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arXiv:1301.3960 · Physical Review A

System-environment coupling derived by Maxwell's boundary conditions from the weak to the ultrastrong light-matter-coupling regime

Motoaki Bamba, Tetsuo Ogawa

Published Jul 9, 2013• 27 citations
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Abstract

In the standard theory of cavity quantum electrodynamics (QED), coupling between photons inside and outside a cavity (cavity system and environment) is given conserving the total number of photons. However, when the cavity photons (ultrastrongly) interact with atoms or excitations in matters, the system-environment coupling must be determined from a more fundamental viewpoint. Based on the Maxwell's boundary conditions in the QED theory for dielectric media, we derive the quantum Langevin equation and input-output relation, in which the total number of polaritons (not photons) inside the cavity and photons outside is conserved.

DOI
10.1103/physreva.88.013814

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Comment on “System-environment coupling derived by Maxwell's boundary conditions from the weak to the ultrastrong light-matter-coupling regime”

Simone De Liberato

In a recent paper, Bamba and Ogawa [Phys. Rev. A 88, 013814 (2013)] developed a microscopic model describing a photonic cavity coupled to an excitonlike resonance. One of the results they obtained studying such a model is that, in the ultrastrong coupling regime, dissipation rates calculated applying the rotating-wave approximation on the system-environment coupling qualitatively differ from the ones calculated using a microscopic theory based on the quantum electrodynamics for dielectric media. Here I show that this result is an artifact, caused by an inconsistent application of the rotating-wave approximation and by an unphysical parameter choice.

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•Jun 10, 2013•0 citations
In the standard theory of cavity quantum electrodynamics (QED), coupling between photons inside and outside a cavity (cavity system and environment) is given conserving the total number of photons. However, when the cavity photons (ultrastrongly) interact with atoms or excitations in matters, the system-environment coupling must be determined from a more fundamental viewpoint. Based on the Maxwell's boundary conditions in the QED theory for dielectric media, we derive the quantum Langevin equation and input-output relation, in which the total number of polaritons (not photons) inside the cavity and photons outside is conserved.
We give a rigorous quantum-field theoretical derivation of the Langevin-equations approach to the problem of determining the radiation field inside and outside a resonator-like cavity by starting from Maxwell's equations with field- matter interaction and taking into account the presence of a cavity with a finite Q value by modeling its input/output port by a dielectric (multislab) wall.1,2 We show that if the transparency of the wall is small compared with unity, in the coarse-grain approximation the field generated and/or amplified by the active medium inside the cavity may be described by quantum Langevin equations. The coarse-grain time is determined by the time of flight of a light signal through the cavity.
In a recent paper, Bamba and Ogawa [Phys. Rev. A 88, 013814 (2013)] developed a microscopic model describing a photonic cavity coupled to an excitonlike resonance. One of the results they obtained studying such a model is that, in the ultrastrong coupling regime, dissipation rates calculated applying the rotating-wave approximation on the system-environment coupling qualitatively differ from the ones calculated using a microscopic theory based on the quantum electrodynamics for dielectric media. Here I show that this result is an artifact, caused by an inconsistent application of the rotating-wave approximation and by an unphysical parameter choice.
When the light interacts with matters in a lossy cavity, in the standard cavity quantum electrodynamics, the dissipation of cavity fields is characterized simply by the strengths of the two couplings: the light-matter interaction and the system-environment coupling through the cavity mirror. However, in the ultrastrong-light-matter-interaction regime, the dissipation depends also on whether the two couplings are mediated by the electric field or the magnetic one (capacitive or inductive in superconducting circuits). Even if we know correctly the microscopic mechanism (Lagrangian) of the system-environment coupling, the coupling Hamiltonian itself is in principle modified due to the ultrastrong interaction in the cavity. In this paper, we show a recipe for deriving a general expression of the Hamiltonian of the system-environment coupling, which is applicable even in the ultrastrong-light-matter-interaction regime in the good-cavity and independent-transition limits.
We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultrastrong light-matter coupling regime, in which the vacuum Rabi frequency is a significant fraction of the active electronic transition frequency and the antiresonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. In the case of a time-independent vacuum Rabi frequency, exact analytical expressions for the operators are obtained, which allows us to characterize the quantum dissipative response of the cavity to an arbitrary initial condition (vacuum, coherent field, thermal excitation). For a vacuum input in both the photonic and electronic polarization modes, the ground state of the cavity system is a two-mode squeezed vacuum state with a finite population in both photonic and electronic modes. These excitations are, however, virtual and cannot escape from the cavity: for a vacuum input, a vacuum output is found, without any trace of the intracavity squeezing. For a coherent photonic input the linear optical response spectra (reflectivity, absorption, transmission) have been studied, and signatures of the ultrastrong coupling have been identified in the asymmetric and peculiar anticrossing of the polaritonic eigenmodes. Finally, we have calculated the electroluminescence spectra in the case of an incoherent electronic input: the emission intensity in the ultrastrong coupling regime results in being significantly enhanced as compared to the case of an isolated quantum well without a surrounding cavity.
We have investigated theoretically a dissipative polariton system in the ultrastrong light-matter coupling regime without using the rotating-wave approximation on system-reservoir coupling. Photons in a cavity and excitations in matter respectively couple two large ensembles of harmonic oscillators (photonic and excitonic reservoirs). Inheriting the quantum statistics of polaritons in the ultrastrong coupling regime, in the ground state of the whole system, the two reservoirs are not in the vacuum states but they are squeezed and correlated. We presume the reservoirs to be in this nonvacuum state in the master equation and in the input-output formalism with Langevin equations. Both approaches consistently guarantee the decay of the polariton system to its ground state; no photon detection is also obtained when the polariton system is in the ground state.
When the light interacts with matters in a lossy cavity, in the standard cavity quantum electrodynamics, the dissipation of cavity fields is characterized simply by the strengths of the two couplings: the light-matter interaction and the system-environment coupling through the cavity mirror. However, in the ultrastrong light-matter interaction regime, the dissipation depends also on whether the two couplings are mediated by the electric field or the magnetic one (capacitive or inductive in superconducting circuits). Even if we know correctly the microscopic mechanism (Lagrangian) of the system-environment coupling, the coupling Hamiltonian itself is in principle modified due to the ultrastrong interaction in the cavity. In this paper, we show a recipe for deriving a general expression of the Hamiltonian of the system-environment coupling, which is applicable even in the ultrastrong light-matter interaction regime in the good-cavity and independent-transition limit.