Ising models, and the physical systems described by them, play a central role in generating entangled states for use in quantum metrology and quantum information.In particular, ultracold atomic gases, trapped ion systems, and Rydberg atoms realize long-ranged Ising models, which even in the absence of a transverse field can give rise to highly non-classical dynamics and long-range quantum correlations.In the first part of this paper, we present a detailed theoretical framework for studying the dynamics of such systems driven (at time t = 0) into arbitrary unentangled non-equilibrium states, thus greatly extending and unifying the work of Foss-Feig et al (2013 Phys.Rev. A 87 042101).Specifically, we derive exact expressions for closed-time-path ordered correlation functions, and use these to study experimentally relevant observables, e.g.Bloch vector and spin-squeezing dynamics.In the second part, these correlation functions are then used to derive closed-form expressions for the dynamics of arbitrary spin-spin correlation functions in the presence 5
Ising models, and the physical systems described by them, play a central role in generating entangled states for use in quantum metrology and quantum information.In particular, ultracold atomic gases, trapped ion systems, and Rydberg atoms realize long-ranged Ising models, which even in the absence of a transverse field can give rise to highly non-classical dynamics and long-range quantum correlations.In the first part of this paper, we present a detailed theoretical framework for studying the dynamics of such systems driven (at time t = 0) into arbitrary unentangled non-equilibrium states, thus greatly extending and unifying the work of Foss-Feig et al (2013 Phys.Rev. A 87 042101).Specifically, we derive exact expressions for closed-time-path ordered correlation functions, and use these to study experimentally relevant observables, e.g.Bloch vector and spin-squeezing dynamics.In the second part, these correlation functions are then used to derive closed-form expressions for the dynamics of arbitrary spin-spin correlation functions in the presence 5
The interplay between interactions and decoherence in many-body systems is of fundamental importance in quantum physics. In a step toward understanding this interplay, we obtain an exact analytic solution for the nonequilibrium dynamics of Ising models with arbitrary couplings (and therefore in arbitrary dimension) and subject to local Markovian decoherence. Our solution shows that decoherence significantly degrades the nonclassical correlations developed during coherent Ising spin dynamics, which relax much faster than predicted by treating decoherence and interactions separately. We also show that the competition of decoherence and interactions induces a transition from oscillatory to overdamped dynamics that is absent at the single-particle or mean-field level. These calculations are applicable to ongoing quantum information and emulation efforts using a variety of atomic, molecular, optical, and solid-state systems. In particular, we apply our results to the NIST Penning trapped-ion experiment and show that the current experiment is capable of producing entanglement amongst hundreds of quantum spins.
Theoretical models of spins coupled to bosons provide a simple setting for studying a broad range of important phenomena in many-body physics, from virtually mediated interactions to decoherence and thermalization. In many atomic, molecular, and optical systems, such models also underlie the most successful attempts to engineer strong, long-ranged interactions for the purpose of entanglement generation. Especially when the coupling between the spins and bosons is strong, such that it cannot be treated perturbatively, the properties of such models are extremely challenging to calculate theoretically. Here, exact analytical expressions for nonequilibrium spin-spin correlation functions are derived for a specific model of spins coupled to bosons. The spatial structure of the coupling between spins and bosons is completely arbitrary, and thus the solution can be applied to systems in any number of dimensions. The explicit and nonperturbative inclusion of the bosons enables the study of entanglement generation (in the form of spin squeezing) even when the bosons are driven strongly and near resonantly, and thus provides a quantitative view of the breakdown of adiabatic elimination that inevitably occurs as one pushes towards the fastest entanglement generation possible. The solution also helps elucidate the effect of finite temperature on spin squeezing. The model considered is relevant to a variety of atomic, molecular, and optical systems, such as atoms in cavities or trapped ions. As an explicit example, the results are used to quantify phonon effects in trapped ion quantum simulators, which are expected to become increasingly important as these experiments push towards larger numbers of ions.
The quantum simulation of complex many body systems holds promise for understanding the origin of emergent properties of strongly correlated systems, such as high-Tc superconductors and spin liquids. Cold atomic systems provide an almost ideal platform for quantum simulation due to their excellent quantum coherence, initialization and readout properties, and their ability to support several forms of interactions. In this thesis, I present experiments on the quantum simulation of long range Ising models in the presence of transverse magnetic fields with a chain of up to sixteen ultracold 171-Yb+ ions trapped in a linear radio frequency Paul trap. Two hyperfine levels in each of the 171-Yb+ ions serve as the spin-1/2 systems. We detect the spin states of the individual ions by observing state-dependent fluorescence with single site resolution, and can directly measure any possible spin correlation function. The spin-spin interactions are engineered by applying dipole forces from precisely tuned lasers whose beatnotes induce stimulated Raman transitions that couple virtually to collective phonon modes of the ion motion. The Ising couplings are controlled, both in sign and strength with respect to the effective transverse field, and adiabatically manipulated to study various aspects of this spin model, such as the emergence of a quantum phase transition in the ground state and spin frustration due to competing antiferromagnetic interactions. Spin frustration often gives rise to a massive degeneracy in the ground state, which can lead to entanglement in the spin system. We detect and characterize this frustration induced entanglement in a system of three spins, demonstrating the first direct experimental connection between frustration and entanglement. With larger numbers of spins we also vary the range of the antiferromagnetic couplings through appropriate laser tunings and observe that longer range interactions reduce the excitation energy and thereby frustrate the ground state order. This system can potentially be scaled up to study a wide range of fully connected spin networks with a few dozens of spins, where the underlying theory becomes intractable on a classical computer.
