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arXiv:1308.1844 · Physical Review B

Dipoles on a two-leg ladder

Søren Gammelmark, Nikolaj Thomas Zinner

Published Dec 30, 2013• 9 citations
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Abstract

We study polar molecules with long-range dipole-dipole interactions confined to move on a two-leg ladder for different orientations of the molecular dipole moments with respect to the ladder. Matrix product states are employed to calculate the many-body ground state of the system as a function of lattice filling fractions, perpendicular hopping between the legs, and dipole interaction strength. We show that the system exhibits zigzag ordering when the dipolar interactions are predominantly repulsive. As a function of dipole moment orientation with respect to the ladder, we find that there is a critical angle at which ordering disappears. This angle is slightly larger than the angle at which the dipoles are noninteracting along a single leg. This behavior should be observable using current experimental techniques.

DOI
10.1103/physrevb.88.245135

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We study polar molecules with long-range dipole-dipole interactions confined to move on a two-leg ladder for different orientations of the molecular dipole moments with respect to the ladder. Matrix product states are employed to calculate the many-body ground state of the system as a function of lattice filling fractions, perpendicular hopping between the legs, and dipole interaction strength. We show that the system exhibits zigzag ordering when the dipolar interactions are predominantly repulsive. As a function of dipole moment orientation with respect to the ladder, we find that there is a critical angle at which ordering disappears. This angle is slightly larger than the angle at which the dipoles are noninteracting along a single leg. This behavior should be observable using current experimental techniques.
A system with externally polarized dipole molecules at half-filling moving along a one-dimensional zigzag chain is studied, including ground-state phase diagrams. The dipoles are oriented in-plane. Together with the geometry of the chain, this gives rise to a bond-alternating nearest-neighbor interaction due to simultaneous attractive and repulsive interactions. By tuning the ratio between the nearest-neighbor interaction and hopping, various phases can be accessed by controlling the polarization angle. In the ultrastrong coupling limit, the system simplifies to a frustrated extended axial Ising model. For the small coupling limit, qualitative discussion of the ordering behavior using effective field theory arguments is provided. We show that when the chain angle is small, the system mostly exhibits BKT-type phase transitions, whereasa large chain angle would drive the system into a gapped (Ising) dimerized phase, where the hopping strength is closely related to the orientation of dimerized pairs.
The ground-state phase diagram of a two-leg fermionic dipolar ladder with inter-site interactions is studied using density matrix renormalization group (DMRG) techniques. We use a state-of-the-art implementation of the DMRG algorithm and finite size scaling to simulate large system sizes with high accuracy. We also consider two different model systems and explore stable phases in half and quarter filling factors. We find that in the half filling, the charge and spin gaps emerge in a finite value of the dipole-dipole and on-site interactions. In the quarter filling case, s-wave superconducting state, charge density wave, homogenous insulating and phase separation phases occur depend on the interaction values. Moreover, in the dipole-dipole interaction, the D-Mott phase emerges when the hopping terms along the chain and rung are the same, whereas, this phase has been only proposed for the anisotropic Hubbard model. In the half filling case, on the other hand, there is either charge-density wave or charged Mott order phase depends on the orientation of the dipole moments of the particles with respect to the ladder geometry.
Dipoles in triangular optical ladders constitute a flexible platform for the study of the interplay between geometric frustration and long-range anisotropic interactions, and in particular for the observation of the spontaneous onset of chirality. Frustration magnifies the effect of the dipolar interactions in itinerant polarized dipolar bosons. As a result, the dipole-induced transition between a chiral superfluid and a nonchiral two-component superfluid may be observed for current state-of-the-art temperatures even for the weak intersite interaction characterizing magnetic atoms in standard optical lattices. On the other hand, pinned spin- 1 / 2 dipoles, which we discuss in the context of polar molecules in two rotational states, realize frustrated dipolar XXZ spin models. By controlling the external electric field strength and orientation, these systems can explore a rich ground-state landscape including chiral and nematic phases, as well as intriguing chiral dynamics.
We employ large-scale density matrix renormalization group calculations to study the quantum phases of dipolar molecules confined in bent (zigzag) endofullerene chains, as a function of the chain angle γγγ. For LiF, ferroelectric order persists across the full range 60∘<γ180∘60^\circ < γ180^\circ60∘<γ180∘, with the critical effective dipole moment increasing as the chain bends and parallel alignment becomes less favorable. Near the equilateral configuration (γ=60∘γ= 60^\circγ=60∘), geometric frustration drives a transition to an antiferroelectric Néel-ordered phase in which neighboring dipoles anti-align along the chain axis. We show that capturing this reorientation requires including dipolar couplings beyond the nearest-neighbor approximation, since next-nearest-neighbor interactions become equally strong at γ=60∘γ= 60^\circγ=60∘. For confined water, o-D2_22​O reproduces both ordered phases, whereas p-H2_22​O -- owing to its large rotational constants -- develops no order at any chain angle despite the enhanced coordination of the bent geometry. Because a zigzag chain is the narrowest stripe of a two-dimensional lattice, these results suggest that engineered endofullerene layers could host a rich variety of dipole-ordered quantum phases beyond the ferroelectric ordering observed in previous work.
We derive a Hamiltonian for a two-leg ladder which includes an arbitrary number of charge and spin interactions which must be weak but are otherwise of arbitrary strength. To illustrate this Hamiltonian we consider two examples and use a renormalization-group technique to evaluate the ground-state phases. The first example is a two-leg ladder with zigzagged legs. We find that increasing the number of interactions in such a two-leg ladder may result in a richer phase diagram, particularly at half-filling where a few exotic phases are possible when the number of interactions are large and the angle of the zigzag is small. In the second example we determine under which conditions a two-leg ladder at quarter-filling is able to support a Tomanaga-Luttinger liquid phase. We show that this is only possible when the spin interactions across the rungs are ferromagnetic. In both examples we focus on lithium purple bronze, a two-leg ladder with zigzagged legs which is thought to support a Tomanaga-Luttinger liquid phase.
This thesis is devoted to the study of dipolar lattice gases, i.e. many-body quantum systems of particles with a strong magnetic or electric dipole moment in optical lattices. Such systems are adequately described by the extended Hubbard model, which accounts for inter-site dipole-dipole interactions (DDI). These interactions, due to their long-range and anisotropic character, result in rich groundstate physics and intriguing dynamics as we illustrate in this thesis for the particular case of bosons in one- and quasi-one-dimensional lattices. We start by focusing on the non-trivial role played by the transversal confinement in one-dimensional dipolar lattice gases. We show that weakening the transversal confinement enhances beyond-nearest-neighbor interactions. Then, we analyze how this affects the ground-state physics of hard-core bosons with repulsive dipolar interactions and reveal quantitative differences to the standard case of the DDI falling off as 1/r^3 where r is the inter-particle distance. With attractive interactions, a new quantum liquid phase of self-bound lattice droplets emerges without the need for super-exchange processes. In the soft-core regime, proper consideration of the transversal confinement not only quantitatively shifts phase boundaries, but introduces novel phases with peculiar correlations in the site occupancies that may be either topological or topologically trivial. Furthermore, we study the effect of the transversal confinement on the dynamical properties of one-dimensional hard-core bosons at half-filling. We show in particular that the localization-to-delocalization transition induced by Hilbert space fragmentation resembles that of a system with an effective power-law decay different from 1/r^3 which can be controlled by the transversal confinement. To conclude this thesis, we analyze ground-state properties of hard-core dipolar bosons in a square ladder at unit rung filling with an energy bias between the two legs. We show that the interplay between the energy bias and the dipolar tail results in a peculiar topological quantum floating phase.