We present a quantum-enhanced atomic clock protocol based on groups of sequentially larger Greenberger-Horne-Zeilinger (GHZ) states that achieves the best clock stability allowed by quantum theory up to a logarithmic correction. Importantly the protocol is designed to work under realistic conditions where the drift of the phase of the laser interrogating the atoms is the main source of decoherence. The simultaneous interrogation of the laser phase with a cascade of GHZ states realizes an incoherent version of the phase estimation algorithm that enables Heisenberg-limited operation while extending the coherent interrogation time beyond the laser noise limit. We compare and merge the new protocol with existing state of the art interrogation schemes, and identify the precise conditions under which entanglement provides an advantage for clock stabilization: it allows a significant gain in the stability for short averaging time.
We present a quantum-enhanced atomic clock protocol based on groups of sequentially larger Greenberger-Horne-Zeilinger (GHZ) states that achieves the best clock stability allowed by quantum theory up to a logarithmic correction. Importantly the protocol is designed to work under realistic conditions where the drift of the phase of the laser interrogating the atoms is the main source of decoherence. The simultaneous interrogation of the laser phase with a cascade of GHZ states realizes an incoherent version of the phase estimation algorithm that enables Heisenberg-limited operation while extending the coherent interrogation time beyond the laser noise limit. We compare and merge the new protocol with existing state of the art interrogation schemes, and identify the precise conditions under which entanglement provides an advantage for clock stabilization: it allows a significant gain in the stability for short averaging time.
We propose a hybrid quantum-classical atomic clock where the interrogation of atoms prepared in a spin-coherent (or weakly squeezed) state is used to feed back one or more highly spin-squeezed atomic states toward their optimal phase-sensitivity point. The hybrid clock overcomes the stability of a single Ramsey clock using coherent or optimal spin-squeezed states and reaches a Heisenberg-limited stability while avoiding nondestructive measurements. When optimized with respect to the total number of particles, the protocol surpasses the state-of-the-art proposals that use Greenberger-Horne-Zeilinger or NOON states. We compare analytical predictions with numerical simulations of clock operations, including correlated 1/f local oscillator noise.
The use of correlated states and measurements promises improvements in the accuracy of frequency metrology and the stability of atomic clocks. However, developing strategies robust against dominant noise processes remains challenging. We address the issue of decoherence due to spontaneous decay and show that Greenberger-Horne-Zeilinger (GHZ) states, in conjunction with a correlated measurement and nonlinear estimation strategy, achieve gains of up to 2.25 dB, comparable to fundamental bounds for up to about 80 atoms in the presence of decoherence. This result is surprising since GHZ states do not provide any enhancement under dephasing due to white frequency noise compared to the standard quantum limit of uncorrelated states. The gain arises from a veto signal, which allows for the detection and mitigation of errors caused by spontaneous emission events. Through comprehensive Monte-Carlo simulations of atomic clocks, we demonstrate the robustness of the GHZ protocol.
Abstract Precise timekeeping is a foundational, often overlooked dependency of both positioning/navigation/timing (PNT) systems and secure communications: satellite navigation requires nanosecond-level clock synchronization to compute position from signal time-of-flight, and time-synchronized cryptographic protocols (including key-exchange window validation and frequency-hopping schemes) depend on clock stability at the transmitting and receiving ends. Current-generation atomic clocks (cesium and rubidium standards) achieve their stability by averaging over many independent, unentangled atoms, a strategy fundamentally limited by the standard quantum limit (SQL), in which timing precision scales with the number of atoms N as N. Quantum-enhanced atomic clocks propose replacing independent-atom ensembles with entangled (GHZ-state) ensembles, whose Heisenberg-limited precision scales instead as N². This study validates the two components of that claim independently: (1) the entanglement-derived precision advantage, via GHZ Ramsey spectroscopy simulated on the PKTron quantum computing framework across probe sizes N = 1, 2, 4, and 6, and cross-checked on IBM Quantum's ibm_fez hardware at N = 4; and (2) accurate recovery of an atomic transition's phase signal, via PKTron's built-in Quantum Phase Estimation (QPE) algorithm, tested against three independent reference phases. Simulation reproduced exact Heisenberg scaling (measured Fisher information of 1.00, 4.00, 16.00, and 36.00 against theoretical N² values of 1, 4, 16, and 36) and exact QPE phase recovery (zero measured error across all three test phases). On real IBM Quantum hardware at N = 4, the zero-drift calibration point returned P(all-zero) = 0.972, and the maximum-sensitivity bias point returned P(all-zero) = 0.500, exactly matching the theoretical prediction. These results constitute a reproducible, multi-method, hardware-validated confirmation of the sensing and phase-extraction primitives that underlie quantum-enhanced atomic clock proposals. This work does not simulate or validate a physical atomic clock, an optical lattice clock, or any oscillator hardware; it validates the underlying discrete-variable sensing and estimation mechanisms only, and should be read accordingly.
Abstract The frequency stability of many optical atomic clocks is limited by the coherence of their local oscillator. Here, we present a measurement protocol that overcomes the laser coherence limit. It relies on engineered dynamical decoupling of laser phase noise and near-synchronous interrogation of two clocks. One clock coarsely tracks the laser phase using dynamical decoupling; the other refines this estimate using a high-resolution phase measurement. While the former needs to have a high signal-to-noise ratio, the latter clock may operate with any number of particles. The protocol effectively enables minute-long Ramsey interrogation for coherence times of few seconds as provided by the current best ultrastable laser systems. We demonstrate implementation of the protocol in a realistic proof-of-principle experiment, where we interrogate for 0.5 s at a laser coherence time of 77 ms. Here, a single lattice clock is used to emulate synchronous interrogation of two separate clocks in the presence of artificial laser frequency noise. We discuss the frequency instability of a single-ion clock that would result from using the protocol for stabilisation, under these conditions and for minute-long interrogation, and find expected instabilities of σy(τ) = 8 × 10−16(τ/s)−1/2 and σy(τ) = 5 × 10−17(τ/s)−1/2, respectively.
The ultimate stability of atomic clocks is limited by the quantum noise of the atoms. To reduce this noise it has been suggested to use entangled atomic ensembles with reduced atomic noise. Potentially this can push the stability all the way to the limit allowed by the Heisenberg uncertainty relation, which is denoted the Heisenberg limit. In practice, however, entangled states are often more prone to decoherence, which may prevent reaching this performance. Here we present an adaptive measurement protocol that in the presence of a realistic source of decoherence enables us to get near-Heisenberg-limited stability of atomic clocks using entangled atoms. The protocol may thus realize the full potential of entanglement for quantum metrology despite the detrimental influence of decoherence.
The frequency stability achieved by an optical atomic clock ultimately depends on the coherence of its local oscillator. Even the best ultrastable lasers only allow interrogation times of a few seconds, at present. Here we present a universal measurement protocol that overcomes this limitation. Engineered dynamic decoupling of laser phase noise allows any optical atomic clock with high signal-to-noise ratio in a single interrogation to reconstruct the laser's phase well beyond its coherence limit. A compound clock is then formed in combination with another optical clock of any type, allowing the latter to achieve significantly higher frequency stability than on its own. We demonstrate implementation of the protocol in a realistic proof-of-principle experiment with a phase reconstruction fidelity of 99 %. The protocol enables minute-long interrogation for the best ultrastable laser systems. Likewise, it can improve clock performance where less stable local oscillators are used, such as in transortable systems.