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arXiv:1303.1453 · Superconductor Science and Technology

Rate of tunneling nonequilibrium quasiparticles in superconducting qubits

Mohammad H. Ansari

Published Feb 6, 2015• 11 citations
arXivHTMLPDF

Abstract

In superconducting qubits the lifetime of quantum states cannot be prolonged arbitrarily by decreasing temperature. At low temperature quasiparticles tunneling between electromagnetic environment and superconducting islands takes the condensate state out of equilibrium due to charge imbalance. We obtain the tunneling rate from a phenomenological model of non-equilibrium, where nonequilibrium quasiparticle tunnelling stimulates a temperature-dependent chemical potential shift in superconductor. As a result we obtain a non-monotonic behavior for relaxation rate as function of temperature. Depending on the fabrication parameters for some qubits the lowest tunneling rate of nonequilibrium quasiparticles can take place only near the onset temperature below which nonequilibrium quasiparticles dominate over equilibrium one. Our theory also indicates that such tunnelings can influence the probability of transitions in qubits through a coupling to the zero-point energy of phase fluctuations.

DOI
10.1088/0953-2048/28/4/045005

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In superconducting qubits the lifetime of quantum states cannot be prolonged arbitrarily by decreasing temperature. At low temperature quasiparticles tunneling between electromagnetic environment and superconducting islands takes the condensate state out of equilibrium due to charge imbalance. We obtain the tunneling rate from a phenomenological model of non-equilibrium, where nonequilibrium quasiparticle tunnelling stimulates a temperature-dependent chemical potential shift in superconductor. As a result we obtain a non-monotonic behavior for relaxation rate as function of temperature. Depending on the fabrication parameters for some qubits the lowest tunneling rate of nonequilibrium quasiparticles can take place only near the onset temperature below which nonequilibrium quasiparticles dominate over equilibrium one. Our theory also indicates that such tunnelings can influence the probability of transitions in qubits through a coupling to the zero-point energy of phase fluctuations.
We directly observe low-temperature nonequilibrium quasiparticle tunneling in charge qubits based on the single-Cooper-pair box. We measure even- and odd-state dwell-time distributions as a function of temperature, and interpret these results using a kinetic theory. While the even-state lifetime is exponentially distributed, the odd-state distribution is more heavily weighted to short times, implying that odd-to-even tunnel events are not described by a homogenous Poisson process. The mean odd-state dwell time increases sharply at low temperature, which is consistent with quasiparticles tunneling out of the island before reaching thermal equilibrium.
As low-loss nonlinear elements, Josephson junctions are the building blocks of superconducting qubits. The interaction of the qubit degree of freedom with the quasiparticles tunneling through the junction represents an intrinsic relaxation mechanism. We develop a general theory for the qubit decay rate induced by quasiparticles, and we study its dependence on the magnetic flux used to tune the qubit properties in devices such as the phase and flux qubits, the split transmon, and the fluxonium. Our estimates for the decay rate apply to both thermal equilibrium and nonequilibrium quasiparticles. We propose measuring the rate in a split transmon to obtain information on the possible nonequilibrium quasiparticle distribution. We also derive expressions for the shift in qubit frequency in the presence of quasiparticles.
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Abstract Non-equilibrium quasiparticles are possible sources for decoherence in superconducting qubits because they can lead to energy decay or dephasing upon tunneling across Josephson junctions (JJs). Here, we investigate the impact of the intrinsic properties of two-dimensional transmon qubits on quasiparticle tunneling (QPT) and discuss how we can use quasiparticle dynamics to gain critical information about the quality of JJ barrier. We find the tunneling rate of the non-equilibrium quasiparticles to be sensitive to the choice of the shunting capacitor material and their geometry in qubits. In some devices, we observe an anomalous temperature dependence of the QPT rate below 100 mK that deviates from a constant background associated with non-equilibrium quasiparticles. We speculate that this behavior is caused by high transmission sites/defects within the oxide barriers of the JJs, leading to spatially localized subgap states. We model this by assuming that such defects generate regions with a smaller effective gap. Our results present a unique in situ characterization tool to assess the uniformity of tunnel barriers in qubit junctions and shed light on how quasiparticles can interact with various elements of the qubit circuit.
Superconducting qubits are among the most promising elements for the implementation of the concept of quantum computing. Quasiparticles are an intrinsic sources of qubit decoherence, and are more generally detrimental to the operation of superconducting devices, e.g., Cooper pair pumps. Experiments reveal that quasiparticles fail to equilibrate and their density remains high even at low temperatures. Planting normal-metal traps on a superconducting device offers a way to reduce the quasiparticle density: once a quasiparticle tunnels into the normal metal and relaxes to subgap energy via inelastic processes, it cannot return to the superconductor. This paper presents a theoretical model for the time-resolved dynamics of quasiparticles injected into a qubit, and experiments with transmon qubits validating the model. The authors show that, contrary to expectations, the effective trapping rate depends on temperature, which is a consequence of the strong energy dependence of the quasiparticle density of states in the superconductor. At low temperatures, the relaxation process in the normal metal is the bottleneck limiting the effectiveness of traps. The authors also show that the trapping rate saturates for larger traps. At saturation, the rate is limited by the inverse of the time it takes for quasiparticles to diffuse across the device.
Bogoliubov quasiparticle excitations are detrimental for the operation of many superconducting devices. In superconducting qubits, quasiparticles interact with the qubit degree of freedom when tunneling through a Josephson junction, and this interaction can lead to qubit relaxation. At millikelvin temperatures, there is substantial evidence of nonequilibrium quasi- particles. While there is no agreed upon explanation for the origin of these excess quasiparticles, it is nevertheless possible to limit the quasiparticle-induced relaxation by steering quasiparticles away from qubit active elements. In this thesis, we study quasiparticle traps that are formed by a normal-metal in tunnel contact with the superconducting electrode of a qubit. We develop a model to explain how a trap can influence the dynamics of the excess quasiparticles injected in a transmontype qubit. This model makes it possible to find the time it takes to evacuate the injected quasiparticles from the transmon as a function of trap parameters. We show when the trap size is increased, the evacuation time decreases monotonically and saturates at a level that depends on the quasiparticles diffusion constant and the qubit geometry. We find the characteristic trap size needed for the evacuation time to approach the saturation value. It turns out that the bottleneck limiting the trapping rate is the slow quasiparticle energy relaxation inside the normal-metal trap, a quantity that is very hard to control. In order to optimize normal-metal quasiparticle trapping, we study the effects of trap size, number, and placement. These factors become important when the trap size increases beyond the characteristic length. We discuss for some experimentally relevant examples how to shorten the evacuation time of the excess quasiparticle density. Moreover, we show that a trap in the vicinity of a Josephson junction can significantly suppress the steady-state quasiparticle density near that junction and reduce the impact of fluctuations in the generation rate of quasiparticles. When such normal-metal elements are connected to a superconducting material, Cooper- pairs can leak into the normal-metal trap. This modifies the superconductor properties and, in turn, affects the qubit coherence. Using the Usadel formalism, we first revisit the proximity effect in uniform NS bilayers; despite the long history of this problem, we present novel findings for the density of states. We then extend our results to describe a non-uniform system in the vicinity of a trap edge. Using these results together with the previously developed model for the suppression of the quasiparticle density due to the trap, we find in a transmon qubit an optimum trap-junction distance at which the qubit relaxation rate is minimized. This optimum distance, of the order of 4 to 20 coherence lengths, originates from the competition between proximity effect and quasiparticle density suppression. We conclude that the harmful influence of the proximity effect can be avoided so long as the trap is farther away from the junction than this optimum.