We show that quantum square ice-namely, the two-dimensional version of proton or spin ice with tunable quantum tunneling of the electric or magnetic dipole moment-exhibits a quantum spin-liquid phase supporting fractionalized spinons. This phase corresponds to a thermally induced, deconfined quantum Coulomb phase of a two-dimensional lattice gauge theory. It emerges at finite, yet exceedingly low temperatures from the melting of two distinct order-by-disorder phases appearing in the ground state: a plaquette valence-bond solid for low tunneling; and a canted Néel state for stronger tunneling. The latter phases appear via the highly nonlinear effect of quantum fluctuations within the degenerate manifold of ice-rule states, and they can be identified as the two competing ground states of a discrete lattice gauge theory (quantum link model) emerging as the effective Hamiltonian of the system within degenerate perturbation theory.
We show that quantum square ice-namely, the two-dimensional version of proton or spin ice with tunable quantum tunneling of the electric or magnetic dipole moment-exhibits a quantum spin-liquid phase supporting fractionalized spinons. This phase corresponds to a thermally induced, deconfined quantum Coulomb phase of a two-dimensional lattice gauge theory. It emerges at finite, yet exceedingly low temperatures from the melting of two distinct order-by-disorder phases appearing in the ground state: a plaquette valence-bond solid for low tunneling; and a canted Néel state for stronger tunneling. The latter phases appear via the highly nonlinear effect of quantum fluctuations within the degenerate manifold of ice-rule states, and they can be identified as the two competing ground states of a discrete lattice gauge theory (quantum link model) emerging as the effective Hamiltonian of the system within degenerate perturbation theory.
At sufficiently low temperatures, interacting electron systems tend to develop orders. Exceptions are quantum critical point (QCP) and quantum spin liquid (QSL), where fluctuations prevent the highly entangled quantum matter to an ordered state down to the lowest temperature. While the ramification of these states may have appeared in high-temperature superconductors, ultracold atoms, frustrated magnets, and quantum moir\'e materials, their unbiased presence remains elusive in microscopic two-dimensional lattice models. Here, we show, by means of large-scale quantum Monte Carlo simulations of correlated electrons on the $\ensuremath{\pi}$-flux square lattice subjected to plaquette Hubbard interaction, that a Gross-Neveu QCP separating massless Dirac fermions and a columnar valence bond solid at finite interaction and a possible Dirac QSL at the infinite yet tractable interaction limit emerge in a coherent sequence. These unexpected quantum states reside in this simple-looking model, unifying ingredients including emergent symmetry, deconfined fractionalization, and the dynamic coupling between emergent matter and gauge fields and will have profound implications both in quantum many-body theory and understanding of the aforementioned experimental systems.
Three dimensional frustrated magnets realized in the rare-earth pyrochlores R_2B_2O_7, R=rare-earth ion, B transition metal ion) have attracted much interest since the discovery of spin ice in Ho_2Ti_2O_7 by Harris et al. Since then, a number of interesting phenomena in pyrochlore magnets have been observed and the interest in these systems, from an experimental and theoretical point of view, has nothing but increased. Perhaps the most appealing and unique possibility is that these systems may realize a quantum disordered phase; a so-called quantum spin ice. Theoretically, it has been predicted by Hermele et al. that a U(1) quantum spin liquid is realized in the XXZ quantum spin ice (with global U(1)xZ_2 symmetry) in the perturbative regime and more recently Savary and Balents have introduced a quantum rotor model with bosonic spinons coupled to U(1) gauge fields to describe non-peturbatively the deconfined phase predicted. They studied an anisotropic quantum spin ice (QSI) model which corresponds to the XXZ QSI with an additional anisotropic coupling. They solved the quantum rotor model using a mean-field approximation combined with a large-N approximation and predicted the possibility of a U(1) liquid in addition to an exotic ferromagnetic phase. Further work by Lee et al. has addressed the more complicated fully frustrated XXZ quantum spin ice regime, where all components of the model are frustrated, by using some insights provided by the previous perturbative results. \n \nIn this thesis, we will address the non-perturbative regime of the fully frustrated XXZ QSI beyond the simplest perturbative treatment. We will begin by mapping the quantum spin ice model to a compact U(1) gauge theory with deconfined electric and magnetic monopoles. Neglecting the interaction between the gapless photon excitation and the electric charges, we will study the matter sector with only electric charges, the so-called spinons. Building up on insights provided by high order degenerate perturbation theory calculations, we will construct some symmetric spin liquid ansatz for the static part of the gauge fields. The two novel spin liquids that we construct break time reversal symmetry and thus have a non-trivial chirality. In order to solve the matter sector of the theory and determine the stability of the deconfined phases, we will introduce a novel representation of a XY quantum rotor in terms of ``exclusive" bosons, a representation which is dynamically implemented in the dilute limit. We will benchmark this mapping in different ways by comparing our results with Quantum Monte Carlo simulations and exact diagonalization in some limiting cases. Using this mapping we will compute the region of stability of the U(1) liquid phase of XXZ QSI. Within this mapping we will reproduce qualitatively the results of previous work by finding only the so-called zero and \\pi-flux U(1) liquids in the vicinity of the classical spin ice point, while improving greatly on the estimation of the exchange coupling at which the bosonic spinons condense to form a superfluid phase. In the fully frustrated XXZ QSI, we will provide evidence, using exact diagonalization of the quantum rotor model, that one of the chiral spin liquid may be realized in the strongly correlated and frustrated QSI regime, where all previous approximations break down.
