, we employ a wave-function approach to investigate the evolution of a two-photon wave packet propagating in a one-dimensional waveguide coupled to the Jaynes-Cummings (JC) system. We derive and solve, both analytically and numerically, a set of equations of motion governing the quantum state of the system. That allows us to provide real-time analysis of the evolution of the wave packet two-photon joint spectrum (2PJS) and the excitation dynamics of the JC system in the course of its interaction with the two-photon pulse. We demonstrate that the 2PJS and the spectrum of the wave packet scattered from the JC system experience transformation for nonzero atom-cavity couplings. Moreover, using Schmidt decomposition, we show that the scattered photons feature frequency entanglement contrary to the incident ones which are not entangled.