We consider theoretically a semiconductor nanostructure embedded in one-dimensional microcavity and study the modification of its electron energy spectrum by the vacuum fluctuations of the electromagnetic field. To solve the problem, a nonperturbative diagrammatic approach based on the Green's function formalism is developed. It is shown that the interaction of the system with the vacuum fluctuations of the optical cavity opens gaps within the valence band of the semiconductor. The approach is verified for the case of large photon occupation numbers, proving the validity of the model by comparing to previous studies of the semiconductor system excited by a classical electromagnetic field. The developed theory is of general character and allows for unification of quantum and classical descriptions of the strong light-matter interaction in semiconductor structures.
We consider theoretically a semiconductor nanostructure embedded in one-dimensional microcavity and study the modification of its electron energy spectrum by the vacuum fluctuations of the electromagnetic field. To solve the problem, a nonperturbative diagrammatic approach based on the Green's function formalism is developed. It is shown that the interaction of the system with the vacuum fluctuations of the optical cavity opens gaps within the valence band of the semiconductor. The approach is verified for the case of large photon occupation numbers, proving the validity of the model by comparing to previous studies of the semiconductor system excited by a classical electromagnetic field. The developed theory is of general character and allows for unification of quantum and classical descriptions of the strong light-matter interaction in semiconductor structures.
Cavity quantum electrodynamics (QED) is the study of the interaction between light conned in a microcavity and material modes (such as single atoms or electrons in quantum wells), where the quantum nature of light is crucial.This thesis theoretically examines four dierent systems where light becomes strongly coupled with dierent material modes leading to dierent eects stemming from the dierent dimensionality and natures of the systems.The rst system consists of a semiconductor slab embedded into a zero-dimensional microcavity, leading to vacuum band gap opening of the electron dispersion caused by the interactions with the cavity photon mode.The second system is a quantum ring coupled to polarized light, calculated non-perturbatively.Since the polarization breaks time reversal symmetry, the particles in the ring will exhibit an energy dierence of particles with the same magnitude of angular momentum but dierent directions.The viability of these resulting in Aharonov-Bohm oscillations in large rings is considered.The third system consists of an array of quantum wires embedded into a planar microcavity.The inhomogeneity of the two directions along and perpendicular to the wires, coupled with the homogeneous two-dimensional photon mode, leads to an emergence of a hyperbolic region and many peculiar eects.The fourth and last work considers an algorithm to modify systems, leading to a ladder of equidistant energies.To illustrate, a radially symmetric nanoparticle with a hydrogenic impurity is analysed.The material composition along the radius can be altered to achieve a cascade of transitions in the Terahertz range.When multiple such particles are embedded into a resonant microcavity, one can convert photons of a higher energy to multiple Terahertz photons.
We consider a semiconductor quantum-well placed in a waveguide microcavity and interacting with the broadband squeezed vacuum radiation, which fills one mode of the waveguide with a large average occupation. The waveguide modifies the optical density of states so that the quantum well interacts mostly with the squeezed vacuum. The vacuum is squeezed around the externally controlled central frequency ${\ensuremath{\omega}}_{0}$, which is tuned above the electron-hole gap Eg, and induces fluctuations in the interband polarization of the quantum well. The power spectrum of scattered light exhibits a peak around ${\ensuremath{\omega}}_{0}$, which is moreover non-Lorentzian and is a result of both the squeezing and the particle-hole continuum. The squeezing spectrum is qualitatively different from the atomic case. We discuss the possibility of observing the above phenomena in the presence of additional nonradiative (e-e, phonon) dephasing.
In this paper, exciting progress of quantum optics in solid state is reviewed. The focus is on semiconductor microcavities with self-assembled quantum dots embedded in the active layer. Due to enormous progress in semiconductor nanotechnology, such photonic structures have become a model system for the study of quantum optics on a scalable and integrable technology platform with high potential for future applications in quantum information technology. Quantum optical phenomena have become accessible due to 3-D confinement of light and matter on the length scale of their wavelength in state-of-the-art semiconductor micro- and nanostructures. This confinement leads to a quantization of the associated photonic and electronic energy levels and requires a quantum mechanical description of the system in the framework of cavity quantum electrodynamics (cQED). This approach considers the dipole interaction between two-level quantum emitters and discrete photonic states of a microcavity. Within the well-known Jaynes-Cummings model, the dipole interaction is described in terms of a coherent exchange of energy between the emitter and the resonator mode. This coherent interaction in the so-called strong coupling regime of cQED is reflected in a normal mode splitting, the vacuum Rabi splitting, of the involved modes and represents a central feature of quantum optics in solid state. Another important example of quantum optics in semiconductor nanostructures is the generation of nonclassical light in specific quantum devices. Of particular interest is the realization of Fock states which represent states containing a well-defined number of photons. Single-photon sources, for instance, allow for the generation of single photons on demand, which is highly desirable for quantum communication systems. In this context, this review paper will present recent experimental studies of quantum optics in solid state. This paper is meant for readers who would like to become familiar with this topic and for experts being interested in the progress in this field. It will cover a broad range of studies ranging from examples of fundamental light-matter interaction in the quantum limit to devices capable of emitting single photons and entangled photon pairs on demand.
