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arXiv:1305.6942 · Nature Communications

Observation of non-Markovian micromechanical Brownian motion

Simon Gröblacher, Alexey Trubarov, N. Prigge, Garrett D. Cole, Markus Aspelmeyer, Jens Eisert

Published Jul 28, 2015• 199 citations
arXivHTMLPDF

Abstract

All physical systems are to some extent open and interacting with their environment. This insight, basic as it may seem, gives rise to the necessity of protecting quantum systems from decoherence in quantum technologies and is at the heart of the emergence of classical properties in quantum physics. The precise decoherence mechanisms, however, are often unknown for a given system. In this work, we make use of an opto-mechanical resonator to obtain key information about spectral densities of its condensed-matter heat bath. In sharp contrast to what is commonly assumed in high-temperature quantum Brownian motion describing the dynamics of the mechanical degree of freedom, based on a statistical analysis of the emitted light, it is shown that this spectral density is highly non-Ohmic, reflected by non-Markovian dynamics, which we quantify. We conclude by elaborating on further applications of opto-mechanical systems in open system identification.

DOI
10.1038/ncomms8606

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All physical systems are to some extent open and interacting with their environment. This insight, basic as it may seem, gives rise to the necessity of protecting quantum systems from decoherence in quantum technologies and is at the heart of the emergence of classical properties in quantum physics. The precise decoherence mechanisms, however, are often unknown for a given system. In this work, we make use of an opto-mechanical resonator to obtain key information about spectral densities of its condensed-matter heat bath. In sharp contrast to what is commonly assumed in high-temperature quantum Brownian motion describing the dynamics of the mechanical degree of freedom, based on a statistical analysis of the emitted light, it is shown that this spectral density is highly non-Ohmic, reflected by non-Markovian dynamics, which we quantify. We conclude by elaborating on further applications of opto-mechanical systems in open system identification.
We propose a representative, globally-admissible phenomenological spectral density of the bath for the non-Markovian Brownian motion of an optomechanical resonator, motivated by the near-resonance experimental observation of a non-Ohmic spectrum in [Nat. Commun. 6, 7606 (2015)]. To avoid divergences arising from a naive global extrapolation, we propose a globally-admissible, phenomenological bath spectrum that extends the experimentally-observed, near-resonance non-Ohmic behavior beyond the measurement window while ensuring finite bath-induced renormalizations and quadrature fluctuations of the resonator. The corresponding model of the structured environment produces a nonlocal mechanical response whose analytic pole structure encodes the observed linewidth. The resulting dissipation kernel exhibits a power-law-modulated exponential decay with transient negativity, signaling memory effects. In the weak-coupling regime, the optical readout based on homodyne detection enables near-resonance spectroscopy and, with a calibrated drive on the resonator, permits, in principle, the reconstruction of the full mechanical susceptibility, thereby providing access to both the dissipative and dispersive bath contributions. Our results provide a consistent route from locally-inferred spectral properties to globally-admissible open-system descriptions and establish a framework for probing structured environments in cavity optomechanics.
We consider a model of non-Markovian quantum Brownian motion that consists of a harmonic oscillator bilinearly coupled to a thermal bath, both via its position and via its momentum operators. We derive the master equation for such a model, and we solve the equations of motion for a generic Gaussian system state. We then investigate the resulting evolution of the first and second moments for both an Ohmic and a super-Ohmic spectral density. In particular, we show that, irrespective of the specific form of the spectral density, the coupling with the momentum enhances the dissipation experienced by the system, accelerating its relaxation to the equilibrium as well as modifying the asymptotic state of the dynamics. Eventually, we characterize explicitly the non-Markovianity of the evolution using a general criterion which relies on the positivity of the master equation coefficients.
The dissipative dynamics of a quantum Brownian particle is studied for different types of environment. We derive analytic results for the time evolution of the mean energy of the system for Ohmic, sub-Ohmic, and super-Ohmic environments, without performing the Markovian approximation. Our results allow one to establish a direct link between the form of the environmental spectrum and the thermalization dynamics. This in turn leads to a natural explanation of the microscopic physical processes ruling the system time evolution both in the short-time non-Markovian region and in the long-time Markovian one. Our comparative study of thermalization for different environments sheds light on the physical contexts in which non-Markovian dissipation effects are dominant.
Dissipation caused by nonhomogeneous bosonic finite chain environments (implementable in, e.g., segmented ion traps) is investigated through an exact diagonalization approach, avoiding common approximations used to describe open systems. Different spectral densities, including band gaps, can be engineered to separately assess different factors leading to memory effects, namely, the environment's size, temperature, proximity of the cutoff frequency, the spectral density's shape (sub-Ohmic, Ohmic, super-Ohmic), and the strength of its coupling to the system. Non-Markovianity is quantified with two recently introduced measures related to information backflow and nondivisibility of the system dynamical map. By sweeping the bath spectrum via tuning of the system frequency we show strongest memory effects at band-gap edges and provide an interpretation based on energy flow between system and environment. A system weakly coupled to a stiff chain ensures a Markovian dynamics, while the size of the environment as well as the local density of modes are not substantial factors. We show an opposite effect when increasing the temperature inside or outside the spectral band gap. Further, non-Markovianity arises for larger (negative and positive) powers of algebraic spectral densities, being the Ohmic case not always the most Markovian one.
We consider a well-known, exactly solvable model of an open quantum system with pure decoherence. The aim of this paper is twofold. Firstly, decoherence is a property of open quantum systems important for both quantum technologies and the fundamental question of the quantum–classical transition. It is worth studying how the long-term rate of decoherence depends on the spectral density characterising the system–bath interaction in this exactly solvable model. Secondly, we address a more general problem of the Markovian embedding of non-Markovian open system dynamics. It is often assumed that a non-Markovian open quantum system can be embedded into a larger Markovian system. However, we show that such embedding is possible only for Ohmic spectral densities (for the case of a positive bath temperature) and is impossible for both sub- and super-Ohmic spectral densities. On the other hand, for Ohmic spectral densities, an asymptotic large-time Markovianity (in terms of the quantum regression formula) takes place.
We generalize the classical theory of Brownian motion so as to reckon with non-Markovian effects on both Klein-Kramers and Smoluchowski equations. For a free particle and a harmonic oscillator, it is shown that such non-Markovian effects account for the differentiability of the Brownian trajectories as well as the breakdown of the energy equipartition of statistical mechanics at short times in some physical situations. This non-Markovian approach is also extended to look at anomalous diffusion. Next, we bring in the dynamical-quantization method for investigating open quantum systems, which does consist in quantizing the classical Brownian motion starting directly from our non-Markovian Klein-Kramers and Smoluchowski equations, without alluding to any model Hamiltonian. Accordingly, quantizing our non-Markovian Klein-Kramers in phase space gives rise to a non-Markovian quantum master equation in configuration space, whereas quantizing our non-Markovian Smoluchowski equation in configuration space leads to a non-Markovian quantum Smoluchowski equation in phase space. In addition, it is worth noticing that non-Markovian quantum Brownian motion takes place in presence of a generic environment (e.g. a non-thermal quantum fluid). As far as the special case of a heat bath comprising of quantum harmonic oscillators is concerned, a non-Markovian Caldeira-Leggett master equation and a thermal quantum Smoluchowski equation are derived and extended to bosonic and fermionic heat baths valid for all temperatures.