In trapped-atom clocks, the primary source of decoherence is often the phase noise of the oscillator. For this case, we derive theoretical performance gains by combining several atomic ensembles. For example, M ensembles of N atoms can be combined with a variety of probe periods, to reduce the frequency variance to M 2^-M times that of standard Ramsey clocks. A similar exponential improvement is possible if the atomic phases of some of the ensembles evolve at reduced frequencies. These ensembles may be constructed from atoms or molecules with lower-frequency transitions, or generated by dynamical decoupling. The ensembles with reduced frequency or probe period are responsible only for counting the integer number of 2 pi phase wraps, and do not affect the clock's systematic errors. Quantum phase measurement with Gaussian initial states allows for smaller ensemble sizes than Ramsey spectroscopy.
In trapped-atom clocks, the primary source of decoherence is often the phase noise of the oscillator. For this case, we derive theoretical performance gains by combining several atomic ensembles. For example, M ensembles of N atoms can be combined with a variety of probe periods, to reduce the frequency variance to M 2^-M times that of standard Ramsey clocks. A similar exponential improvement is possible if the atomic phases of some of the ensembles evolve at reduced frequencies. These ensembles may be constructed from atoms or molecules with lower-frequency transitions, or generated by dynamical decoupling. The ensembles with reduced frequency or probe period are responsible only for counting the integer number of 2 pi phase wraps, and do not affect the clock's systematic errors. Quantum phase measurement with Gaussian initial states allows for smaller ensemble sizes than Ramsey spectroscopy.
The stability of several clock protocols based on 2 to 20 entangled atoms is evaluated numerically by a simulation that includes the effect of decoherence due to classical oscillator noise. In this context the squeezed states discussed by André, Sørensen and Lukin [PRL 92, 239801 (2004)] offer reduced instability compared to clocks based on Ramsey's protocol with unentangled atoms. When more than 15 atoms are simulated, the protocol of Bužek, Derka and Massar [PRL 82, 2207 (1999)] has lower instability. A large-scale numerical search for optimal clock protocols with two to eight qubits yields improved clock stability compared to Ramsey spectroscopy, and for two to three qubits performance matches the analytical protocols. In the simulations, a laser local oscillator decoheres due to flicker-frequency (1/f) noise. The oscillator frequency is repeatedly corrected, based on projective measurements of the qubits, which are assumed not to decohere with one another.
Improving the clock stability is of fundamental importance for the development of quantum-enhanced metrology. One of the main limitations arises from the randomly fluctuating local oscillator (LO) frequency, which introduces ``phase slips'' for long interrogation times and hence the failure of the frequency-feedback loop. Here we propose a strategy to improve the stability of atomic clocks by interrogating two atomic ensembles sharing the same LO. The two ensembles are prepared in coherent spin states pointing along orthogonal directions in the Bloch sphere. While standard Ramsey interrogation can only determine phases unambiguously in the interval $[\ensuremath{-}\ensuremath{\pi}/2,\ensuremath{\pi}/2]$, the joint interrogation allows for an extension to $[\ensuremath{-}\ensuremath{\pi},\ensuremath{\pi}]$, resulting in a relaxed restriction of the Ramsey time and improvement of absolute clock stability. Theoretical predictions are supported by ab initio numerical simulation for white and correlated LO noise. While our basic protocol uses uncorrelated atoms, we further extended it to include spin-squeezing and further improving the scaling of clock stability with the number of atoms. Our protocol can be readily tested in current state-of-the-art experiments.
This thesis describes new results on the entanglement of atomic spins in Ramsey interferometry, optical atomic clocks and trapped ions. It is divided into three parts: First, we investigate improvements to conventional Ramsey interferometry with entanglement and adding only rotations of the collective spin to adjust the signal and measurement directions. The geometric degrees of freedom, connected to the rotations, are analytically optimized for a large class of generalized Ramsey protocols to allow efficient optimization of all parameters. Besides a unification of existing approaches, the main result is that there is only one new protocol, where a previously unused double inversion is applied. Studies of the local sensitivity show that this protocol reaches the fundamental quantum Fisher information limit and is yet robust against errors during preparation and measurement. In the second section we investigate the conditions under which optical atomic clocks exhibit increased long-term stability when applying weakly entangled, spin squeezed states. We discuss the common case of an atomic clock with a single ensemble, typical Brownian frequency noise and finite dead time. Theoretical modelling of the servo loop allows quantitative predictions of the optimal stability for given values of dead time and laser noise, in very good agreement with numerical simulations of the closed feedback loop. The main result is that, even with the current most stable lasers, the clock stability can only be improved for ensembles below a critical atom number of about one thousand in optical Sr lattice clocks. Even with a future improvement of the laser performance by one order of magnitude, the critical atom number still remains below 100,000. In contrast, clocks based on smaller, non-scalable ensembles, such as ion clocks, can already benefit from squeezed states with current clock lasers. Thus the last section considers the robust generation of entanglement in ion traps. An error budget including relevant experimental error sources is calculated for state-of-the-art quantum gates, driven by oscillating microwave gradients in surface traps. Amplitude modulation of the driving fields is shown to efficiently counteract the current limitations from motional mode instability. The predicted increase of the gate quality was demonstrated by the group of C. Ospelkaus at PTB Braunschweig, who measured gates with errors as low as ~ 10^(-3). In a similar approach, interactions between spin and motion can also be generated by combining oscillating rf-fields with a static magnetic field gradient. Penning traps designed for precision spectroscopy already feature large magnetic field gradients at the edge of a magnetic bottle configuration. We present parameters and conditions under which laser-free coupling of spin and quantized motion for (anti-)protons is possible at these points, in a step towards quantum logic spectroscopy for (anti-)protons.
