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arXiv:1306.0690 · Physical Review Letters

Dynamical Steady States in Driven Quantum Systems

Thomas M. Stace, Andrew C. Doherty, D. J. Reilly

Published Oct 30, 2013• 25 citations
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Abstract

We derive dynamical equations for a driven, dissipative quantum system in which the environment-induced relaxation rate is comparable to the Rabi frequency, avoiding assumptions on the frequency dependence of the environmental coupling. When the environmental coupling varies significantly on the scale of the Rabi frequency, secular or rotating wave approximations break down. We avoid these approximations, yielding dynamical steady states which account for the interaction between driven quantum dots and their phonon environment. The theory, which is motivated by recent experimental observations, qualitatively and quantitatively describes the transition from asymmetric unsaturated resonances at weak driving to population inversion at strong driving.

DOI
10.1103/physrevlett.111.180602

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We derive dynamical equations for a driven, dissipative quantum system in which the environment-induced relaxation rate is comparable to the Rabi frequency, avoiding assumptions on the frequency dependence of the environmental coupling. When the environmental coupling varies significantly on the scale of the Rabi frequency, secular or rotating wave approximations break down. We avoid these approximations, yielding dynamical steady states which account for the interaction between driven quantum dots and their phonon environment. The theory, which is motivated by recent experimental observations, qualitatively and quantitatively describes the transition from asymmetric unsaturated resonances at weak driving to population inversion at strong driving.
The Rabi model considers a two-level system (or spin 1/2) coupled to a quantized harmonic oscillator and describes the simplest interaction between matter and light. The recent experimental progress in solid-state circuit quantum electrodynamics has engendered theoretical efforts to quantitatively describe the mathematical and physical aspects of the light-matter interaction beyond the rotating-wave approximation. We develop a stochastic Schr\"odinger equation approach which enables us to access the strong-coupling limit of the Rabi model and study the effects of dissipation and ac drive in an exact manner. We include the effect of Ohmic noise on the non-Markovian spin dynamics, resulting in Kondo-type correlations, as well as cavity losses. We compute the time evolution of spin variables in various conditions. As a consideration for future work, we discuss the possibility of reaching a steady state with one polariton in realistic experimental conditions.
We study optically driven Rabi rotations of a quantum dot exciton transition between 5 and 50 K, and for pulse areas of up to 14π. In a high driving field regime, the decay of the Rabi rotations is nonmonotonic, and the period decreases with pulse area and increases with temperature. By comparing the experiments to a weak-coupling model of the exciton-phonon interaction, we demonstrate that the observed renormalization of the Rabi frequency is induced by fluctuations in the bath of longitudinal acoustic phonons, an effect that is a phonon analogy of the Lamb shift.
We show that the interaction between carriers confined in a quantum dot and the surrounding lattice under external driving of carrier dynamics has a dynamical, resonant character. The quality of Rabi oscillations in such a system depends on the relation between nonlinear spectral characteristics of the driven dynamics and the spectral density of effectively coupled lattice modes (phonon frequencies and density of states). For a large number of Rabi oscillations within a fixed time (allowed by, e.g., exciton recombination) the spectrum of the dynamics extends towards high frequencies, coming into resonance with acoustic and optical phonons. Thus, this resonant lattice response strongly restricts the possibility of fully coherent control over the charge state in a quantum dot.
Understanding quantum coherence and proposing protection mechanisms has become one of the fundamental challenges in quantum physics research. We investigate a generic driven open quantum system, i.e., the driven spin-boson model, beyond the rotating-wave approximation. Although steady-state coherence vanishes in Floquet-Markov and Bloch-Redfield approaches, it becomes finite within a time-non-local master equation with a memory kernel. We analytically reveal that the steady-state coherence is associated with the overlap between the spectral densities associated with neighboring Floquet quasifrequencies. Motivated by this, we show that increasing temperature and introducing mixed transverse and longitudinal baths broadens the spectral density, thereby enhancing steady-state coherence. This is described by resonance fluorescence spectra, which exhibit clear spectral broadening and enhanced steady-state values. For a transverse dissipative coupling to the bath, three transition frequencies emerge in the Floquet basis, corresponding to the Mollow triplet. For weak resonant driving, these quasienergies become nearly degenerate, leading to closely spaced peaks in the resonance fluorescence spectrum, and the steady-state quantum coherence asymptotically approaches its maximum. For a longitudinal coupling to the bath, the quantum system exhibits a single transition frequency, thereby resulting in a complete suppression of the steady-state quantum coherence. We systematically investigate the influences of driving strength, frequency, temperature, and various dissipative baths on steady-state quantum coherence. These findings provide a foundational framework for efficiently engineering steady-state quantum coherence in nanoscale open quantum devices under optical field excitation.
Semiconductor quantum dots (SQDs) exhibit optical responses that are strongly influenced by their internal level structure, relaxation pathways, and excitation intensity. This study investigates the time- and intensity-dependent population dynamics of a continuously driven single -type three-level SQD using the density-matrix formalism within the rotating-wave approximation. Dissipative processes are incorporated through Lindblad-type relaxation terms, while the transient and stationary responses are obtained, respectively, by numerical time integration and steady-state solution of the density-matrix equations. Special attention is given to the relaxation channel and the off-resonant transition dipole moment . The results show that primarily controls the transient redistribution route and the timescale required to reach the stationary regime, whereas the early oscillatory behavior remains dominated by the resonantly driven transition. In the steady-state regime, mainly determines how population leaving the upper state is partitioned between the two lower states, while governs how readily the off-resonant branch becomes active as the driving intensity increases. Consequently, the crossover from predominantly resonant two-level-like behavior to genuine three-level population redistribution is controlled by the combined action of relaxation-path asymmetry and off-resonant coupling strength. These findings provide a clearer mechanism-based interpretation of driven population redistribution in effective multilevel SQD systems.
We explore the dynamics and the steady state of a driven quantum spin coupled to a bath of fermions, which can be realized with a strongly imbalanced mixture of ultracold atoms using currently available experimental tools. Radio-frequency driving can be used to induce tunneling between the spin states. The Rabi oscillations are modified due to the coupling of the quantum spin to the environment, which causes frequency renormalization and damping. The spin-bath coupling can be widely tuned by adjusting the scattering length through a Feshbach resonance. When the scattering potential creates a bound state, by tuning the driving frequency it is possible to populate either the ground state, in which the bound state is filled, or a metastable state in which the bound state is empty. In the latter case, we predict an emergent inversion of the steady-state magnetization. Our work shows that different regimes of dissipative dynamics can be explored with a quantum spin coupled to a bath of ultracold fermions.