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arXiv:1408.3007 · Physical Review Letters

Hierarchy of Modes in an Interacting One-Dimensional System

Oleksandr Tsyplyatyev, A. J. Schofield, Yizheng Jin, M. Moreno, W. K. Tan, Christopher J. B. Ford, Jonathan P. Griffiths, Ian A. Farrer, Glenn A Jones, D. A. Ritchie

Published May 11, 2015• 22 citations
arXivHTMLPDF

Abstract

Studying interacting fermions in one dimension at high energy, we find a hierarchy in the spectral weights of the excitations theoretically, and we observe evidence for second-level excitations experimentally. Diagonalizing a model of fermions (without spin), we show that levels of the hierarchy are separated by powers of R^{2}/L^{2}, where R is a length scale related to interactions and L is the system length. The first-level (strongest) excitations form a mode with parabolic dispersion, like that of a renormalized single particle. The second-level excitations produce a singular power-law line shape to the first-level mode and multiple power laws at the spectral edge. We measure momentum-resolved tunneling of electrons (fermions with spin) from or to a wire formed within a GaAs heterostructure, which shows parabolic dispersion of the first-level mode and well-resolved spin-charge separation at low energy with appreciable interaction strength. We find structure resembling the second-level excitations, which dies away quite rapidly at high momentum.

