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arXiv:1311.2923 · Physical Review A

Spectral origin of non-Markovian open-system dynamics: A finite harmonic model without approximations

Ruggero Vasile, Fernando Galve, Roberta Zambrini

Published Feb 14, 2014• 51 citations
arXivHTMLPDF

Abstract

Dissipation caused by nonhomogeneous bosonic finite chain environments (implementable in, e.g., segmented ion traps) is investigated through an exact diagonalization approach, avoiding common approximations used to describe open systems. Different spectral densities, including band gaps, can be engineered to separately assess different factors leading to memory effects, namely, the environment's size, temperature, proximity of the cutoff frequency, the spectral density's shape (sub-Ohmic, Ohmic, super-Ohmic), and the strength of its coupling to the system. Non-Markovianity is quantified with two recently introduced measures related to information backflow and nondivisibility of the system dynamical map. By sweeping the bath spectrum via tuning of the system frequency we show strongest memory effects at band-gap edges and provide an interpretation based on energy flow between system and environment. A system weakly coupled to a stiff chain ensures a Markovian dynamics, while the size of the environment as well as the local density of modes are not substantial factors. We show an opposite effect when increasing the temperature inside or outside the spectral band gap. Further, non-Markovianity arises for larger (negative and positive) powers of algebraic spectral densities, being the Ohmic case not always the most Markovian one.

