Many areas of physics rely upon adiabatic state transfer protocols, allowing a quantum state to be moved between different physical systems for storage and retrieval or state manipulation. However, these state-transfer protocols suffer from dephasing and dissipation. In this thesis we go beyond the standard open-systems treatment of quantum dissipation allowing us to consider non-Markovian environments. We use adiabatic perturbation theory in order to give analytic descriptions for various quantum state-transfer protocols. The leading-order corrections will give rise to additional terms adding to the geometric phase preventing us from achieving a perfect fidelity. We obtain analytical descriptions for the effects of the geometric phase in non-Markovian regimes. The Markovian regime is usually treated by solving a standard Bloch-Redfield master equation, while in the non-Markovian regime, we perform a secular approximation allowing us to obtain a solution to the density matrix without solving master equations. This solution contains all the relevant phase information for our state-transfer protocol. After developing the general theoretical tools, we apply our methods to adiabatic state transfer between a four-level atom in a driven cavity. We explicitly consider dephasing effects due to unavoidable photon shot noise and give a protocol for performing a phase gate. These results will be useful to ongoing experiments in circuit quantum electrodynamics (QED) systems.
Many areas of physics rely upon adiabatic state transfer protocols, allowing a quantum state to be moved between different physical systems for storage and retrieval or state manipulation. However, these state-transfer protocols suffer from dephasing and dissipation. In this thesis we go beyond the standard open-systems treatment of quantum dissipation allowing us to consider non-Markovian environments. We use adiabatic perturbation theory in order to give analytic descriptions for various quantum state-transfer protocols. The leading-order corrections will give rise to additional terms adding to the geometric phase preventing us from achieving a perfect fidelity. We obtain analytical descriptions for the effects of the geometric phase in non-Markovian regimes. The Markovian regime is usually treated by solving a standard Bloch-Redfield master equation, while in the non-Markovian regime, we perform a secular approximation allowing us to obtain a solution to the density matrix without solving master equations. This solution contains all the relevant phase information for our state-transfer protocol. After developing the general theoretical tools, we apply our methods to adiabatic state transfer between a four-level atom in a driven cavity. We explicitly consider dephasing effects due to unavoidable photon shot noise and give a protocol for performing a phase gate. These results will be useful to ongoing experiments in circuit quantum electrodynamics (QED) systems.
In the first part of this thesis, we investigate the dynamics of open quantum systems coupled in a purely dephasing way to their environment, which is a paradigmatic example of decoherent dynamics. We focus more specifically on the emergence of non-Markovian effects in the dynamics of such open systems. After reviewing different measures of non-Markovianity, we obtain an analytical expression for the reduced density operator of a finite-dimensional open system coupled with its environment through time-dependent purely dephasing interactions. When the system is initially uncorrelated with its environment, we obtain the time-local master equation that describes its dynamics. In this case, we also derive an exact expression for the witness of non-Markovianity based on the volume of accessible states of the open system. These results are then applied to spin systems coupled to either a spin or a bosonic environment. For spin environments, we study non-Markovianity for different ranges of interaction and in different thermodynamical limits. Moreover, the generation of entanglement between the open system and its environment as well as between spins within the open system is investigated. For bosonic environments, we study the effect of the initial state of the environment on non-Markovianity. We also show that time-dependent modulations of the system-environment coupling can dramatically alter the non-Markovian behavior of the open system. Finally, we consider the case of an open quantum system simultaneously coupled to spin and bosonic baths. In that case, we study how the coupling between the different baths and of the presence of initial correlations in the environment affect the non-Markovianity displayed by the open quantum system. The second part of this thesis is a contribution to the investigation of how quantum systems can be used to process information. More precisely, we focus on the implementation of gate-based quantum computing using neutral atoms trapped in optical or magnetic lattices and interacting through dipole-dipole interactions when excited to Rydberg states. In this context, we present protocols implementing two-qubit quantum gates between atoms far apart in the lattice. To this end, we propose to use a chain of non-coding ancilla atoms to transfer the state of the control qubit to an atom near the target qubit. Before discussing entangling gates between distant qubits, we present two protocols that implement state transfer along a chain of two-level atoms relying respectively on single- and two-atom laser pulses combined with dipole blockade. After reviewing protocols implementing CZ and CNOT gates between nearby qubits using dipole-dipole interactions, we show how the state-transfer protocols previously presented can be used to perform entangling gates between distant qubits. The performance of the state-transfer and gate protocols are assessed using the process fidelity. Moreover, we provide a theoretical explanation for the behavior of the process fidelity with respect to dissipation and imperfect blockade.