We theoretically study quantum-optical properties of one- and two-dimensional semiconductor nanostructures, where the electronic band structure is described by a two-band tight-binding model. Since the focus of our work is on analyzing quantum-optical effects of systems with a continuous band structure, many-body processes like electron-electron and electron-phonon interactions are neglected. The quantum-optical interband excitations are fully incorporated and described by a Jaynes-Cummings-type model. The exciting quantum light can be a state with arbitrary photon statistics. For simplicity, the results discussed here are limited to single-photon and two-photon Fock states. Our analytical approach is based on the eigenvalue problem and can be utilized to obtain explicit expressions for the steady-state properties of the system. Numerical simulations are based on solutions of the equations of motion and allow for a more precise analysis of the dynamics and nonresonant excitations of the system. We demonstrate that during the interaction process, a collective excitation of the conduction band is formed. For nonresonant excitations, this collective dynamics results in interesting steady states, in which the resonantly addressed eigenstates are occupied. The presented model provides a framework for microscopic simulations of quantum-optically excited extended semiconductor nanostructures.
In modern physics, the investigation of the interaction between light and matter is important from both a fundamental and an applied point of view. Cavity quantum electrodynamics (cavity QED) is the study of the interaction between light confined in a reflective cavity and atoms or other particles where the quantum nature of light photons is significant. The strong interaction between an exciton and cavity photon in a high-finesse microcavity can induce a hybrid light-matter eigenstate which is usually named as polariton in solid-state systems. This strong light-matter interaction can be achieved when this interaction is larger than all broadenings caused by other various factors e.g. electron phonon scattering and cavity loss. The polariton is now stimulating tremendous research interests due to its high potential in cavity quantum electrodynamics (QED) and the achievement of polaritonic devices. Moreover, when the interaction strength between an excitation and the cavity photon, quantified by vacuum Rabi frequency, becomes comparable to or larger than the corresponding electronic transition frequency in a cavity, the system can enter an ultrastrong coupling regime, which has been experimentally observed. In this regime, the standard rotating-wave approximation is no longer valid and the antiresonant term of the interaction Hamiltonian starts to play an important role, giving rise to exciting effects in cavity QED. The Aharonov-Bohm (AB) effect is a fundamental quantum phenomenon that bears the significance of the nature of electromagnetic fields and potentials. Besides its fundamental significance in quantum theory, its importance for applications in interferometric devices is omnipresent. Recently, since the 2D materials have triggered immense interest, some work has been done to integrate the AB effect with the electronic and transport properties of 2D materials. This thesis consists of two parts. In the first part, the light-matter coupling between cyclotron transition and photon is theoretically investigated in some 2-D materials such as the monolayer MoS2, graphene and monolayer black phosphorene (BP) systems. The results show that, in these 2-D materials, the ultrastrong light-matter coupling can be achieved at a high filling factor of Landau levels. Furthermore, we show that, in contrast to the case for conventional semiconductor resonators, the MoS2 system shows a vacuum instability. In monolayer MoS2 resonator, the diamagnetic term can still play an important role in determining magnetopolariton dispersion which is different from monolayer graphene system. The diamagnetic term arises from electron-hole asymmetry which indicates that electron-hole asymmetry can influence the quantum phase transition. Meanwhile, we show that, similar with some other 2D materials such as graphene and MoS2, the monolayer BP system shows a vacuum instability. However, in contrast with other 2D materials, the BP system displays a large energy gap between three branches of polaritons because of its strong anisotropic behavior in the eigenstates of the band structures. For the graphene system, we investigate the coupling of cyclotron transition and a multimode cavity described by a multimode Dicke model. This model exhibits a superradiant quantum phase transition, which we describe exactly in an effective Hamiltonian approach. The complete excitation spectrum in both the normal phase and superradiant phase regimes is given. At last, in contrast to the single mode case, multimode coupling of cavity photon and cyclotron transition can greatly reduce the critical vacuum Rabi frequency required for quantum phase transition, and dramatically enhance the superradiant emission by fast modulating the Hamiltonian. Our study provides new insights in cavity-controlled magneto-transport in these 2-D systems, which could lead to the development of polariton-based devices. The second part is a diversion from the main content of this thesis; readers who are not interested in foundational issues of physics can skip this part. For one charged quantum particle P moving in an electromagnetic vector potential Aˆµ = ( φˆ, - Aˆ ) created by some other charged particles, we can either use the framework of one particle quantum mechanics (OPQM) to calculate the evolutions of P, or we can treat this as an multi-particles problem in the framework of quantum field theory and calculate the evolution of P. These two methods need to be equivalent, i.e., they produce the same result for the evolution of P. One open question is how to describe the evolution of P within the framework of quantum field theory and show that these two methods yield the same result? In chapter 5, we are going to derive the OPQM from the quantum field theory, i.e., the quantum electrodynamics (QED) to be specific. We start with the discussions on the AB effect then raise a plausible interpretation within the QED framework. We provide a quantum treatment of the source of the electromagnetic potential and argue that the underlying mechanism in AB effect can be viewed as interactions between electrons described by QED theory where the interactions are mediated by virtual photons. On further analysis, we show that the framework of one particle quantum mechanics (OPQM) can be given, in general, as a mathematically approximated model which is reformulated from QED theory while the AB effect scheme provides a platform for our derivations. In addition, the classical Maxwell equations are derived from QED scattering process while both classical electromagnetic fields and potentials serve as mathematical tools that are constructed to approximate the interactions among elementary particles described by QED physics. This work opens up a new perspective on the nature of electromagnetic fields and potentials.
Based on a formalism that describes atom-light interactions in terms of the classical electromagnetic Green's function, we study the optical response of atoms and other quantum emitters coupled to one-dimensional photonic structures, such as cavities, waveguides, and photonic crystals. We demonstrate a clear mapping between the transmission spectra and the local Green's function, identifying signatures of dispersive and dissipative interactions between atoms. We also demonstrate the applicability of our analysis to problems involving three-level atoms, such as electromagnetically induced transparency. Finally we examine recent experiments, and anticipate future observations of atom-atom interactions in photonic band gaps.