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arXiv:1409.7993 · Physical Review Letters

Quantum Imaging by Coherent Enhancement

Guang Hao Low, Theodore J. Yoder, Isaac L. Chuang

Published Mar 11, 2015• 18 citations
arXivHTMLPDF

Abstract

Conventional wisdom dictates that to image the position of fluorescent atoms or molecules, one should stimulate as much emission and collect as many photons as possible. That is, in this classical case, it has always been assumed that the coherence time of the system should be made short, and that the statistical scaling ∼1/√t defines the resolution limit for imaging time t. However, here we show in contrast that given the same resources, a long coherence time permits a higher resolution image. In this quantum regime, we give a procedure for determining the position of a single two-level system and demonstrate that the standard errors of our position estimates scale at the Heisenberg limit as ∼1/t, a quadratic, and notably optimal, improvement over the classical case.

DOI
10.1103/physrevlett.114.100801

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Conventional wisdom dictates that to image the position of fluorescent atoms or molecules, one should stimulate as much emission and collect as many photons as possible. That is, in this classical case, it has always been assumed that the coherence time of the system should be made short, and that the statistical scaling ∼1/√t defines the resolution limit for imaging time t. However, here we show in contrast that given the same resources, a long coherence time permits a higher resolution image. In this quantum regime, we give a procedure for determining the position of a single two-level system and demonstrate that the standard errors of our position estimates scale at the Heisenberg limit as ∼1/t, a quadratic, and notably optimal, improvement over the classical case.
Classical imaging works by scattering photons from an object to be imaged, and achieves resolution scaling as 1/t1/\sqrt{t}1/t​, with ttt the imaging time. By contrast, the laws of quantum mechanics allow one to utilize quantum coherence to obtain imaging resolution that can scale as quickly as 1/t1/t1/t -- the so-called ``Heisenberg limit.'' However, ambiguities in the obtained signal often preclude taking full advantage of this quantum enhancement, while imaging techniques designed to be unambiguous often lose this optimal Heisenberg scaling. Here we demonstrate an imaging technique which combines unambiguous detection of the target with Heisenberg scaling of the resolution. We also demonstrate a binary search algorithm which can efficiently locate a coherent target using the technique, resolving a target trapped ion to within 0.3% of the 1/e21/{e}^{2}1/e2 diameter of the excitation beam.
Quantum imaging exploits the spatial correlations between photons to image object features with a higher resolution than a corresponding classical light source could achieve. Using a quantum correlated NNN-photon state, the method of optical centroid measurement (OCM) was shown to exhibit a resolution enhancement by improving the classical Rayleigh limit by a factor of 1/N1/N1/N. In this work, the theory of OCM is formulated within the framework of an imaging formalism and is implemented in an exemplary experiment by means of a conventional entangled photon pair source. The expected resolution enhancement of a factor of two is demonstrated. The here presented experiment allows for single-shot operation without scanning or iteration to reproduce the object in the image plane. Thereby, photon detection is performed with a newly developed integrated time-resolving detector array. Multi-photon interference effects responsible for the observed resolution enhancement are discussed and possible alternative implementation possibilities for higher photon number are proposed.
Quantum imaging exploits the spatial correlations between photons to image object features with a higher resolution than a corresponding classical light source could achieve. Using a quantum correlated N-photon state, the method of optical centroid measurement (OCM) was shown to exhibit a resolution enhancement by improving the classical Rayleigh limit by a factor of 1/N. In this work, the theory of OCM is formulated within the framework of an imaging formalism and is implemented in an exemplary experiment by means of a conventional entangled photon pair source. The expected resolution enhancement of a factor of two is demonstrated. The here presented experiment allows for single-shot operation without scanning or iteration to reproduce the object in the image plane. Thereby, photon detection is performed with a newly developed integrated time-resolving detector array. Multi-photon interference effects responsible for the observed resolution enhancement are discussed and possible alternative implementation possibilities for higher photon number are proposed.
High Resolution Image Download MS PowerPoint Slide The resolution of a classical imaging system is limited by diffraction. This limit can be overcome, for example, by implementing various forms of localization microscopy in which the center of a fluorescence distribution is estimated to an accuracy scaling with the square root of the number of detected photons, N . In quantum imaging the object can be illuminated using correlated photon-pairs, leading early work to suggest that a 2 improvement could be obtained as a result of averaging the position of N = 2 events. However, similar to quantum lithography, which relies upon quantum illumination using entangled photon-pairs and two-photon absorption, the minimum resolvable feature size is reduced by a factor of 2, not just 2 . Quantum imaging schemes can also lead to a factor of 2 improvement. By using a similar source of correlated photon-pairs to illuminate an object, a single-photon sensitive camera to detect the photon-pairs, and an image processing algorithm to record and sum the bisector positions of the transmitted photon-pairs, we realize a similar factor of ×2 improvement in image resolution, surpassing that of most earlier quantum imaging work.
The spatial resolution of an imaging apparatus is limited by the Rayleigh diffraction bound, a consequence of the imager's finite spatial extent. We show some NNN-photon strategies that permit resolution of details that are smaller than this bound, attaining either a 1∕N1∕\sqrt{N}1∕N​ enhancement (standard quantum limit) or a 1∕N1∕N1∕N enhancement (Heisenberg-like scaling) over standard techniques. In the incoherent imaging regime, the methods presented are loss resistant, since classical light sources suffice. Our results may be of importance in many applications: microscopy, telescopy, lithography, metrology, etc.
Motivated by the importance of optical microscopes to science and engineering, scientists have pondered for centuries how to improve their resolution and the existence of fundamental resolution limits. In recent years, a new class of microscopes that overcome a long-held belief about the resolution have revolutionized biological imaging. Termed "superresolution" microscopy, these techniques work by accurately locating optical point sources from far field. To investigate the fundamental localization limits, here I derive quantum lower bounds on the error of locating point sources in free space, taking full account of the quantum, nonparaxial, and vectoral nature of photons. These bounds are valid for any measurement technique, as long as it obeys quantum mechanics, and serve as general no-go theorems for the resolution of microscopes. To arrive at analytic results, I focus mainly on the cases of one and two classical monochromatic sources with an initial vacuum optical state. For one source, a lower bound on the root-mean-square position estimation error is on the order of λ0/Nλ_0/\sqrt{N}λ0​/N​, where λ0λ_0λ0​ is the free-space wavelength and NNN is the average number of radiated photons. For two sources, owing to the statistical effect of nuisance parameters, the error bound diverges when their radiated fields overlap significantly. The use of squeezed light to enhance further the accuracy of locating one classical point source and the localization limits for partially coherent sources and single-photon sources are also discussed. The presented theory establishes a rigorous quantum statiscal inference framework for the study of superresolution microscopy and points to the possibility of using quantum techniques for true resolution enhancement.