The measurement of correlations between different degrees of freedom is an important, but in general extremely difficult task in many applications of quantum mechanics. Here, we report an all-optical experimental detection and quantification of quantum correlations between the polarization and the frequency degrees of freedom of single photons by means of local operations acting only on the polarization degree of freedom. These operations only require experimental control over an easily accessible two-dimensional subsystem, despite handling strongly mixed quantum states comprised of a continuum of orthogonal frequency states. Our experiment thus represents a photonic realization of a scheme for the local detection of quantum correlations in a truly infinite-dimensional continuous-variable system, which excludes an efficient finite-dimensional truncation.
The measurement of correlations between different degrees of freedom is an important, but in general extremely difficult task in many applications of quantum mechanics. Here, we report an all-optical experimental detection and quantification of quantum correlations between the polarization and the frequency degrees of freedom of single photons by means of local operations acting only on the polarization degree of freedom. These operations only require experimental control over an easily accessible two-dimensional subsystem, despite handling strongly mixed quantum states comprised of a continuum of orthogonal frequency states. Our experiment thus represents a photonic realization of a scheme for the local detection of quantum correlations in a truly infinite-dimensional continuous-variable system, which excludes an efficient finite-dimensional truncation.
Developing techniques for characterizing quantum mechanical systems has been a major topic of research, especially in recent years, as quantum technologies, such as quantum communication and quantum cryptography, have grown to become an important asset in modern society. Although techniques such as quantum state tomography is an effective method to characterize a system consisting of two-level systems, the characterization of continuous degree of freedom such as space or frequency stills represents a time-consuming task as the state space scales exponentially with the dimension of the system. In this work, we show an indirect approach for measuring properties of high-dimensional degrees of freedom by coupling them to two-dimensional subsystems that can be measured efficiently via quantum state tomography. In our case, the property of interest is the correlation factor of the joint spectral amplitude describing the two-photon frequency states, which are coupled to the polarization degree of freedom using a completely positive trace-preserving map, called a dephasing channel. The action of the map on the polarization state induces a decoherence effect that depends on the initial frequency state, thus allowing to retrieve information about the frequency correlation factor by only measuring the decoherence in the polarization state. In the experimental part, we produced a pair of photons using spontaneous parametric down-conversion and characterized the joint spectral intensity with stimulated emission tomography. The decoherence was controlled with a birefringent material that acts as a dephasing channel. The polarization state was measured after the dephasing channel for two different initial frequency configurations using quantum state tomography. The bounds for the frequency correlation factor were calculated from the fidelity of the two polarization states and the generalized data processing inequality. The results of this work show that the polarization decoherence can be used as a tool to measure the frequency correlation factor of the joint spectral amplitude.
Entanglement is a key resource for fundamental tests of physics and emerging quantum technologies. In quantum optics, two perspectives on entanglement coexist. In the continuous-variable framework, entanglement is understood as holding between optical modes. In contrast, discrete-variable quantum optics focuses on quantum correlations in degrees of freedom such as polarization that label fixed numbers of photons. In this paper, we show that entanglement can transcend this separation. Spontaneous parametric down-conversion inherently generates correlations in optical phase space, photon number, and labelling degrees of freedom simultaneously. In polarization, this structure is traditionally described by macroscopic Bell states. Existing witnesses, however, fail to detect the genuine hybrid entanglement of these states, which goes beyond the continuous-discrete-variable categorization. Here, we lay the groundwork for a general framework unifying continuous- and discrete-variable notions of entanglement. In particular, we derive an operational witness providing a sufficient criterion for genuine hybrid number-polarization entanglement and outline its experimental implementation. Finally, we discuss exemplary states which, together with our results on macroscopic Bell states, motivate a broader classification of genuine hybrid quantum correlations.
Photonic quantum technologies utilize various degrees of freedom (DOFs) of light, such as polarization, frequency, and spatial modes, to encode quantum information. In the effort of further improving channel capacity of quantum communication, and for increasing the complexity of available quantum operations, high-dimensional and hyperentangled states are now gaining interest. However, efficiently measuring these high dimensional states is challenging due to the large number of measurements required for reconstructing the full density matrix via quantum state tomography (QST), and the fact that each measurement requires some modification in the experimental setup. Here, we propose a framework for reconstructing the density matrix of a single-photon hyperentangled across multiple DOFs using a single intensity-measurement obtainable from traditional cameras, and discuss extensions for multiphoton hyperentangled states. Our method hinges on the spatial DOF of the photon and uses it to encode the quantum information from the other DOFs. We numerically demonstrate this method for single-photon OAM-spin and OAM-frequency entangled states using an ideal coupler and a multimode fiber, to perform the information mixing and transfer the encoding to spatial information, where it is detected using a simple camera. This technique simplifies the experimental setup and reduces acquisition time compared to traditional QST-based methods. Moreover, it allows the recovery of DOFs that conventional cameras cannot detect, such as polarization, thus eliminating the need for projection measurements.
