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Quantum Spin-Ice and Dimer Models with Rydberg Atoms

Alexander W. Glaetzle, Marcello Dalmonte, Ramesh Nath (4116697), Ioannis Rousochatzakis, Roderich Moessner, P. Zoller

Published Nov 25, 2014• 137 citations
OpenAlex

Abstract

Quantum spin-ice represents a paradigmatic example of how the physics of frustrated magnets is related to gauge theories. In the present work, we address the problem of approximately realizing quantum spin ice in two dimensions with cold atoms in optical lattices. The relevant interactions are obtained by weakly laser-admixing Rydberg states to the atomic ground-states, exploiting the strong angular dependence of van der Waals interactions between Rydberg p states together with the possibility of designing steplike potentials. This allows us to implement Abelian gauge theories in a series of geometries, which could be demonstrated within state-of-the-art atomic Rydberg experiments. We numerically analyze the family of resulting microscopic Hamiltonians and find that they exhibit both classical and quantum order by disorder, the latter yielding a quantum plaquette valence bond solid. We also present strategies to implement Abelian gauge theories using both s- and p-Rydberg states in exotic geometries, e.g., on a 4-8 lattice.

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•Jul 8, 2015•0 citations
Quantum spin-ice represents a paradigmatic example of how the physics of frustrated magnets is related to gauge theories. In the present work, we address the problem of approximately realizing quantum spin ice in two dimensions with cold atoms in optical lattices. The relevant interactions are obtained by weakly laser-admixing Rydberg states to the atomic ground-states, exploiting the strong angular dependence of van der Waals interactions between Rydberg p states together with the possibility of designing steplike potentials. This allows us to implement Abelian gauge theories in a series of geometries, which could be demonstrated within state-of-the-art atomic Rydberg experiments. We numerically analyze the family of resulting microscopic Hamiltonians and find that they exhibit both classical and quantum order by disorder, the latter yielding a quantum plaquette valence bond solid. We also present strategies to implement Abelian gauge theories using both s- and p-Rydberg states in exotic geometries, e.g., on a 4-8 lattice.
We show how a broad class of lattice spin-1/2 models with angular- and distance-dependent couplings can be realized with cold alkali atoms stored in optical or magnetic trap arrays. The effective spin-1/2 is represented by a pair of atomic ground states, and spin-spin interactions are obtained by admixing van der Waals interactions between fine-structure split Rydberg states with laser light. The strengths of the diagonal spin interactions as well as the "flip-flop," and "flip-flip" and "flop-flop" interactions can be tuned by exploiting quantum interference, thus realizing different spin symmetries. The resulting energy scales of interactions compare well with typical temperatures and decoherence time scales, making the exploration of exotic forms of quantum magnetism, including emergent gauge theories and compass models, accessible within state-of-the-art experiments.
Solving strongly coupled gauge theories in two or three spatial dimensions is of fundamental importance in several areas of physics ranging from high-energy physics to condensed matter.On a lattice, gauge invariance and gauge-invariant (plaquette) interactions involve (at least) four-body interactions that are challenging to realize.Here, we show that Rydberg atoms in configurable arrays realized in current tweezer experiments are the natural platform to realize scalable simulators of the Rokhsar-Kivelson Hamiltonian-a 2D U(1) lattice gauge theory that describes quantum dimer and spin-ice dynamics.Using an electromagnetic duality, we implement the plaquette interactions as Rabi oscillations subject to Rydberg blockade.Remarkably, we show that by controlling the atom arrangement in the array we can engineer anisotropic interactions and generalized blockade conditions for spins built of atom pairs.We describe how to prepare the resonating valence bond and the crystal phases of the Rokhsar-Kivelson Hamiltonian adiabatically and probe them and their quench dynamics by on-site measurements of their quantum correlations.We discuss the potential applications of our Rydberg simulator to lattice gauge theory and exotic spin models.
