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arXiv:1301.0808 · Physical Review B

Magnetometry with nitrogen-vacancy ensembles in diamond based on infrared absorption in a doubly resonant optical cavity

Yannick Dumeige, Mayeul Chipaux, V. Jacques, François Treussart, Jean-François Roch, Thierry Debuisschert, Víctor M. Acosta, Andrey Jarmola, Kasper Jensen, Pauli Kehayias, Dmitry Budker

Published Apr 8, 2013• 77 citations
arXivHTMLPDF

Abstract

We propose using an optical cavity to enhance the sensitivity of a magnetometer relying on the detection of the spin state of a high-density nitrogen-vacancy ensemble in diamond using infrared optical absorption. The role of the cavity is to obtain a contrast in the absorption-detected magnetic resonance approaching unity at room temperature. We project an increase in the photon shot-noise limited sensitivity of two orders of magnitude in comparison with a single-pass approach. Optical losses can limit the enhancement to one order of magnitude, which could still enable room-temperature operation. Finally, the optical cavity also allows us to use less pumping power when the cavity is resonant at both the pump and the infrared probe wavelength.

DOI
10.1103/physrevb.87.155202

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We propose using an optical cavity to enhance the sensitivity of a magnetometer relying on the detection of the spin state of a high-density nitrogen-vacancy ensemble in diamond using infrared optical absorption. The role of the cavity is to obtain a contrast in the absorption-detected magnetic resonance approaching unity at room temperature. We project an increase in the photon shot-noise limited sensitivity of two orders of magnitude in comparison with a single-pass approach. Optical losses can limit the enhancement to one order of magnitude, which could still enable room-temperature operation. Finally, the optical cavity also allows us to use less pumping power when the cavity is resonant at both the pump and the infrared probe wavelength.
We demonstrate a cavity-enhanced room-temperature magnetic field sensor based on nitrogen-vacancy centers in diamond. Magnetic resonance is detected using absorption of light resonant with the 1042 nm spin-singlet transition. The diamond is placed in an external optical cavity to enhance the absorption, and significant absorption is observed even at room temperature. We demonstrate a magnetic field sensitivity of 2.5  nT/Hz2.5\text{ }\text{ }\mathrm{nT}/\sqrt{\mathrm{Hz}}2.5  nT/Hz​, and project a photon shot-noise-limited sensitivity of 70  pT/Hz70\text{ }\text{ }\mathrm{pT}/\sqrt{\mathrm{Hz}}70  pT/Hz​ for a few mW of infrared light, and a quantum projection-noise-limited sensitivity of 250  fT/Hz250\text{ }\text{ }\mathrm{fT}/\sqrt{\mathrm{Hz}}250  fT/Hz​ for the sensing volume of $\ensuremath{\sim}90\text{ }\text{ }\mathrm{\ensuremath{\mu}}\mathrm{m}\ifmmode\times\else\texttimes\fi{}90\text{ }\text{ }\mathrm{\ensuremath{\mu}}\mathrm{m}\ifmmode\times\else\texttimes\fi{}200\text{ }\text{ }\mathrm{\ensuremath{\mu}}\mathrm{m}$.
Magnetometry with nitrogen-vacancy (NV) centers in diamond has so far been measured via emission of light from NV centers or via absorption at the singlet transition at 1042 nm. Here, we demonstrate a phenomenon of broadband optical absorption by the NV centers starting in the emission wavelength and reaching up to 1000 nm. The measurements are enabled by a high-finesse cavity, which is used for room-temperature continuous wave pump-probe experiments. The red to infrared probe beam shows the typical optically detected magnetic resonance (ODMR) signal of the NV spin with contrasts up to 42 %. This broadband optical absorption has not yet been reported in terms of NV magnetometry. We argue that the lower level of the absorbing transition could be the energetically lower NV singlet state, based on the increased optical absorption for a resonant microwave field and the spectral behavior. Investigations of the photon-shot-noise-limited sensitivity show improvements with increasing probe wavelength, reaching an optimum of 7.5pT/Hz. The results show significantly improved ODMR contrast compared to emission-based magnetometry. This opens a new detection wavelength regime with coherent laser signal detection for high-sensitivity NV magnetometry.
