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arXiv:1405.1470 · New Journal of Physics

Interfacing GHz-bandwidth heralded single photons with a warm vapour Raman memory

Patrick Michelberger, T. F. M. Champion, Michael Sprague, K. T. Kaczmarek, Marco Barbieri, Xian‐Min Jin, Duncan G. England, W. Steven Kolthammer, D. J. Saunders, J. Nunn, Ian A. Walmsley

Published Apr 2, 2015• 102 citations
arXivHTMLPDF

Abstract

Broadband quantum memories, used as temporal multiplexers, are a key component in photonic quantum information processing, as they make repeat-until-success strategies scalable. We demonstrate a prototype system, operating on-demand, by interfacing a warm vapour, high time-bandwidth-product Raman memory with a travelling wave spontaneous parametric down-conversion source. We store single photons and observe a clear influence of the input photon statistics on the retrieved light, which we find currently to be limited by noise. We develop a theoretical model that identifies four-wave mixing as the sole important noise source and point towards practical solutions for noise-free operation.

DOI
10.1088/1367-2630/17/4/043006

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Broadband quantum memories, used as temporal multiplexers, are a key component in photonic quantum information processing, as they make repeat-until-success strategies scalable. We demonstrate a prototype system, operating on-demand, by interfacing a warm vapour, high time-bandwidth-product Raman memory with a travelling wave spontaneous parametric down-conversion source. We store single photons and observe a clear influence of the input photon statistics on the retrieved light, which we find currently to be limited by noise. We develop a theoretical model that identifies four-wave mixing as the sole important noise source and point towards practical solutions for noise-free operation.
Quantum memories are key components in quantum information networks. Their ability to store and retrieve information on demand makes repeat-until-success strategies scalable. Warm alkali-metal vapours are interesting candidates for the implementation of such memories, thanks to their long storage times and experimental simplicity. Operation with the Raman protocol enables high time-bandwidth products, which allows for multiple synchronisation trials of probabilistically operating quantum gates via memory-based temporal multiplexing. This makes the Raman memory a promising tool, whose broad spectral bandwidth facilitates direct interfacing with other photonic primitives, such as single photon sources. Here, such a light-matter interface is implemented in a warm caesium vapour. Firstly, we study the storage of polarisation-encoded information in the memory. High quality polarisation preservation for bright coherent state input signals can be achieved, when operating the Raman memory in a dual-rail configuration inside a polarisation interferometer. Secondly, heralded single photons are stored in the memory. To this end, the memory is operated on-demand by feed-forward of source heralding events, which is a key technological capability. Prior to storage, single photons are produced in a spontaneous parametric down conversion source, whose bespoke design spectrally tailors the photons to the memory acceptance line. The faithful retrieval of stored single photons is found to be currently limited by noise in the memory, with a signal-to-noise ratio of 0.3 in the memory output. Nevertheless, a clear influence of the input's quantum nature is observed in the retrieved light by measuring signal's photon statistics. Finally, the memory noise processes are examined in detail. Four-wave-mixing noise is determined as the sole important noise source for the Raman memory.
Photonics offers a route to fast and distributed quantum computing in ambient conditions, provided that photon sources and logic gates can be operated deterministically. Quantum memories, capable of storing and re-emitting photons on demand, enable quasi-deterministic operations by synchronising stochastic events. We recently interfaced a Raman-type quantum memory with a travelling-wave heralded photon source. Here we discuss the trade-space for the spectral characteristics of such sources, and we present measurements of our source, which represents a practical compromise enabling passive stability, high brightness in a single-pass configuration, high purity and good matching to our Cs vapour memory.
Photonics offers a route to fast and distributed quantum computing in ambient conditions, provided that photon sources and logic gates can be operated deterministically. Quantum memories, capable of storing and re-emitting photons on demand, enable quasi-deterministic operations by synchronizing stochastic events. Interfaced source–memory systems are thus a key building block in photonics-based quantum information processors. We discuss the design of the single-photon source in this type of light–matter interface and present an experimental system based on a Raman-type quantum memory. In addition to the spectral purity of the produced heralded single photons, we find that their temporal distinguishability also becomes important due to the implicit temporal binning derived from photon storage in the memory. When aiming to operate the source–memory system at high repetition rates, a practical compromise between both of these requirements needs to be found. Our implemented photon source system demonstrates such a solution and enables passive stability, high brightness in a single-pass configuration, high purity as well as good mode matching to our Raman memory.
Photonic quantum information processing has emerged as a powerful platform for realising quantum-enhanced technologies. In order to be scalable, many of these technologies depend on the availability of a suitable quantum memory for the coherent storage and on-demand retrieval of photonic quantum states. In this thesis, I investigate broadband light storage in a room-temperature Raman memory, implemented both in free space and, for the first time, inside a low-finesse optical cavity designed for low-noise operation. The ability of the Raman memory to preserve phase coherence was tested by storing coherent polarisation states in two spatially separate atomic ensembles. Polarisation storage with a fidelity of up to 97 ± 1% was demonstrated by performing full process tomography on the system. The Raman memory was then interfaced for the first time with a spontaneous parametric downconversion (SPDC) source of heralded, GHz-bandwidth single photons. The memory performance was characterised by measuring the second-order autocorrelation of the retrieved fields. While the SPDC input photon statistics showed a clear influence on the statistics of the retrieved field, four-wave mixing (FWM) noise, stimulated by spontaneous Raman scattering, prevented the preservation of non-classical photon statistics during read-out. Suppressing this source of noise represents the last remaining challenge for realising a broadband single-photon Raman memory suitable for quantum information applications. To this end, I demonstrate a novel cavity implementation of the Raman memory which reduces the FWM contribution relative to the signal field by re-distributing the density of states into which the noise photons can be scattered. Cavity-enhanced memory operation was investigated using weak coherent input states, showing a significant improvement of the signal-to-noise ratio compared to the free-space memory implementation. This proof-of-principle demonstration suggests that cavity Raman memories may offer a practical route towards low-noise, high-bandwidth quantum storage at room temperature.
An optical quantum memory, a device which can store and retrieve on demand an arbitrary quantum state at the single photon level, has been identified as a significant cornerstone of photonic quantum technologies. The development of such a memory would allow the creation and development of a large number of quantum technologies. These would range from the ability to synchronise processing steps in an optical quantum computer, to the construction of a quantum repeater which would allow faithful transmission of quantum states over arbitrarily long distances. In this thesis I investigate broadband light storage in a room-temperature Raman memory for purposes of quantum information processing with photons. During the course of this thesis, a novel scheme to suppress four-wave mixing noise is simulated, based on equations derived to describe the physics of the memory interaction. The experimental arrangement to test the suppression method is described and an original method using photon statistics is demonstrated. The results of these experiments prove the ability of the memory to retrieve and maintain the non-classicality of the state, given a single photon input. Following the affirmation that, using this noise suppression technique, the memory can function at the single-photon level, I go on to consider how the temporal-spectral properties of a pulsed mode of light may be manipulated using the memory. There are two primary reasons for this investigation: 1) Increasing the efficiency of the read-in process by carving the optimum mode of the memory 2) Using the memory as a device operating in a high dimensional quantum information basis. The restrictions of such applications are considered and a method to test the efficacy of transformations in this basis is devised and experimentally tested. I also perform demonstrations of light storage using conventional temporal modes using a novel method of velocity selection within warm vapour. Finally I detail further experiments that are achievable with the Raman quantum memory given the progress that has been achieved during my DPhil research. The results show that the Raman memory is a viable candidate for a practical route towards low-noise quantum storage and for manipulation of temporal modes of light.