Continuous variable entanglement is usually set between pairs of optical modes sharing the same geometrical property where distinguishability is demanded to polarization and/or frequency. Thus, the inherent non-local correlation shows-up in quantum quadratures relative to two distinct e.m. modes. In this contribution we will show how the polarization d.o.f. of a pair of entangled modes is coupled to the optical orbital angular momentum giving, at the end, a pair of entangled modes that have orthogonal OAM and polarization. We also show how this experimental scheme can be extended to give more than a pair of entangled modes paving the way to CV entanglement multiplexing.
With recent advances in nanophotonics, metasurfaces based on nano-resonators have facilitated novel types of optical devices. In particular, the interplay between different degrees of freedom, involving polarization and spatial modes, boosted classical polarization measurements and imaging applications. However, the use of metasurfaces for measuring the quantum states of light remains largely unexplored. Conventionally, the task of quantum state tomography is realized with several bulk optical elements, which need to be reconfigured multiple times. Such setups can suffer from decoherence, and there is a fundamental and practical interest in developing integrated solutions for measurement of multi-photon quantum states. We present a new concept and the first experimental realization of all-dielectric metasurfaces with no tuneable elements for imaging-based reconstruction of the full quantum state of entangled photons. Most prominently, we implement multi-photon interferometric measurements on a sub-wavelength thin optical element, which delivers ultimate miniaturization and extremely high robustness. Specifically, we realize a highly transparent all-dielectric metasurface, which spatially splits different components of quantum-polarization states. Then, a simple one-shot measurement of correlations with polarization-insensitive on-off click detectors enables complete reconstruction of multi-photon density matrices with high precision. In our experiment, we prepare sets of polarization states and reconstruct their density matrices with a high fidelity of over 99% for single photon states and above 95% for two-photon states. Our work provides a fundamental advance in the imaging of quantum states, where multi-photon quantum interference takes place at sub-wavelength scale.
In 1935 Einstein, Podolsky and Rosen used the assumption of local realism to conclude in a Gedankenexperiment with two entangled particles that quantum mechanics is not complete. For this reason EPR motivated an extension of quantum mechanics by so-called local hidden variables. Based on this idea in 1964 Bell constructed a mathematical inequality whereby experimental tests could distinguish between quantum mechanics and local-realistic theories. Many experiments have since been done that are consistent with quantum mechanics, disproving the concept of local realism. But all these tests suffered from loopholes allowing a local-realistic explanation of the experimental observations by exploiting either the low detector efficiency or the fact that the detected particles were not observed space-like separated. In this context, of special interest is entanglement between different quantum objects like atoms and photons, because it allows one to entangle distant atoms by the interference of photons. The resulting space-like separation together with the almost perfect detection efficiency of the atoms allows a first loophole-free test of Bell's inequality. The primary goal of the present thesis is the experimental realization of entanglement between a single localized atom and a single spontaneously emitted photon at a wavelength suitable for the transport over long distances. In the experiment a single optically trapped Rb87 atom is excited to a state which has two selected decay channels. In the following spontaneous decay a photon is emitted coherently with equal probability into both decay channels. This accounts for perfect correlations between the polarization state of the emitted photon and the Zeeman state of the atom after spontaneous decay. Because these decay channels are spectrally and in all other degrees of freedom indistinguishable, the spin state of the atom is entangled with the polarization state of the photon. To verify entanglement, appropriate correlation measurements in complementary bases of the photon polarization and the internal quantum state of the atom are performed. It is shown, that the generated atom-photon state yields an entanglement fidelity of 0.82. The experimental results of this work mark an important step towards the generation of entanglement between space-like separated atoms for a first loophole-free test of Bell's inequality. Furthermore entanglement between a single atom and a single photon is an important tool for new quantum communication and information applications, e.g. the remote state preparation of a single atom over large distances.