Quantum mechanics has both deepened our understanding of the physical reality and allowed development of quantum technologies beating their classical counterparts in efficiency, security, and sensitivity. As a major downside, the quantum properties behind these technologies are very sensitive to the effects the system’s interaction with its environment. The theory of open quantum systems describes how such interaction influences the system, and as a consequence, how the quantum features are lost, controlled, and possibly returned by manipulating the environment. This thesis begins with a short description of the most relevant features and results of the open quantum system theory. We continue by presenting some commonly used measures to quantify the information encoded in quantum systems and the correlations between spatially or temporally separated parties. The literature review ends with discussion of non-Markovianity and memory effects which combine the fields of open quantum systems and quantum information in a natural way. The rest of the thesis presents the main results of Publications I – VII. We study the memory effects and physicality conditions of open system dynamics described by the vast family of phase-covariant master equations. We show how the open quantum system picture can be exploited to design probing protocols to extract information without knowing how the probe and system interact. Such protocols are considered also from the point-of view of efficiently obtaining the information required in the probing, both in theory and by experimental implementation. The experiment serves also as evidence for applicability of recently developed geometric tools to design informationally incomplete measurements for solving so-called membership problems. We present and experimentally realize a protocol where control over intial correlations between polarization and frequency gives full freedom to implement any dephasing dynamics in the open system polarization, thus dictating how its information content changes in time. We study the two-qubit memory effects of dephasing dynamics and compare them to the effect of such noise in the transmission efficiency in superdense coding. Optimal noise configurations in different situations are found. Finally, we characterize the families of initial states for which the decay of quantum correlations depends or does not depend on the noise location.
An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..
We introduce an alternative way to derive the generalized form of the master equation recently presented by J. P. Pekola et al. [Phys. Rev. Lett. 105, 030401 (2010)] for an adiabatically steered two-level quantum system interacting with a Markovian environment. The original derivation employed the effective Hamiltonian in the adiabatic basis with the standard interaction picture approach but without the usual secular approximation. Our approach is based on utilizing a master equation for a nonsteered system in the first superadiabatic basis. It is potentially efficient in obtaining higher-order equations. Furthermore, we show how to select the phases of the adiabatic eigenstates to minimize the local adiabatic parameter and how this selection leads to states which are invariant under a local gauge change. We also discuss the effects of the adiabatic noncyclic geometric phase on the master equation.
A three-level atom in a Λ configuration trapped in an optical cavity forms a basic unit in a number of proposed protocols for quantum information processing. Through control with an appropriate laser, this system allows for efficient storage of cavity photons into long-lived atomic excitations, and their retrieval with high fidelity. This process presumes an adiabatic transfer through the `dark state', a coherent superposition of the two lower levels of the Λ system, by a slow variation of the intensity of the control laser. We study the full quantum mechanics of this transfer process with a view to examine the nonadiabatic effects, as the control laser is varied in time. The nonadiabatic effects arise due to inevitable excitations of the system to states involving the highest level of the Λ configuration, which is radiative. We formulate the problem in terms of the instantaneous eigenstates and solve it numerically, allowing for spontaneous decays from the excited level. We present detailed results for both storage and retrieval for a suitable range of variation rates and intensity of the control laser, and examine optimum conditions for the transfer process.
Accurate control of a quantum system is complicated to achieve partly due to the system being coupled to its surrounding environment. The coupling induces dissipation and decoherence not only destroying the coherent quantum state but making the application of control unpredictable. When the control results from manipulation of external fields, it is usually referred to as driving and its joint effect with decoherence constitutes an active field of study in reduced-density-operator theory. Recently, this field has been pushed forward by its necessity in simulating Cooper pair pumping where the geometric nature of quantum evolution allows for controlled transport of charge carriers in superconducting circuits. Such circuits themselves are under constant investigation as they grant access to fundamental quantum phenomena and facilitate promising applications such as those in quantum information processing.\nIn this dissertation, driven quantum systems under decoherence are investigated. Extensions and improvements to a recent master equation for nearly adiabatic driving are presented and analyzed. The emergent properties in quantum evolution are studied both analytically and numerically. Related to the findings, a general conservation law of operator current is derived and used to explain observed nonconservation in previous theoretical studies. The derived theory is applied to Cooper-pair pumping and shown to lead to important properties such as superadiabatic ground-state pumping. A recent pumping experiment is simulated and the breakdown point for ideal pumping is found with feasible physical parameters. A study of charge transport in the presence of flux noise is presented leading to detectable dissipative currents and the typical description of the device used for pumping is extended to include a nonvanishing loop inductance.\nA novel approach to implement control of quantum systems is proposed based on constructing a tunable coupling to an artificial environment using either a coplanar waveguide cavity or coupled quantum LC resonators. Tunability allowing for both efficient initialization and protected evolution is theoretically demonstrated. Finally, a general framework for quantum driving is constructed without the typical assumption of a classical driving force leading to peculiar results.\nThis dissertation presents original research on both modeling the control of open quantum systems as well as the realization of such control. The work simulates physical phenomena in superconducting circuits and makes predictions for future experiments. In addition, it introduces novel theoretical tools and approaches that advance the state of the art.