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arXiv:1309.5583 · Physical Review A

Creating a tunable spin squeezing via a time-dependent collective atom-photon coupling

Lixian Yu, Jingtao Fan, Shiqun Zhu, Gang Chen, Suotang Jia, Franco Nori

Published Feb 21, 2014• 19 citations
arXivHTMLPDF

Abstract

We present an experimentally feasible method to produce a large and tunable spin squeezing when an ensemble of many four-level atoms interacts simultaneously with a single-mode photon and classical driving lasers. Our approach is to simply introduce a time-dependent collective atom-photon coupling. We show that the maximal squeezing factor measured experimentally can be well controlled by both its driving magnitude and driving frequency. In particular, when increasing the driving magnitude, the maximal squeezing factor increases and thus can be rapidly enhanced. We also demonstrate explicitly in the high-frequency approximation that this spin squeezing arises from a strong repulsive spin-spin interaction induced by the time-dependent collective atom-photon coupling. Finally, we evaluate analytically, by using current experimental parameters, the maximal squeezing factor, which can reach 40 dB. This squeezing factor is far larger than previous ones.

DOI
10.1103/physreva.89.023838

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We present an experimentally feasible method to produce a large and tunable spin squeezing when an ensemble of many four-level atoms interacts simultaneously with a single-mode photon and classical driving lasers. Our approach is to simply introduce a time-dependent collective atom-photon coupling. We show that the maximal squeezing factor measured experimentally can be well controlled by both its driving magnitude and driving frequency. In particular, when increasing the driving magnitude, the maximal squeezing factor increases and thus can be rapidly enhanced. We also demonstrate explicitly in the high-frequency approximation that this spin squeezing arises from a strong repulsive spin-spin interaction induced by the time-dependent collective atom-photon coupling. Finally, we evaluate analytically, by using current experimental parameters, the maximal squeezing factor, which can reach 40 dB. This squeezing factor is far larger than previous ones.
Squeezed spin states and squeezed light are both key resources for quantum metrology and quantum information science, but have been separately investigated in experiments so far. Simultaneous generation of these two types of quantum states in one experiment setup is intriguing but remains a challenging goal. Here, we propose a novel protocol based on judiciously engineered symmetric atom-light interaction, and report proof-of-principle experimental results of concurrent spin squeezing of 0.61±0.09 dB and light squeezing of 0.65_{-0.10}^{+0.11} dB in a hot atomic ensemble. The squeezing process is deterministic, yielding fixed squeezing directions for both the light field and the collective atomic spin. Furthermore, the squeezed light modes lie in the multiple frequency sidebands of a single spatial mode. This new type of dual squeezed state is applicable for quantum enhanced metrology and quantum networks. Our method can be extended to other quantum platforms such as optomechanics, cold atoms, and trapped ions.
It has been shown elsewhere that two spatially separated atoms can jointly absorb one photon, whose frequency is equal to the sum of the transition frequencies of the two atoms. We describe this process in the presence of an ensemble of many two-level atoms and show that it can be used to generate spin squeezing and entanglement. This resonant collective process allows us to create a sizable squeezing already at the single-photon limit. It represents a way to generate many-body spin-spin interactions, yielding a two-axis twisting-like interaction among the spins, which is very efficient for the generation of spin squeezing. We perform explicit calculations for ensembles of magnetic molecules coupled to a superconducting coplanar cavities. This system represents an attractive on-chip architecture for the realization of improved sensing.
Unitary control of qudits can improve the collective spin squeezing of an atomic ensemble. Preparing the atoms in a state with large quantum fluctuations in magnetization strengthens the entangling Faraday interaction. The resulting increase in interatomic entanglement can be converted into metrologically useful spin squeezing. Further control can squeeze the internal atomic spin without compromising entanglement, providing an overall multiplicative factor in the collective squeezing. We model the effects of optical pumping and study the tradeoffs between enhanced entanglement and decoherence. For realistic parameters we see improvements of ~10 dB.
The interaction of classical and quantized electromagnetic fields with an ensemble of atoms in an optical cavity is considered. Four fields drive a double-lambda level scheme in the atoms, consisting of a pair of lambda systems sharing the same set of lower levels. Two of the fields produce maximum coherence, rho12 = -1/2, between the ground state sublevels 1 and 2. This pumping scheme involves equal intensity fields that are resonant with both the one and two-photon transitions of the lambda system. There is no steady-state absorption of these fields, implying that the fields induce a type electromagnetically-induced transparency (EIT) in the medium. An additional pair of fields interacting with the second lambda system, combined with the EIT fields, leads to squeezing of the atom spin associated with the ground state sublevels. Our method involves a new mechanism for creating steady-state spin squeezing using an optical cavity. As the cooperativity parameter C is increased, the optimal squeezing varies as C^{-1/3}. For experimentally accessible values of C, squeezing as large as 90% can be achieved.
An advantageous architecture for producing deterministic spin squeezing is cavity QED. We show that the recently discovered one photon - two atom excitation process can be used to generate optimal squeezing (scaling as 1/N1/N1/N) of an ensemble of NNN spins coupled to a single-mode cavity. This method has some remarkable features. It is a resonant phenomenon mediated by real photons, which provides the advantage of tunability. This allows to create a sizeable squeezing already at the single-photon limit. Finally, in the strong cavity-driving regime the effective theory is similar to a two-axis Hamiltonian. We calculate that reaching −30-30−30dB is possible already with the known reported spin-cavity and decoherence rates in magnetic molecules coupled to superconducting circuit resonators. This system represents an attractive on-chip architecture for the realization of technological solutions in sensing.
Quantum control of many body atomic spins is often pursued in the context of an atom-light quantum interface, where a quantized light field acts as a "quantum bus" that can be used to entangle distant atoms. One key challenge is to improve the coherence of the atom-light interface and the amount of atom-light entanglement it can generate, given the constraints of working with multilevel atoms and optical fields in a 3D geometry. We have explored new ways to achieve this, through rigorous optimization of the spatial geometry, and through control of the internal atomic state. Our basic setup consists of a quantized probe beam passing through an atom cloud held in a dipole trap, first generating spin-probe entanglement through the Faraday interaction, and then using backaction from a measurement of the probe polarization to squeeze the collective atomic spin. The relevant figure of merit is the metrologically useful spin squeezing determined by the enhancement in the resolution of rotations of the collective spin, relative to the commonly used spin coherent state. With an optimized free-space geometry, and by using a 2-color probe scheme to suppress tensor light shifts, we achieve 3(2) dB of metrologically useful spin squeezing. We can further increase atom-light coupling by implementing internal state control to prepare spin states with larger initial projection noise relative to the spin coherent state. Under the right conditions this increase in projection noise can lead to stronger measurement backaction and increased atom-atom entanglement. With further internal state control the increased atom-atom entanglement can then be mapped to a basis where it corresponds to improved squeezing of, e.g., the physical spin-angular momentum or the collective atomic clock pseudospin. In practice, controlling the collective spin of N ~ 10⁶ atoms in this fashion is an extraordinarily difficult challenge because errors in the control of individual atoms tend to be highly correlated. By employing precise internal state control, we have prepared and detected projection noise limited "cat" states (which have initial projection noise that is larger by a factor of 2f = 8 for Cs relative to the spin coherent state) and estimate that we can generate up to 6.0(5) dB of metrologically useful spin squeezing, demonstrating the advantage of using the internal atomic structure as a resource for ensemble control.