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arXiv:1408.1415 · European Journal of Mass Spectrometry

Trapped Ion Chain Thermometry and Mass Spectrometry through Imaging

Vaishnavi Rajagopal, Joan P. Marler, Mark Kokish, Brian Odom

Published Feb 1, 2016• 16 citations
arXivHTMLPDF

Abstract

We demonstrate a spatial-imaging thermometry technique for ions in a one-dimensional Coulomb crystal by relating their imaged spatial extent along the linear radiofrequency ion trap axis to normal modes of vibration of coupled oscillators in a harmonic potential. We also use the thermal spatial spread of "bright" ions in the case of a two-species mixed chain to measure the center-of-mass resonance frequency of the entire chain and infer the molecular composition of the co-trapped "dark" ions. These non-destructive techniques create new possibilities for better understanding of sympathetic cooling in mixed-ion chains, improving few-ion mass spectrometry, and trapped-ion thermometry without requiring a scan of Doppler cooling parameters.

DOI
10.1255/ejms.1408

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We demonstrate a spatial-imaging thermometry technique for ions in a one-dimensional Coulomb crystal by relating their imaged spatial extent along the linear radiofrequency ion trap axis to normal modes of vibration of coupled oscillators in a harmonic potential. We also use the thermal spatial spread of "bright" ions in the case of a two-species mixed chain to measure the center-of-mass resonance frequency of the entire chain and infer the molecular composition of the co-trapped "dark" ions. These non-destructive techniques create new possibilities for better understanding of sympathetic cooling in mixed-ion chains, improving few-ion mass spectrometry, and trapped-ion thermometry without requiring a scan of Doppler cooling parameters.
We report on observations of the thermal motion of a single, Doppler-cooled ion along the axis of a linear radio-frequency quadrupole trap. We show that for a harmonic potential the thermal occupation of energy levels leads to a Gaussian distribution of the ion's axial position. The dependence of the spatial thermal spread on the trap potential is used for precise calibration of our imaging system's point spread function and sub-millikelvin thermometry. We employ this technique to investigate the laser detuning dependence of the Doppler temperature.
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We describe our work on trapping, cooling and detecting mixed ion species for a scalable ion trap quantum information processing architecture. These mixed species chains in linear RF traps may help solve several problems with scaling ion trap quantum computation to large numbers of qubits. Initial temperature measurements of linear Coulomb crystals containing barium and ytterbium ions indicate that the mass difference does not significantly impede sympathetic cooling of normal modes that couple well to the coolant ions (Ba in our case). Average motional occupation numbers are estimated to be 10 to 20 quanta per mode for these well cooled modes for chains with small numbers of ions, consistent with the Doppler limit temperature. For normal modes that do not couple significantly to the coolant atoms, the occupation numbers are significantly higher, of order several thousand. Strategies for better cooling of these modes are discussed. Further, we are working to implement these techniques in microfabricated surface traps in order to exercise greater control over ion chain ordering and positioning.
Coulomb crystals of cold trapped ions are a leading platform for the realization of quantum processors and quantum simulations and, in quantum metrology, for the construction of optical atomic clocks and for fundamental tests of the standard model. For these applications, it is not only essential to cool the ion crystal in all its degrees of freedom down to the quantum ground state but also to be able to determine its temperature with a high accuracy. However, when a large ground-state cooled crystal is interrogated for thermometry, complex many-body interactions take place, making it challenging to accurately estimate the temperature with established techniques. In this work, we present a new thermometry method tailored for ion crystals. The method is applicable to all normal modes of motion and does not suffer from a computational bottleneck when applied to large ion crystals. We test the temperature estimate with two experiments, namely with a one-dimensional linear chain of four ions and a two-dimensional crystal of 19 ions and verify the results, where possible, using other methods. The results show that the new method is an accurate and efficient tool for thermometry of ion crystals.
This thesis reports on the setup of a new ion trap apparatus designed for experiments with single ⁴⁰Ca⁺ ions to perform molecular spectroscopy. The calcium ion is laser cooled, allowing for sympathetic cooling of the nonfluorescing molecular ion. The aim of these experiments is to explore loading and identifying molecular ions in RF-Paul traps, as well as developing new spectroscopic tools to measure transitions of molecular ions via the fluorescence of co-trapped ⁴⁰Ca⁺ ions. Ground state cooling of a mixed ion pair is implemented as a first step towards increasing the sensitivity of our technique to the level necessary to measure transitions with low scattering rates (like those present in molecular ions). Doppler cooling on the S(1/2)->P(1/2) transition of the calcium ion results in the formation of a Coulomb crystal, the behavior of which may be used to infer properties of the molecular ion. Following cooling, sideband spectroscopy on the narrow S(1/2)->D(5/2) quadrupole transition of calcium may be used to identify the mass of single molecular ions. This method is verified via a non-destructive measurement on ⁴⁰CaH⁺ and ⁴⁰Ca¹⁶O⁺. The normal modes of the Coulomb crystal can also be used to extract information from the target ion to the control ion. By driving the blue side of a transition, laser induced heating can be put into the two ion system, which leads to changes in fluorescence of the ⁴⁰Ca⁺ ion, first demonstrated with two Ca⁺ isotopes. Increasing the sensitivity of this technique requires ground state cooling of both the ⁴⁰Ca⁺ ion and the ion of interest, enabling the transfer of the ion's motional state into the ground state with high probability. This thesis demonstrates ground state cooling of the atomic ion and sympathetic cooling of a second ion (⁴⁴Ca⁺). Once in the ground state, heating of the Coulomb crystal by scattering photons off of the spectroscopy ion can be measured by monitoring the resolved motional sidebands of the S(1/2)->D(5/2) transition of ⁴⁰Ca⁺, allowing for spectral lines to be inferred. Future experiments will investigate this technique with molecular ions.
Coulomb crystals of cold trapped ions are a leading platform for the realization of quantum processors and quantum simulations and, in quantum metrology, for the construction of optical atomic clocks and for fundamental tests of the standard model.For these applications, it is not only essential to cool the ion crystal in all its degrees of freedom down to the quantum ground state but also to be able to determine its temperature with a high accuracy.However, when a large ground-state cooled crystal is interrogated for thermometry, complex many-body interactions take place, making it challenging to accurately estimate the temperature with established techniques.In this work, we present a new thermometry method tailored for ion crystals.The method is applicable to all normal modes of motion and does not suffer from a computational bottleneck when applied to large ion crystals.We test the temperature estimate with two experiments, namely with a one-dimensional linear chain of four ions and a two-dimensional crystal of 19 ions and verify the results, where possible, using other methods.The results show that the new method is an accurate and efficient tool for thermometry of ion crystals.