We demonstrate magnetic-field sensing using an ensemble of nitrogen-vacancy centers by recording the variation in the pump-light absorption due to the spin-polarization dependence of the total ground-state population. Using a 532 nm pump laser, we measure the absorption of native nitrogen-vacancy centers in a chemical-vapor-deposited diamond placed in a resonant optical cavity. For a laser pump power of 0.4 W and a cavity finesse of 45, we obtain a noise floor of $\ensuremath{\sim}100 \mathrm{nT}/\sqrt{\mathrm{Hz}}$ spanning a bandwidth up to 125 Hz. We project a photon shot-noise-limited sensitivity of $\ensuremath{\sim}1 \mathrm{pT}/\sqrt{\mathrm{Hz}}$ by optimizing the nitrogen-vacancy concentration and the detection method.
The negatively charged nitrogen vacancy center in diamond is widely used for quantum sensing due to the sensitivity of the spin triplet in the electronic ground state to external perturbations such as strain and electromagnetic fields, which makes it an excellent probe for changes in these perturbations. The spin state can be measured through optically detected magnetic resonance, which is most commonly achieved by detecting the photoluminescence after exciting the spin-triplet transition. Recently, methods have been proposed and demonstrated that use the absorption of the infrared singlet transition at 1042 nm instead. These methods, however, require cryogenic temperatures or external cavities to enhance the absorption signal. Here, we report on our efforts to optimize the magnetometer sensitivity at room temperature and without cavities. We reach a sensitivity of 18 pT / Hz , surpassing previously reported values, and a calculated shot-noise limit of 5 pT / Hz . We also report on a defect that is native to diamond grown by chemical vapor deposition and thus absent in high-pressure high-temperature diamond, the excitation of which impacts the measured singlet absorption signal.
The negatively charged nitrogen vacancy center in diamond is widely used for quantum sensing due to the sensitivity of the spin triplet in the electronic ground state to external perturbations such as strain and electromagnetic fields, which makes it an excellent probe for changes in these perturbations.The spin state can be measured through optically detected magnetic resonance, which is most commonly achieved by detecting the photoluminescence after exciting the spin-triplet transition.Recently, methods have been proposed and demonstrated that use the absorption of the infrared singlet transition at 1042 nm instead.These methods, however, require cryogenic temperatures or external cavities to enhance the absorption signal.Here, we report on our efforts to optimize the magnetometer sensitivity at room temperature and without cavities.We reach a sensitivity of 18 pT/ √ Hz, surpassing previously reported values, and a calculated shot-noise limit of 5 pT/ √ Hz .We also report on a defect that is native to diamond grown by chemical vapor deposition and thus absent in high-pressure high-temperature diamond, the excitation of which impacts the measured singlet absorption signal.
Nitrogen-vacancy (NV) centers have considerable promise as high sensitivity magnetometers; however, they are commonly limited by inefficient collection and low contrasts. Laser threshold magnetometry (LTM) enables efficient collection and high contrasts, providing a path toward higher sensitivity magnetometry. We demonstrate an infrared LTM using an ensemble of NV centers in a single-crystal diamond plate integrated into a vertical external cavity surface emitting laser. The laser was tuned to the spin-dependent absorption line of the NV centers, allowing for optical readout by monitoring the laser output power. We demonstrate a magnetic sensitivity of 7.5 nT/Hz in the frequency range between 10 and 50 Hz. Furthermore, the contrast and the projected photon shot noise limited (PSNL) sensitivity are shown to improve significantly by operating close to the lasing threshold, achieving 18.4% and 26.6 pT/Hz near the threshold. In addition, an unexpected saturable absorption phenomenon was observed near the threshold, which enhanced the contrast and projected PSNL sensitivity.