The stability of an optical atomic clock is a critical figure of merit for almost all clock applications. To this end, much optical atomic clock research has focused on reducing clock instability by increasing the atom number, lengthening the coherent interrogation times, and introducing entanglement to push beyond the standard quantum limit. In this work, we experimentally demonstrate an alternative approach to reducing clock instability using a phase estimation approach based on individually controlled atomic ensembles in a strontium (Sr) optical lattice clock. We first demonstrate joint Ramsey interrogation of two spatially resolved atom ensembles that are out of phase with respect to each other, which we call “quadrature Ramsey spectroscopy,” resulting in a factor of 1.36(5) reduction in absolute clock instability as measured with interleaved self-comparisons. We then leverage the rich hyperfine structure of Sr87 to realize independent coherent control over multiple ensembles with only global laser addressing. Finally, we utilize this independent control over four atom ensembles to implement a form of phase estimation, achieving a factor of greater than 3 enhancement in coherent interrogation time and a factor of 2.08(6) reduction in instability over an otherwise identical single-ensemble clock with the same local oscillator and the same number of atoms. We expect that multiensemble protocols similar to those demonstrated here will result in reduction in the instability of any optical lattice clock with an interrogation time limited by the local oscillator. Published by the American Physical Society 2024
Atomic clocks have reached the Quantum Projection Noise (QPN) limit of stability and it has been proposed to use the entangled atomic ensemble in order to overcome the QPN limit. We have proposed a new method to lock the phase of the Local Oscillator (LO) to the atomic phase and call, "atomic phase lock (APL)." This APL could possibly overcome the QPN limit without need of preparing the entangled atomic ensemble. Traditional Ramsey method destroys the coherence of the atomic spin due to the projection measurement at each cycle. This destruction and initialization of the phase at each cycle introduce additional noise and the performance of the atomic clock is limited at the white frequency noise level. APL employs dispersion measurements, i.e. Faraday rotation, in order to measure the phase difference without destroying the atomic phase. By repeating the measurement cycle with sufficiently small dead time, one can suppress the LO noise down to white phase noise level, achieving the τ-1 dependence of the Allan variance that can eventually overcome the QPN limit in long term. We are preparing a proof-of-principle experiment using the ensemble of trapped 171Yb+ ions with hyperfine splitting (12.6 GHz) as a clock transition and report the current status of the experiment as well.
We present a number of analytical means for the analysis of the evolution of an atom clock, emphasizing the role of many-body processes in the population and coherence loss. A master equation with one-body and two-body losses included is presented for a thermal cloud ensemble, suitable for modelling atom clock evolution. Approximate solutions for the coupled rate equations with one-body and two-body losses are obtained for the case of Ramsey free evolution, and their validity is analyzed. An approach is suggested to combine the analytical trap-induced fringe envelope function with a numerically evaluated many-body envelope function. A set of Ramsey and spin echo models is offered with analytical solutions for the off-resonant and on-resonant regimes with one-body population loss and phenomenological dephasing. Their detuning spectra are presented and the difference between them and the standard Ramsey model is shown: the Rabi pedestal in the present model has no spectral ripples due to the pi/2-pulse duration equal to a quarter of a Rabi oscillation, even off resonance, in contrast to the Ramsey method where the pi/2-pulse duration is not corrected off resonance and causes spectral ripples. the off-resonant and on-resonant regimes with one-body population loss and phenomenological dephasing. Their detuning spectra are presented and the difference between them and the standard Ramsey model is shown: the Rabi pedestal in the present model has no spectral ripples due to the pi/2-pulse duration equal to a quarter of a Rabi oscillation, even off resonance, in contrast to the Ramsey method where the pi/2-pulse duration is not corrected off resonance and causes spectral ripples. An interferometric fringe in long evolution experiments is typically measured with a visibility decay primarily due to phase diffusion, phase instability, trapping effects and many-body losses. It constitutes a problem to extract parameters from a fringe obtained in the time domain because of the growing uncertainty of the fringe amplitude and phase. This visibility loss can be compensated for systems with unequal state population losses, as the one we have, by tailoring the pulse durations. Methods are suggested for the one-body and many-body cases.A comprehensive set of experiments is conducted on the characterization of the stability of the trapped atom clock: with condensate and thermal cloud ensembles, with phase-domain Ramsey and spin echo interferometries, with synchronization from a rubidium frequency standard and from an oven-controlled quartz oscillator. The types of noise present in the system are identified by means of an Allan deviation analysis. Despite the 50 times different cloud densities of the condensate and the thermal clouds, an equality of the phase stability in the Ramsey interferometry with BEC and thermal clouds is demonstrated. The spin echo interferometry has shown a slightly superior stability with the thermal clouds as compared to the BEC.