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arXiv:1402.4234 · Physical Review B

Time-optimal universal control of two-level systems under strong driving

C. Avinadav, Ran Fischer, Paz London, D. Gershoni

Published Jun 27, 2014• 50 citations
arXivHTMLPDF

Abstract

We report on a theoretical and experimental study of time-optimal construction of arbitrary single-qubit rotations under a single strong driving field of finite amplitude. Using radiation-dressed states of nitrogen vacancy centers in diamond we realize a strongly driven two-level system, with driving frequencies four times larger than its precession frequency. We implement time-optimal universal rotations on this system, characterize their performance using quantum process tomography, and demonstrate a dual-axis multiple-pulse control sequence where the qubit is rotated on time scales faster than its precession period. Our results pave the way for applying fast qubit control and high-density pulse schemes in the fields of quantum information processing and quantum metrology.

DOI
10.1103/physrevb.89.245311

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We report on a theoretical and experimental study of time-optimal construction of arbitrary single-qubit rotations under a single strong driving field of finite amplitude. Using radiation-dressed states of nitrogen vacancy centers in diamond we realize a strongly driven two-level system, with driving frequencies four times larger than its precession frequency. We implement time-optimal universal rotations on this system, characterize their performance using quantum process tomography, and demonstrate a dual-axis multiple-pulse control sequence where the qubit is rotated on time scales faster than its precession period. Our results pave the way for applying fast qubit control and high-density pulse schemes in the fields of quantum information processing and quantum metrology.
Two-level systems are at the core of numerous real-world technologies such as magnetic resonance imaging and atomic clocks. Coherent control of the state is achieved with an oscillating field that drives dynamics at a rate determined by its amplitude. As the strength of the field is increased, a different regime emerges where linear scaling of the manipulation rate breaks down and complex dynamics are expected. By calibrating the spin rotation with an adiabatic passage, we have measured the room-temperature "strong-driving" dynamics of a single nitrogen vacancy center in diamond. With an adiabatic passage to calibrate the spin rotation, we observed dynamics on sub-nanosecond time scales. Contrary to conventional thinking, this breakdown of the rotating wave approximation provides opportunities for time-optimal quantum control of a single spin.
The strong-driving regime occurs when a quantum two-level system is driven with an external field whose amplitude is greater than or equal to the energy splitting between the system's states and is typically identified with the breaking of the rotating wave approximation (RWA). We report an experimental study in which the spin of a single nitrogen-vacancy (NV) center in diamond is strongly driven with microwave fields of arbitrary polarization. We measure the NV center spin dynamics beyond the RWA and characterize the limitations of this technique for generating high-fidelity quantum gates. Using circularly polarized microwave fields, the NV spin can be harmonically driven in its rotating frame regardless of the field amplitude, thus allowing rotations around arbitrary axes. Our approach can effectively remove the RWA limit in quantum-sensing schemes and assist in increasing the number of operations in QIP protocols.
The NV-center in diamond is a promising system for quantum information processing. The typical qubits are the electron spin in the NV-center and the surrounding 13C nuclear spins. Fast and precise control of many 13C spins is desirable but challenging due to crosstalk. Crosstalk is the unwanted effect of a control pulse on the other qubits. The coupled NV-13C system is explored, and numerical techniques to optimize the control of multiple and single qubits are used. In this report the effect of the Bloch-Siegert shift in the weak driving regime is investigated first. This is done by studying the effect of a π-pulse when two carbon qubits are driven at the same time on resonance. It turns out that in this weak driving regime the effect of the off resonance is very small, and changes the fidelity not more than 0.3%. Furthermore the effect of a square πpulse on 4 nearby qubits is studied. If the pulse is not optimized (thus square), the pulse cannot be done in less than 100µs while retaining at least 99% fidelity. By optimizing the envelope of the driving field using constrained optimization the pulse can be done in 22µs while retaining at least 99% fidelity.
The implementation of a high-fidelity two-qubit quantum logic gate remains an outstanding challenge for isolated solid-state qubits such as nitrogen-vacancy (NV) centers in diamond. In this work, we show that by driving pairs of NV centers to undergo photon scattering processes that flip their qubit states simultaneously, we can achieve a unitary two-qubit gate conditioned upon a single photon-detection event. Further, by exploiting quantum interference between the optical transitions of the NV centers' electronic states, we realize the existence of two special drive frequencies: a ``magic'' point where the spin-preserving elastic scattering rates are suppressed and a ``balanced'' point where the state-flipping scattering rates are equal. We analyzed four different gate operation schemes that utilize these two special drive frequencies, and various combinations of polarizations in the drive and collection paths. Our theoretical and numerical calculations show that the gate fidelity can be as high as 98%. The proposed unitary gate, combined with available single-qubit unitary operations, forms a universal gate set for quantum computing.
During the last ten years, basic quantum operations on a single electronic spins in the nitrogen-vacancy defect center in diamond have been a rich field of study. Quantum operations coherently manipulating the spin of the nitrogen-vacancy center have become promising candidates for easy to manipulate qubits. However in order to implement these qubits in quantum computers robust high-fidelity control is needed. Building on an existing confocal microscopy setup, pulsed and quadrature-amplitude modulated microwave signals were used to realize coherent spin manipulation measurements. Especially designed Smooth Optimal Control pulses (robust against detuning and different control amplitudes) were used to develop measurement schemes resulting in the aforementioned increase of fidelity. The first part of the thesis describes the implementation of these pulses into the existing experimental setup and the calibration work necessary prior to measurements, due to imperfections of devices in the microwave chain. The second part is dedicated to the analysis of the pulses applied to a single spin by comparing the experimental results to theoretical simulations. This was done not only for one resonant spin with accurate control amplitude, but also for a range of different detunings and amplitudes. A more thorough analysis of the pulses was then achieved by using state/process tomography, resulting in a complete description of the process induced by these optimized pulses. Finally, after verifying the effect of the pulses, measurement schemes for sensing alternating magnetic fields were implemented, resulting in measurements with improved sensitivity for magnetic fields.
Quantum control of systems plays an important role in modern science and technology. The ultimate goal of quantum control is to achieve high-fidelity universal control in a time-optimal way. Although high-fidelity universal control has been reported in various quantum systems, experimental implementation of time-optimal universal control remains elusive. Here, we report the experimental realization of time-optimal universal control of spin qubits in diamond. By generalizing a recent method for solving quantum brachistochrone equations [X. Wang et al., Phys. Rev. Lett. 114, 170501 (2015)], we obtained accurate minimum-time protocols for multiple qubits with fixed qubit interactions and a constrained control field. Single- and two-qubit time-optimal gates are experimentally implemented with fidelities of 99% obtained via quantum process tomography. Our work provides a time-optimal route to achieve accurate quantum control and unlocks new capabilities for the emerging field of time-optimal control in general quantum systems.