DOI
10.1103/physrevlett.114.196401

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Studying interacting fermions in one dimension at high energy, we find a hierarchy in the spectral weights of the excitations theoretically, and we observe evidence for second-level excitations experimentally. Diagonalizing a model of fermions (without spin), we show that levels of the hierarchy are separated by powers of R^{2}/L^{2}, where R is a length scale related to interactions and L is the system length. The first-level (strongest) excitations form a mode with parabolic dispersion, like that of a renormalized single particle. The second-level excitations produce a singular power-law line shape to the first-level mode and multiple power laws at the spectral edge. We measure momentum-resolved tunneling of electrons (fermions with spin) from or to a wire formed within a GaAs heterostructure, which shows parabolic dispersion of the first-level mode and well-resolved spin-charge separation at low energy with appreciable interaction strength. We find structure resembling the second-level excitations, which dies away quite rapidly at high momentum.
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An electron is usually considered to have only one form of kinetic energy, but could it have more, for its spin and charge, by exciting other electrons? In one dimension (1D), the physics of interacting electrons is captured well at low energies by the Tomonaga-Luttinger model, yet little has been observed experimentally beyond this linear regime. Here, we report on measurements of many-body modes in 1D gated wires using tunneling spectroscopy. We observe two parabolic dispersions, indicative of separate Fermi seas at high energies, associated with spin and charge excitations, together with the emergence of two additional 1D "replica" modes that strengthen with decreasing wire length. The interaction strength is varied by changing the amount of 1D intersubband screening by more than 45%. Our findings not only demonstrate the existence of spin-charge separation in the whole energy band outside the low-energy limit of the Tomonaga-Luttinger model but also set a constraint on the validity of the newer nonlinear Tomonaga-Luttinger theory.
The properties of fermions in one dimension are markedly different from those in higher dimensions. In two or three dimensions, the many-body behaviour of fermions is described by the Fermi liquid model, whose most prominent result is that, instead of studying the behaviour of individual particles, it is better to describe the emergent phenomena of the whole system, known as quasiparticles. These are collective modes of excitations born out of particle-particle interactions, which resemble the constituent single particles, albeit with renormalised mass. In one dimension, however, the formation of such a correlated state is unfavourable and the quasiparticles are completely absent. Instead, 1D fermions are described by a model known as the Tomonaga-Luttinger liquid. Central to this model is the process of bosonisation, a mathematical technique which maps the excitation of fermions to bosonic modes of spin-density and charge-density waves. As a prerequisite of the bosonisation technique, the fermionic single-particle dispersion is approximated as a linear function. Consequently, the Luttinger liquid model is limited in its scope of applicability. Specifically, it is valid only in the vicinity of the Fermi points, where the excitation energy is low. Recent advancement in the theoretical field has expanded our understanding of 1D interacting fermions beyond the limit of linearity. The mobile-impurity model, proposed by L. Glazman and his co-authors, is a generalised model of 1D fermions which extends the scope of applicability of the Tomanaga-Luttinger model, accounting for the curvature of single-particle dispersion relations. It extends the region of validity of the tradition TLL theory from the neighbourhood of the Fermi points to a band which follows the single-particle dispersion. This thesis presents the results of an experimental work which provides direct evidence of non-linear behaviour predicted by the new model. It revolves around the measurement of the spectral function of electrons in surface-gate-defined quantum wires on a double-quantum-well, GaAs/AlGaAs device, and the comparison and fitting of the result to the non-linear theory. The spectral function is a theoretical concept frequently used in discussions on many-body problems. Its physical interpretation makes it closely related to experimental observables, such as the tunnelling current between the double quantum wells in this work. This thesis consists of three parts. Part one concerns the theories of the various many-body models and the experimental technique: Chapter 1 briefly introduces the concept of Fermi liquid, before focusing on a detailed account of the Luttinger-liquid model. The mobile-impurity model will be introduced in the framework of the Luttinger liquid model afterwards, followed by a review of experimental works reported in the literature on the study of TLL physics. In Chapter 2, the principles of the experimental tunnelling spectroscopy technique are described. The second part of the thesis details the structure of the test device used in the experiment and its fabrication. In particular, we will discuss the intricacies of the three-dimensional EBL fabrication process developed specifically for this project. The setup and running of the measurement circuit will also be discussed in this part of the thesis, in the context of a prerequisite sample characterisation measurement. In the final part of the work, data from the main experiment will be presented and analysed, in search for the electron-electron interaction effects which are predicted by the theoretical discussions in the first chapter.
A continuum of excitations in interacting one-dimensional systems is bounded from below by a spectral edge that marks the lowest possible excitation energy for a given momentum. We analyze short-range interactions between Fermi particles and between Bose particles (with and without spin) using Bethe-ansatz techniques and find that the dispersions of the corresponding spectral edge modes are close to a parabola in all cases. Based on this emergent phenomenon we propose an empirical model of a free, nonrelativistic particle with an effective mass identified at low energies as the bare electron mass renormalized by the dimensionless Luttinger parameter KKK (or ${K}_{\ensuremath{\sigma}}$ for particles with spin). The relevance of the Luttinger parameters beyond the low-energy limit provides a more robust method for extracting them experimentally using a much wider range of data from the bottom of the one-dimensional band to the Fermi energy. The empirical model of the spectral edge mode complements the mobile impurity model to give a description of the excitations in proximity of the edge at arbitrary momenta in terms of only the low-energy parameters and the bare electron mass. Within such a framework, for example, exponents of the spectral function are expressed explicitly in terms of only a few Luttinger parameters.
We compute the spectral function rho (q, omega ) of the one-dimensional Luttinger model. We discuss the distinct influences of charge-spin separation and of the anomalous dimensions of the fermion operators and their evolution with correlation strength. Charge-spin separation shows up in finite spectral weight at frequencies between v sigma q and v rho q, where v sigma and v rho are the velocities of spin and charge fluctuations, while spectral weight above v rho q and below -v rho q is generated by the hybridization of the Fermi surface at +or-k F by interactions. There are non-universal power-law singularities at these special frequencies. We discuss the consistency of recent photoemission experiments on low-dimensional conductors with a Luttinger-liquid picture, which then would suggest very strong long-range interactions. It is pointed out that many-particle correlation functions in principle exhibit similar singularities, but they probe different and complementary aspects of the Fermi-surface interactions.
Interactions between electrons in one dimension are fully described at low energies by only a few parameters of the Tomonaga-Luttinger model, which is based on linearization of the spectrum. We consider a model of spinless fermions with short-range interaction via the Bethe-Ansatz technique and show that a Luttinger parameter emerges in an observable beyond the low-energy limit. A distinct feature of the spectral function, the edge that marks the lowest possible excitation energy for a given momentum, is parabolic for arbitrary momenta and the prefactor is a function of the Luttinger parameter, KKK.