Quantum spin liquids are exotic phases of matter whose low-energy physics is described as the deconfined phase of an emergent gauge theory. With recent theory proposals and an experiment showing preliminary signs of Z 2 topological order [G. Semeghini , ], Rydberg atom arrays have emerged as a promising platform to realize a quantum spin liquid. In this work, we propose a way to realize a U(1) quantum spin liquid in three spatial dimensions, described by the deconfined phase of U(1) gauge theory in a pyrochlore lattice Rydberg atom array. We study the ground state phase diagram of the proposed Rydberg system as a function of experimentally relevant parameters. Within our calculation, we find that by tuning the Rabi frequency, one can access both the confinement-deconfinement transition driven by a proliferation of “magnetic” monopoles and the Higgs transition driven by a proliferation of “electric” charges of the emergent gauge theory. We suggest experimental probes for distinguishing the deconfined phase from ordered phases. This work serves as a proposal to access a confinement-deconfinement transition in three spatial dimensions on a Rydberg-based quantum simulator.
Interacting ultracold atomic quantum gases provide an ideal test bed to study strongly correlated quantum matter. The interactions between atoms in such an ultracold quantum gas are typically short-ranged and well described by an effective contact potential. Introducing longer-range interactions promises the realization of novel quantum phases which are absent in systems with only short-range interactions. Trapped atoms, resonantly laser-coupled to highly excited, strongly interacting Rydberg states have been proposed as a versatile platform to realize such long-range interacting quantum matter. In a first experiment presented in this thesis, we combined the single-atom-sensitive local preparation and detection enabled by a quantum gas microscope to prepare and microscopically characterize an ensemble of rubidium-87 atoms trapped in an optical lattice in the regime of strong Rydberg blockade. There, we observe collectively enhanced optical coupling in an effective two-level system, the so-called “superatom”, and infer the presence of entanglement. Detuned optical coupling to Rydberg states, termed “Rydberg dressing”, has been proposed as an alternative approach to induce long-range interactions. Rather than directly exciting an atom to a Rydberg state, the properties of the latter are admixed to a ground state, which consequently acquires long-range interactions. In the context of this thesis, we have designed a laser system in the ultraviolet spectral range to admix Rydberg P-state character to the ground state of atoms in an optical lattice. In an emerging Ising quantum magnet, the presence of Rydberg-dressed interactions was demonstrated by an interferometric technique combined with spatially resolved spin correlation measurements. The theoretically predicted tunability of the isotropy and range of the interaction were confirmed experimentally. While these initial measurements exhibited unexpected dissipation, in a subsequent experiment in a one-dimensional spin chain this dissipation was overcome. We substantiated the improved coherence times by tracking the time evolution of the magnetization upon suddenly switching on interactions and observing coherent collapse and revival dynamics, one of the hallmarks of coherent quantum evolution. Our results establish Rydberg-dressed interactions in ultracold gases and pave the way to realize and study novel exotic quantum phases.
Recent achievements in ultra-cold experiments have made quantum simulation of interacting many-body systems possible in a well controllable environment. Of many candidates as quantum simulators, Rydberg atoms have been extensively utilised due to its exaggerated and fascinating atomic properties. Example includes high susceptibility to electric fields and relatively long life time in comparison to atoms in low-lying states. The tunable interaction between Rydberg atoms have made them even more versatile in simulating quantum many-body systems, e.g. interacting spin-1/2 particles. We will start the thesis by reviewing these properties of Rydberg atoms and explain how they lead to the Rydberg lattice gases that of interest. Following the review of the essential knowledge of Rydberg atoms, we first study the ground states of interacting Rydberg lattice gases in both one-dimension and two-dimensions. The many-body system we are interested in is initially prepared in a Mott-insulator state, with each lattice site containing one atom that is laser coupled to its highly excited Rydberg state. The extremely huge van der Waals interactions between Rydberg atoms at close distance leads to an interesting Rydberg blockade effect. As we shall show, these strong interactions lead to rich phases and critical behaviours in the ground states of the many-body Hamiltonians that describes the systems. The aim of the first three chapters is to analyse these ground states in detail. Having investigated the static properties, we then move on to study the dynamical behaviour of a class of generic spin models which can in principal be realised by Rydberg lattice gases with tunable blockade radius. By deriving an effective master equation, and comparing it to the exact calculation, we will demonstrate how different pure initial states eventually evolve to the same equilibrium state and analysed in detail the time evolution and the steady state.