By applying complementary analytic and numerical methods, we investigate the dynamics of spin-21XXZ models with variable-range interactions in arbitrary dimensions. The dynamics we consider is initiated from uncorrelated states that are easily prepared in experiments; it can be equivalently viewed as either Ramsey spectroscopy or a quantum quench. Our primary focus is the dynamical emergence of correlations and entanglement in these far-from-equilibrium interacting quantum systems: We characterize these correlations by the entanglement entropy, concurrence, and squeezing, which are inequivalent measures of entanglement corresponding to different quantum resources. In one spatial dimension, we show that the time evolution of correlation functions manifests a nonperturbative dynamic singularity. This singularity is characterized by a universal power-law exponent that is insensitive to small perturbations. Explicit realizations of these models in current experiments using polar molecules, trapped ions, Rydberg atoms, magnetic atoms, and alkaline-earth and alkali-metal atoms in optical lattices, along with the relative merits and limitations of these different systems, are discussed.
The study of quantum dynamics is an increasingly important aspect of atomic, molecular and optical physics, as well as condensed-matter physics and other disciplines. It is essential in order to understand non-equilibrium phenomena which do not fit within the framework of equilibrium thermodynamics, such as many-body localization, dynamical quantum phase transitions, and non-equilibrium steady states in driven-dissipative systems. However, the exact calculation of dynamical observables is extremely difficult in general for several reasons, which makes it challenging for theoretical predictions and analyses to keep pace with rapidly advancing experiments. In this thesis I use and develop several computational methods to investigate the dynamics of quantum many-body systems, with the two goals of better understanding the evolution of local observables and correlation functions in spin and Fermion systems as well as creating and testing more effective numerical methods for solving quantum dynamics problems. I explore quantum dynamics by using Hamiltonian parameter quenches in several commonly-used models in AMO physics and elsewhere: the Fermi-Hubbard model, the XXZ model, and the transverse-Ising model. The first represents a system of short-range interacting Fermions, while the latter two represent spin systems with different spin-spin couplings and magnetic field terms. All of these models can be realized in current experiments. First, I derive an exact solution for an extreme interaction quench in the Fermi-Hubbard model, from a strongly-interacting initial state to a noninteracting final Hamiltonian. From this result I show that there are nontrivial transient connected correlations, despite the fact that the system has very high temperature and a noninteracting Hamiltonian. Those features would suppress such correlations in equilibrium, but the dynamical correlations are still significant. Then, I develop and examine two numerical methods for solving dynamics of the spin expectation values and correlation functions in the transverse-Ising and XXZ models. Both methods rely on approximating a thermodynamically large system with a much smaller and more computationally tractable cluster of lattice sites, or a series of clusters. The first method is a dynamical numerical linked cluster expansion (NLCE). NLCEs have already been used successfully on systems in thermodynamic equilibrium, and I extended the technique to directly compute the dynamics of an observable after a quantum quench. I review the general NLCE method, describe my dynamical variant of it, and compute the quench dynamics of spin and correlation observables in the transverse-Ising and XXZ models. The second method, which I term the adaptive-boundary cluster method, relies on recently refined bounds on information propagation in quantum systems to choose a cluster of lattice sites that minimizes the finite size error bound of a dynamical computation. I briefly review these bounds, and describe a new algorithm which uses them to construct a cluster whose boundary is chosen according to a related error estimate. Such an adaptive-boundary cluster has the property that there exists a computable upper bound on the finite size error of observables measured at the cluster center, and this error bound is nearly minimal when compared to that of other clusters of the same size. I then compute the quench dynamics of spin and correlation observables in the transverse-Ising model using the adaptive boundary clusters. I apply this method to both uniform and strongly disordered systems. To evaluate the effectiveness of both dynamical NLCE and adaptive-boundary clusters, I compare the results obtained using them to results from a standard and general purpose numerical method: exact solvers applied a rectangular cluster with periodic boundary conditions. Both of the new methods usually converge faster and are more accurate than the standard method for comparable cluster sizes. This thesis illustrates that choosing numerical methods which take advantage of the geometric and entanglement structure of the initial state and Hamiltonian can substantially enhance our ability to study quantum dynamics, by reducing the computational cost of numerically exact solutions. I conclude with a discussion of various avenues for future research to build on this work.
Quantum simulation of spin models can provide insight into problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. We studied quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of (9)Be(+) ions in a Penning trap. We verified entanglement in spin-squeezed states of up to 219 ions, directly observing 4.0 ± 0.9 decibels of spectroscopic enhancement, and observed states with non-Gaussian statistics consistent with oversqueezed states. The good agreement with ab initio theory that includes interactions and decoherence lays the groundwork for simulations of the transverse-field Ising model with variable-range interactions, which are generally intractable with classical methods.