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arXiv:1402.0594 · Physical Review A

Non-Abelian geometric phase in the diamond nitrogen-vacancy center

Mark Kowarsky, Lloyd C. L. Hollenberg, A. Martin

Published Oct 22, 2014• 20 citations
arXivHTMLPDF

Abstract

This paper introduces a theoretical framework for understanding the accumulation of non-Abelian geometric phases in rotating nitrogen-vacancy centers in diamond. Specifically, we consider how degenerate states can be achieved and demonstrate that the resulting geometric phase for multiple paths is non-Abelian. We find that the non-Abelian nature of the phase is robust to fluctuations in the path and magnetic field. In contrast to previous studies of the accumulation of Abelian geometric phases for nitrogen-vacancy centers under rotation we find that the limiting time scale is ${T}_{1}$. As such a non-Abelian geometric phase accumulation in nitrogen-vacancy centers has potential advantages for applications as gyroscopes.

DOI
10.1103/physreva.90.042116

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This paper introduces a theoretical framework for understanding the accumulation of non-Abelian geometric phases in rotating nitrogen-vacancy centers in diamond. Specifically, we consider how degenerate states can be achieved and demonstrate that the resulting geometric phase for multiple paths is non-Abelian. We find that the non-Abelian nature of the phase is robust to fluctuations in the path and magnetic field. In contrast to previous studies of the accumulation of Abelian geometric phases for nitrogen-vacancy centers under rotation we find that the limiting time scale is T1{T}_{1}T1​. As such a non-Abelian geometric phase accumulation in nitrogen-vacancy centers has potential advantages for applications as gyroscopes.
Geometric phases encode the holonomy acquired under cyclic control of a quantum Hamiltonian: for nondegenerate eigenstates the effect is Abelian (a scalar phase), while in degenerate manifolds the Wilczek-Zee generalization yields a matrix-valued holonomy that can mix states and depends on path ordering. We present an overview of measuring Abelian and non-Abelian geometric phases in nitrogen-vacancy (NV) centers in diamond and propose a non-rotating measurement protocol enabled by the intrinsic14 N{ }^{14} ~\mathrm{N}14 Nhyperfine manifold. As a first step, we propose to measure the Abelian Berry phase on a single hyperfine-resolved two-level transition using microwaveengineered closed loops with dynamical-phase cancellation by loop reversal. We then propose a non-Abelian protocol that engineers a two-dimensional degenerate dark subspace in an NV-14 N{ }^{14} ~\mathrm{N}14 Nmanifold via RF dressing and three phase-coherent microwave couplings (a tripod Hamiltonian). Two closed control loops implemented by winding independent microwave phases generate non-commuting SU(2) holonomies, which can be verified using final-only population readout and minimal tomography. We also present timing trade-off curves, full unitary Schrödinger evolution of the four-level tripod, and projected dark-subspace diagnostics that quantify both leakage and non-commuting holonomy.
We propose an approach for an optical qubit rotation in the negatively charged nitrogen vacancy (NV) center in diamond. The qubit is encoded in the ground degenerate states at a relatively low-temperature limit. The basic idea of the rotation procedure is the non-Abelian geometric phase in an adiabatic passage, which is produced by the non-adiabatic transition between the two degenerate dark states. The feasibility is based on the success of modeling the NV center as an excited-doublet four-level atom. By applying two pump and two Stokes laser pulses, we found that the behavior of the adiabatic passage depends crucially on the applied intensity of each applied laser field and the detunings between the laser frequencies and their corresponding atomic transition. Particularly, a non-adiabatic transition appears when the applied pump and Stokes laser pulses are off resonance with their corresponding atomic transition.
Abstract Fast quantum spin manipulation is needed to design spin-based quantum logic gates and other quantum applications. Here, we construct the exact evolution operator of the nitrogen-vacancy-center (NV) spin in diamond under external magnetic fields, and investigate the nonadiabatic geometric phases—both cyclic and non-cyclic—in these fast-manipulated NV spin systems. It is believed that the nonadiabatic geometric phases can be measured in future experiments, and that these fast quantum manipulations can be useful in designing spin-based quantum applications.
The Nitrogen-Vacancy(NV) center has recently emerged as a powerful quantum system, combining the good coherence properties and control techniques of atomic systems with the small size and fabrication capabilities of solid-state devices. We report on a measurement of a single electron-spin phase shift arising directly from physical rotation. This phase shift is observed by measuring the phase difference in a distortion microwave frequency of 2880 MHz, and it can accumulate nonlinearly in time. Carrier rotation information can be obtained by measuring the quantum geometric phase accumulation. We demonstrate quantum control of a NV center within a specific rotation system and a rotational period comparable to the NV spin coherence time T2*. These characteristics contribute as well to make this quantum system a sensitive and compact rotation sensor.
We propose solid-state gyroscopes based on ensembles of negatively charged nitrogen-vacancy (${\mathrm{NV}}^{\ensuremath{-}}$) centers in diamond. In one scheme, rotation of the NV${}^{\ensuremath{-}}$ symmetry axis will induce Berry phase shifts in the ${\mathrm{NV}}^{\ensuremath{-}}$ electronic ground-state coherences proportional to the solid angle subtended by the symmetry axis. We estimate a sensitivity in the range of $5\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}3}$ $\mathrm{rad}\phantom{\rule{4pt}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}\phantom{\rule{4pt}{0ex}}{\mathrm{Hz}}^{\ensuremath{-}1/2}$ in a 1-mm3{}^{3}3 sensor volume using a simple Ramsey sequence. Incorporating dynamical decoupling to suppress dipolar relaxation may yield a sensitivity at the level of ${10}^{\ensuremath{-}5}$ $\mathrm{rad}\phantom{\rule{4pt}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}\phantom{\rule{4pt}{0ex}}{\mathrm{Hz}}^{\ensuremath{-}1/2}$. With a modified Ramsey scheme, Berry phase shifts in the 14N{}^{14}\mathrm{N}14N hyperfine sublevels would be employed. The projected sensitivity is in the range of ${10}^{\ensuremath{-}5}$ $\mathrm{rad}\phantom{\rule{4pt}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}\phantom{\rule{4pt}{0ex}}{\mathrm{Hz}}^{\ensuremath{-}1/2}$, however, the lower gyromagnetic ratio of 14N{}^{14}\mathrm{N}14N nuclei reduces the sensitivity to magnetic-field noise by several orders of magnitude. Reaching ${10}^{\ensuremath{-}5}$ $\mathrm{rad}\phantom{\rule{4pt}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}\phantom{\rule{4pt}{0ex}}{\mathrm{Hz}}^{\ensuremath{-}1/2}$ would represent an order of magnitude improvement over other compact, solid-state gyroscope technologies.