DOI
10.1103/physreva.89.022109

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Dissipation caused by nonhomogeneous bosonic finite chain environments (implementable in, e.g., segmented ion traps) is investigated through an exact diagonalization approach, avoiding common approximations used to describe open systems. Different spectral densities, including band gaps, can be engineered to separately assess different factors leading to memory effects, namely, the environment's size, temperature, proximity of the cutoff frequency, the spectral density's shape (sub-Ohmic, Ohmic, super-Ohmic), and the strength of its coupling to the system. Non-Markovianity is quantified with two recently introduced measures related to information backflow and nondivisibility of the system dynamical map. By sweeping the bath spectrum via tuning of the system frequency we show strongest memory effects at band-gap edges and provide an interpretation based on energy flow between system and environment. A system weakly coupled to a stiff chain ensures a Markovian dynamics, while the size of the environment as well as the local density of modes are not substantial factors. We show an opposite effect when increasing the temperature inside or outside the spectral band gap. Further, non-Markovianity arises for larger (negative and positive) powers of algebraic spectral densities, being the Ohmic case not always the most Markovian one.
For many open quantum systems, a master equation approach employing the Markov approximation cannot reliably describe the dynamical behaviour. This is the case, for example, in a number of solid state or biological systems, and it has motivated a line of research aimed at quantifying the amount of non-Markovian behaviour in a given model. Within this framework, we investigate the dynamics of a quantum harmonic oscillator linearly coupled to a bosonic bath. We focus on Gaussian states, which are suitably treated using a covariance matrix approach. Concentrating on an entanglement based non-Markovian behaviour quantifier (NMBQ) proposed by Rivas et. al. [1], we consider the role that near resonant and off-resonant modes play in affecting the NMBQ. By using a large but finite bath of oscillators for both Ohmic and super Ohmic spectral densities we find, by systematically increasing the coupling strength, initially the near resonant modes provide the most significant non-Markovian effects, while after a certain threshold of coupling strength the off-resonant modes play the dominant role. We also consider the NMBQ for two other models where we add a single strongly coupled oscillator to the model in extra bath mode and 'buffer' configurations, which affects the modes that determine non-Markovian behaviour.
We study quantum non-Markovian dynamics of the Caldeira-Leggett model, a prototypical model for quantum Brownian motion describing a harmonic oscillator linearly coupled to a reservoir of harmonic oscillators. Employing the exact analytical solution of this model one can determine the size of memory effects for arbitrary couplings, temperatures, and frequency cutoffs. Here, quantum non-Markovianity is defined in terms of the flow of information between the open system and its environment, which is quantified through the Bures metric as distance measure for quantum states. This approach allows us to discuss quantum memory effects in the whole range from weak to strong dissipation for arbitrary Gaussian initial states. A comparison of our results with the corresponding results for the spin-boson problem show a remarkable similarity in the structure of non-Markovian behavior of the two paradigmatic models.
In open quantum systems, the environment is typically modelled as a collection of harmonic oscillators, whereas realistic environments often exhibit unique non-Markovian effects due to the anharmonicity of the environment. Here we present a framework for modelling anharmonic environments in open quantum systems numerically exactly, in which, via a matching criterion, we map the anharmonic environment onto an effective harmonic one. This results in an effective spectral density that is a collection of shifted bare spectra arising from the non-equidistant energy gaps of the anharmonic environment, along with a unique zero-frequency term that effectively acts as static disorder on the system. This is due to the non-zero variance of the diagonal of the bath coupling operator. In tandem, we develop a framework for investigating the effects of environments comprising a few damped anharmonic modes where the matching criterion fails to work due to the non-Gaussianity of the environment. For both continuous and discrete damped anharmonic environments, this work investigates their unique influence on the system's dynamics, including enhanced non-Markovianity compared to a harmonic approximation, novel effects in the absorption spectrum, and the potential for anharmonic environments to enhance energy transport.
Non-Markovianity is the property that a physical system's future state depends on its previous dynamical history, namely the system has memory of its past. It is a key resource for quantum technologies but it is difficult to engineer without specific strategies. Here, we show that introducing a band gap in the environmental spectral density of both bosonic and fermionic baths provides a direct route to tuning non-Markovianity over a wide range. We demonstrate this effect by means of numerical simulations across bosonic and fermionic environments and discuss experimental tests of our predictions.
Non-Markovian effects in open quantum systems are central to understanding spectral lineshape. Here, we quantify the non-Markovianity associated with both overdamped and underdamped vibrations in terms of information flow between the bath and the system and compare this with the broadening and ellipticity of two-dimensional spectra. Using the Breuer Laine Piilo (BLP) measure, we link the well-known stochastic models for spectral lineshape with modern quantum information theory. Specifically, we study the effect of non-Markovianity in a system in contact with underdamped vibrations and examine the differences observed on increasing the damping to the overdamped limit. The open quantum system dynamics are evolved using the hierarchical equations of motion, efficiently terminated with a Markovian cutoff, where separate hierarchies are derived for the underdamped and overdamped environments. It is shown that the BLP measure is quantitatively correlated with the ellipticity of two-dimensional spectra and memory effects are more pronounced in underdamped environments, due to the long-lived feedback of information between the system and its bath, compared to overdamped environments. Environmental signatures in spectral lineshapes emerge as a result of information flow from the bath back into the system.
Understanding the non-Markovian dynamics of dissipative processes induced by memory effects of the environment is a fundamental subject of open quantum systems. Because of the complexity of open quantum systems, e.g., the multiple energy scales involving that of the system, the environment, and their mutual coupling, it is generally a challenging task to characterize the relationship among the parameters of the system dynamics and the reservoir spectra. For the two-level spontaneous emission model within structured environments, it was shown in a recent literature (Opt. Lett. 38, 3650) that a functional relation could be established between the asymptotically non-decaying population and the spectral density of the reservoir as the system undergoes a long-time evolution. It hence renders a distinct perspective to look into the character of long-lived quantum coherence in the corresponding non-Markovian process. This article is devoted to further investigate the phenomena of limit cycle oscillations possibly occurring in such non-Markovian dissipative systems in a long-time evolution. For a two-level system subjected to an environment with Ohmic class spectra, due to the presence of a unique bound-state mode of the system, the evolution trajectory of the given initial states will converge to a limit cycle in the Bloch space. The dependence of the radius and the location of the limit cycle on the spectral density function of the reservoir are manifested by virtue of the described functional relation. For the model subjected to a photonic crystal environment with multiple bands, our studies reveal that, owing to the presence of two or more bound states, the evolution trajectory of the system will converge to a toric curve of a paraboloid in the Bloch space and the phenomena of periodic or quasi-periodic oscillations could exhibit. While the equation of the parabolic curve is fully determined by the initial values of the state vector in the Bloch space, our results reveal that the scope of the evolution trajectory inside the toric curve is related to the spectral density of the reservoir and their quantified relation is distinctly characterized. Finally, the asymptotic dynamics of the correlations of a two-qubit system is discussed when it is subjected locally to the non-Markovian dissipative process.