Quantum spin-ice represents a paradigmatic example of how the physics of frustrated magnets is related to gauge theories. In the present work, we address the problem of approximately realizing quantum spin ice in two dimensions with cold atoms in optical lattices. The relevant interactions are obtained by weakly laser-admixing Rydberg states to the atomic ground-states, exploiting the strong angular dependence of van der Waals interactions between Rydberg p states together with the possibility of designing steplike potentials. This allows us to implement Abelian gauge theories in a series of geometries, which could be demonstrated within state-of-the-art atomic Rydberg experiments. We numerically analyze the family of resulting microscopic Hamiltonians and find that they exhibit both classical and quantum order by disorder, the latter yielding a quantum plaquette valence bond solid. We also present strategies to implement Abelian gauge theories using both s- and p-Rydberg states in exotic geometries, e.g., on a 4-8 lattice.
We explore the ground-state physics of two-dimensional spin-1/2 U(1) quantum link models, one of the simplest nontrivial lattice gauge theories with fermionic matter within experimental reach for quantum simulations. Whereas in the large mass limit we observe Neél-like vortex-antivortex and striped crystalline phases, for small masses there is a transition from the striped phases into a disordered phase whose properties resemble those at the Rokhsar-Kivelson point of the quantum dimer model. This phase is characterized on ladders by boundary Haldane-like properties, such as vanishing parity and finite string ordering. Moreover, from studies of the string tension between gauge charges, we find that, whereas the striped phases are confined, the novel disordered phase present clear indications of being deconfined. Our results open exciting perspectives of studying highly nontrivial physics in quantum simulators, such as spin-liquid behavior and confinement-deconfinement transitions, without the need of explicitly engineering plaquette terms.
The low-energy physics of quantum spin ice is known to support an emergent form of quantum electrodynamics (QED), where magnetic monopoles exist and the fine-structure constant is material dependent. In this article, we show how this QED is modified via a coupling to dynamical matter on the centered pyrochlore lattice, a structure that has recently been synthesized using metal-organic frameworks. Specifically, we study the low-energy properties of the S = 1 / 2 quantum XXZ model on the centered pyrochlore lattice, with a focus on the sign-problem-free region. At fourth order in degenerate perturbation theory, this model hosts a quantum spin liquid distinct from the well-known U(1) quantum spin ice on the pyrochlore because of the presence of dynamical matter in the ground state. Exact diagonalization results are consistent with this quantum spin liquid over an extended region of the ground-state phase diagram, although potential quantum critical points within this region could indicate a richer phase structure. Our work thus expands the physics of quantum spin ice in an experimentally motivated geometry, showing how the emergent QED can be coupled to dynamical matter at zero temperature.
Quantum fluctuations of the Néel state of the square lattice antiferromagnet are usually described by a CP 1 theory of bosonic spinons coupled to a U(1) gauge field, and with a global SU(2) spin rotation symmetry.Such a theory also has a confining phase with valence bond solid (VBS) order, and upon including spin-singlet charge-2 Higgs fields, deconfined phases with Z 2 topological order possibly intertwined with discrete broken global symmetries.We present dual theories of the same phases starting from a mean-field theory of fermionic spinons moving in π flux in each square lattice plaquette.Fluctuations about this π-flux state are described by (2 þ 1)-dimensional quantum chromodynamics (QCD 3 ) with a SU(2) gauge group and N f ¼ 2 flavors of massless Dirac fermions.It has recently been argued by Wang et al. [Deconfined Quantum Critical Points: Symmetries and Dualities, Phys. Rev. X 7, 031051 (2017).]that this QCD 3 theory describes the Néel-VBS quantum phase transition.We introduce adjoint Higgs fields in QCD 3 and obtain fermionic dual descriptions of the phases with Z 2 topological order obtained earlier using the bosonic CP 1 theory.We also present a fermionic spinon derivation of the monopole Berry phases in the U(1) gauge theory of the VBS state.The global phase diagram of these phases contains multicritical points, and our results imply new boson-fermion dualities between critical gauge theories of these points.