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arXiv:1401.4842

Influence of finite size of molecules on spectrum of fully polarized dipolar BECs: Generalization of Bogoliubov's spectrum

Pavel A. Andreev, L. S. Kuz’menkov

Published Jan 20, 2014• 0 citations
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Abstract

We discuss complete theory of point-like particles in fully polarized BECs describing difference in behaviour of electrically- and magnetically polarized BECs. Next we present generalization of this theory on finite size particles to include contribution of size of real molecules on dynamical properties of dipolar BECs. As an application of obtained equation we calculate spectrum of linear collective excitations getting generalization of the Bogoliubov's spectrum. We show absence of roton instability due to positivity of polarization contribution in the excitation spectrum. We found that new type of instabilities appears in small wave length limit due to finite size of molecules.

DOI
10.48550/arxiv.1401.4842

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We discuss complete theory of point-like particles in fully polarized BECs describing difference in behaviour of electrically- and magnetically polarized BECs. Next we present generalization of this theory on finite size particles to include contribution of size of real molecules on dynamical properties of dipolar BECs. As an application of obtained equation we calculate spectrum of linear collective excitations getting generalization of the Bogoliubov's spectrum. We show absence of roton instability due to positivity of polarization contribution in the excitation spectrum. We found that new type of instabilities appears in small wave length limit due to finite size of molecules.
Further development of the method of quantum hydrodynamics in application for Bose-Einstein condensates (BECs) is presented. To consider evolution of polarization direction along with particles movement we have developed corresponding set of quantum hydrodynamic equations. It includes equations of the polarization evolution and the polarization current evolution along with the continuity equation and the Euler equation (the momentum balance equation). Dispersion properties of the transverse waves including the electromagnetic waves propagating through the BECs are considered. To this end we consider full set of the Maxwell equations for description of electromagnetic field dynamics. This approximation gives us possibility to consider the electromagnetic waves along with the matter waves. We find a splitting of the electromagnetic wave dispersion on two branches. As a result we have four solutions, two for the electromagnetic waves and two for the matter waves, the last two are the concentration-polarization waves appearing as a generalization of the Bogoliubov mode. We also obtain that if the matter wave propagate perpendicular to external electric field when dipolar contribution does not disappear (as it follows from our generalization of the Bogoliubov spectrum). In this case exist a small dipolar frequency shift due to transverse electric field of perturbation.
The Gross–Pitaevskii equation for polarized molecules is an integro-differential equation, consequently it is complicated for solving. We find a possibility to represent it as a nonintegral nonlinear Schrödinger equation, but this equation should be coupled with two linear equations describing the electric field. These two equations are the Maxwell equations. We recapture the dispersion of collective excitations in the three-dimensional electrically polarized BEC with no evolution of the electric dipole moment directions. We trace the contribution of the electric dipole moment. We explicitly consider the contribution of the electric dipole moment in the interaction constant for the short-range interaction. We show that the spectrum of dipolar BEC does not reveal instability at repulsive short-range interaction. Nonlinear excitations are also considered. We present dependence of the bright soliton characteristics on the electric dipole moment.
Abstract We consider a BEC of rigid rotor molecules confined to quasi-2D through harmonic trapping. The molecules are subjected to an external electric field which polarizes the gas, and the molecules interact via dipole–dipole interactions. We present a description of the ground state and low-energy excitations of the system including an analysis of the mean-field energy, polarization, and stability. Under large electric fields the gas becomes fully polarized and we reproduce a well known density-wave instability which arises in polar BECs. Under smaller applied electric fields the gas develops an in-plane polarization leading to the emergence of a new global instability as the molecules ‘tilt’. The character of these instabilities is clarified by means of momentum-space density–density structure factors. A peak at zero momentum in the spin–spin structure factor for the in-plane component of the polarization indicates that the tilt instability is a global phonon-like instability.
Recent experimental advances in creating stable dipolar systems, including polar molecules with large electric dipole moments, have led to vigorous theoretical activities. Here we discuss our work on homogeneous 2D dipolar bosons with dipoles oriented at an angle to the direction perpendicular to the confining 2D plane, i.e. for non-zero tilt angles. Using Bogoliubov-de Gennes equations, we obtain T=0 excitation spectrum of the dipolar Bose gas, and explore instabilities at varying tilt angle, density and dipolar coupling. We map out a phase diagram a function of tilt angle, dipole strength and density. We find the development of maxon-roton behavior leading to roton instabilities at large densities for small tilt angles, and at low densities for large tilt angles. The behavior is anisotropic in k-space; accordingly the roton instabilities occur in the k y direction, suggestive of inhomogeneity and stripe phase, with density mode becoming soft in the y direction. Our results compare favorably with existing Quantum Monte Carlo calculations for non-zero tilt angles.
We present the Gross–Pitaevskii equation for Bose–Einstein condensates (BECs) possessing the electric dipole and the electric quadrupole moments in a non-integral form. These equations are coupled with the Maxwell equations. The model under consideration includes the dipole–dipole, the dipole–quadrupole, and the quadrupole–quadrupole interactions in terms of the electric field created by the dipoles and quadrupoles. We apply this model to obtain the Bogoliubov spectrum for three-dimensional BECs with a repulsive short-range interaction. We obtain an extra term in the Bogoliubov spectrum in comparison with the dipolar BECs. We show that the quadrupole–quadrupole interaction gives a positive contribution in the Bogoliubov spectrum. Hence, this spectrum is stable.
We present an analytic Bogoliubov description of a Bose-Einstein condensate of polar molecules trapped in a quasi-two-dimensional geometry and interacting via internal state-dependent dipole-dipole interactions. We derive the mean-field ground-state energy functional, and we derive analytic expressions for the dispersion relations, Bogoliubov amplitudes, and static structure factors. This method can be applied to any homogeneous, two-component system with linear coupling and direct, momentum-dependent interactions. The properties of the mean-field ground state, including polarization and stability, are investigated, and we identify three distinct instabilities: a density-wave rotonization that occurs when the gas is fully polarized, a spin-wave rotonization that occurs near zero polarization, and a mixed instability at intermediate fields. The nature of these instabilities is clarified by means of the real-space density-density correlation functions, which characterize the spontaneous fluctuations of the ground state, and the momentum-space structure factors, which characterize the response of the system to external perturbations. We find that the gas is susceptible to both density-wave and spin-wave responses in the polarized limit but only a spin-wave response in the zero-polarization limit. These results are relevant for experiments with rigid rotor molecules such as RbCs, $\mathrm{\ensuremath{\Lambda}}$-doublet molecules such as ThO that have an anomalously small zero-field splitting, and doublet-$\mathrm{\ensuremath{\Sigma}}$ molecules such as SrF where two low-lying opposite-parity states can be tuned to zero splitting by an external magnetic field.