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arXiv:1407.0431 · New Journal of Physics

Radio-frequency spectrum of the Feshbach molecular state to deeply bound molecular states in ultracold40K Fermi gases

Lianghui Huang, Pengjun Wang, Brandon Ruzic, Zhengkun Fu, Zengming Meng, Peng Peng, John L. Bohn, Jing Zhang

Published Mar 3, 2015• 4 citations
arXivHTMLPDF

Abstract

Spectroscopic measurements are made and obtained for three molecular levels within 50 MHz of the atomic continuum, along with their variation of magnetic field in ultracold 40 K Fermi gases. We use spectroscopic measurements to modify the scattering properties near magnetic Fano–Feshbach resonances with a radio-frequency (RF) field by measuring the loss profile versus magnetic field. This work provides the high accuracy locations of ground molecular states near the s-wave Fano–Feshbach resonance, which can be used to study the crossover regime from a Bose–Einstein condensate to a Bardeen–Cooper–Schrieffer superfluid in the presence of an RF field.

DOI
10.1088/1367-2630/17/3/033013

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Chinese Physics B•Jan 1, 2014•6 citations
Spectroscopic measurements are made and obtained for three molecular levels within 50 MHz of the atomic continuum, along with their variation of magnetic field in ultracold 40 K Fermi gases. We use spectroscopic measurements to modify the scattering properties near magnetic Fano–Feshbach resonances with a radio-frequency (RF) field by measuring the loss profile versus magnetic field. This work provides the high accuracy locations of ground molecular states near the s-wave Fano–Feshbach resonance, which can be used to study the crossover regime from a Bose–Einstein condensate to a Bardeen–Cooper–Schrieffer superfluid in the presence of an RF field.
We use laser light near resonant with a molecular bound-to-bound transition to control a magnetic Feshbach resonance in ultracold Fermi gases of 40{}^{40}40K atoms. The spectrum of excited molecular states is measured by applying a laser field that couples the ground Feshbach molecular state to electronically excited molecular states. Nine strong bound-to-bound resonances are observed below the 2P1/2+2S1/2{}^{2}{P}_{1/2}+{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}2P1/2​+2S1/2​ threshold. We use radio-frequency spectroscopy to characterize the laser-dressed bound state near a specific bound-to-bound resonance and show clearly the shift of the magnetic Feshbach resonance using light. The demonstrated technology could be used to modify interatomic interactions with high spatial and temporal resolutions in the crossover regime from a Bose-Einstein condensate to a Bardeen-Cooper-Schrieffer superfluid.
The use of Feshbach resonances in the field of ultracold gases has received a lot of attention recently. In first instance it was realized that these resonances can be used to alter the interaction strength in an atomic gas, by means of tuning an external magnetic field. Furthermore, by sweeping the magnetic field from one side of the resonance to the other, a degenerate gas of bosonic molecules can be created, a significant accomplishment. By making the interactions between fermionic atoms strongly attractive, a fermionic superfluid was recently made, a feat that has drawn a lot of attention in the physics community and from the media. We present work that describes these many-particle systems near a Feshbach resonance in a comprehensive way by using the concept of dressed molecules. These dressed molecules are essentially two-particle states that are a superposition of a tightly bound bare molecule, and two unbound bare atoms. This description reduces to the correct paired wave-function in the two-body limit. Moreover it gives a physically correct description of all the phenomena mentioned above: the Bose-condensation of a gas near a Feshbach resonance, that contains molecules, is more correctly interpreted as a Bose-condensation of dressed molecules. The fermionic superfluid contains a condensate of bosonic pairs, normally called Cooper pairs, that can be understood as the dressed molecules. For the latter case, the dressed-molecule picture also gives an elegant characterization of the crossover between a Bose condensate of pure molecules on one side of the resonance, to a fermionic Bardeen-Cooper-Schrieffer superfluid on the other side. Then, the dressed molecules change continuously from being mostly a bare molecule, to being mostly a loose pair of two atoms. It is clear that the nature of the dressed molecules is much determined by the probability for it to be in the bare-molecular state. This probability we denote with a single parameter Z. We present various ways of calculating it, and study how it affects the macroscopic physics.
A trapped Fermi gas near a collisional resonance provides a unique laboratory for testing many-body theories in a variety of fields. The ultracold Fermi gas produced in our lab is comprised of the lowest two spin states of 6^66Li. At 834 G there is a collisional or Feshbach resonance between the two spin states. The scattering length between trapped atoms of opposing spins far exceeds the interparticle spacing of the gas. On resonance, a strongly interacting, unitary, Fermi gas is created which exhibits universal behavior. The unitary Fermi gas is a prototype for other exotic systems in nature from nuclear matter to neutron stars and high temperature superconductors. \n For magnetic fields less than 834 G the scattering length is positive, and pairs Fermi atoms can form molecular dimers. These dimers, comprised of two fermions, are bosons. At ultracold temperatures the molecular bosons populate the lowest energy level and form a Bose Einstein Condensate (BEC). For magnetic fields greater than 834G the scattering length between fermions in opposing spin states is negative, like Cooper pairs formed between electrons in a superconductor. The Bardeen, Cooper, and Shriefer (BCS) theory was developed to describe the pairing effect in the context of superconductors. In our experiment we produce an ultracold unitary gas. By tuning the magnetic field to either side of the Feshbach resonance we can transform the gas into a weakly interacting BEC or BCS superfluid. Therefore, the region near a Feshbach resonance is called the BEC-BCS crossover. \n This dissertation presents a precision measurement of the hydrodynamic sound velocity in an ultracold Fermi gas near a Feshbach resonance. The sound velocity is measured at various magnetic fields both above and below resonance. Moreover, we are able compare our measurements to theoretical descriptions of hydrodynamic sound propagation. Further, our measurement of sound velocity exactly reproduces the non-perturbative case, eliminating the need to consider nonlinear effects. At resonance the sound velocity exhibits universal scaling with the Fermi velocity to within 1.8\\% over a factor of 30 in density. In a near zero temperature unitary gas the average sound velocity at the axial center was measured, c(0)/vFc(0)/v_Fc(0)/vF​ = 0.364(0.005), as well as the universal constant, beta\\betabeta = -0.565(0.015). The measurement of sound velocity in an ultracold gas throughout the BEC-BCS crossover provides further evidence of the continuous connection between the physics of the BEC, unitary, and BCS systems.
We have observed and located more than 60 magnetic field-induced Feshbach resonances in ultracold collisions of ground-state 133Cs^{133}\mathrm{Cs}133Cs atoms. Multiple extremely weak Feshbach resonances associated with ggg-wave molecular states are detected through variations in the radiative collision cross sections. The Feshbach spectroscopy allows us to determine the interactions between ultracold cesium atoms and the molecular energy structure near the dissociation continuum with unprecedented precision. Our work not only represents a very successful collaboration of experimental and theoretical efforts, but also provides essential information for cesium Bose-Einstein condensation, Cs2{\mathrm{Cs}}_{2}Cs2​ molecules, and atomic clock experiments.
We study the superfluid state of atomic Fermi gases using a BCS-Bose-Einstein-condensation crossover theory. Our approach emphasizes noncondensed fermion pairs which strongly hybridize with their (Feshbach-induced) molecular boson counterparts. These pairs lead to pseudogap effects above Tc{T}_{c}Tc​ and non-BCS characteristics below. We discuss how these effects influence the experimental signatures of superfluidity.
We create weakly bound Feshbach molecules in ultracold Fermi gas 40 K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency (RF) technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.