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arXiv:1310.0277 · Condensed Matter Physics

Magnetocaloric effect in the spin-1/2 Ising-Heisenberg diamond chain with the four-spin interaction

Lucia Gálisová

Published Jan 1, 2014• 30 citations
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Abstract

The magnetocaloric effect in the symmetric spin-1/2 Ising-Heisenberg diamond chain with the Ising four-spin interaction is investigated using the generalized decoration-iteration mapping transformation and the transfermatrix technique.The entropy and the Grüneisen parameter, which closely relate to the magnetocaloric effect, are exactly calculated to compare the capability of the system to cool in the vicinity of different field-induced ground-state phase transitions during the adiabatic demagnetization.

DOI
10.5488/cmp.17.13001

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The magnetocaloric effect in the symmetric spin-1/2 Ising-Heisenberg diamond chain with the Ising four-spin interaction is investigated using the generalized decoration-iteration mapping transformation and the transfermatrix technique.The entropy and the Grüneisen parameter, which closely relate to the magnetocaloric effect, are exactly calculated to compare the capability of the system to cool in the vicinity of different field-induced ground-state phase transitions during the adiabatic demagnetization.
We calculate the entropy and cooling rate of the antiferromagnetic spin-12\frac{1}{2}21​ XXZXXZXXZ chain under an adiabatic demagnetization process using the quantum transfer-matrix technique and nonlinear integral equations. The limiting case of the Ising chain (corresponding to infinitely large anisotropy) is presented for comparison. Our exact results for the Heisenberg chain are used as a cross-check for the numerical exact diagonalization as well as quantum Monte Carlo simulations and allow us to benchmark the numerical methods. Close to field-induced quantum phase transitions we observe a large magnetocaloric effect. Furthermore, we verify universal low-temperature power laws in the cooling rate and entropy, in particular, linear scaling of entropy with temperature TTT in the gapless Luttinger-liquid state and scaling as T\sqrt{T}T​ at field-induced transitions to gapped phases.
The entropy and cooling rate of the both antiferromagnetic spin-1/2 double sawtooth IsingHeisenberg model and mixed-spin (1,1/2) double sawtooth Ising-Heisenberg model on the distorted ladders are rigorously investigated under an adiabatic demagnetization process using the quantum transfer-matrix technique. The models include the XXZ interaction between the interstitial Heisenberg dimers, the Ising coupling between nearest-neighbor spins of the legs and rungs, and additional cyclic four-spin exchange (ring exchange) in the square plaquette of each block. Close to field-induced quantum phase transitions, we compare both models together in the ability of cooling/heating near the quantum critical points. However, we observe a large magnetocaloric effect for both models, the mixed-spin double sawtooth ladder shows much more magneticaloric efficiency than the spin-1/2 double sawtooth ladder. During an adiabatic demagnetization process it can be seen a temperature dropping in the vicinity of the zero-temperature quantum phase transitions. Various fixed values of the Isotropic and anisotropic parameters explicitly alter the quality of the magnetocaloric effect. This properties suggest double sawtooth Ising-Heisenberg ladders as promising alternative refrigerant materials for low-temperature magnetic refrigeration.
The ground state, entropy, and magnetic Grüneisen parameter of the antiferromagnetic spin-1/2 Ising-Heisenberg model on a double sawtooth ladder are rigorously investigated using the classical transfer-matrix technique. The model includes the XXZ interaction between the interstitial Heisenberg dimers, the Ising coupling between nearest-neighbor spins of the legs and rungs, and additional cyclic four-spin Ising term in each square plaquette. For a particular value of the cyclic four-spin exchange, we found in the ground-state phase diagram of the Ising-Heisenberg ladder a quadruple point, at which four different ground states coexist together. During an adiabatic demagnetization process, a fast cooling accompanied with an enhanced magnetocaloric effect can be detected near this quadruple point. The ground-state phase diagram of the Ising-Heisenberg ladder is confronted with the zero-temperature magnetization process of the purely quantum Heisenberg ladder, which is calculated by using exact diagonalization based on the Lanczos algorithm for a finite-size ladder of 24 spins and the density-matrix renormalization group simulations for a finite-size ladder with up to 96 spins. Some indications of the existence of intermediate magnetization plateaus in the magnetization process of the full Heisenberg model for a small but nonzero four-spin Ising coupling were found. The DMRG results reveal that the quantum Heisenberg double sawtooth ladder exhibits some quantum Luttinger spin-liquid phase regions that are absent in the Ising-Heisenberg counterpart model. Except this difference, the magnetic behavior of the full Heisenberg model is quite analogous to its simplified Ising-Heisenberg counterpart and, hence, may bring insight into the fully quantum Heisenberg model from rigorous results for the Ising-Heisenberg model.
Abstract A symmetric spin‐1/2 Ising–Heisenberg diamond chain with the Ising four‐spin interaction is exactly solved by means of the generalized decoration‐iteration mapping transformation. The ground state, the magnetization process and thermodynamics are particularly examined for the case of antiferromagnetic pair interactions (Ising and isotropic Heisenberg ones). It is shown that an interplay between pair interactions, the four‐spin interaction and the external magnetic field gives rise to several quantum ground states with entangled spin states in addition to some semi‐classically ordered ones. Besides, the temperature dependence of the magnetic susceptibility multiplied by the temperature is studied and the interesting triple‐peak specific heat curve is also detected when considering the zero‐field region rather close to the triple point, where three different ground states coexist.
We study the magnetocaloric effect for the integrable antiferromagnetic high spin chain. We present an exact computation of the Grüneisen parameter, which is closely related to the magnetocaloric effect, for the quantum spin- s chain in the thermodynamical limit by means of Bethe ansatz techniques and the quantum transfer matrix approach. We have also calculated the entropy S and the isentropes in the ( H , T ) plane. We have been able to identify the quantum critical points H c ( s ) = 2/( s + 1/2) looking at the isentropes and/or the characteristic behaviour of the Grüneisen parameter.