Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1210.7419 · New Journal of Physics

Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics

K H Madsen, P Lodahl

Published Feb 7, 2013• 21 citations
arXivHTMLPDF

Abstract

We present detuning-dependent spectral and decay-rate measurements to study the difference between the spectral and dynamical properties of single quantum dots embedded in micropillar and photonic crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes–Cummings model, whereas systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to the coupling of other exciton lines to the cavity and interference of different propagation paths toward the detector of the fields emitted by the quantum dot. In contrast, quantitative information about the system can readily be extracted from the dynamical measurements. In the case of photonic crystal cavities, we observe an anti-crossing in the spectra when detuning a single quantum dot through resonance, which is the spectral signature of a strong coupling. However, time-resolved measurements reveal that the actual coupling strength is significantly smaller than anticipated from the spectral measurements and that the quantum dot is rather weakly coupled to the cavity. We suggest that the observed Rabi splitting is due to cavity feeding by other quantum dots and/or multi-exciton complexes giving rise to collective emission effects.

DOI
10.1088/1367-2630/15/2/025013

Related papers

Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics:Paper

Madsen, Kristian Høeg, Peter Lodahl

We present detuning-dependent spectral and decay-rate measurements to study the difference between the spectral and dynamical properties of single quantum dots embedded in micropillar and photonic crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes–Cummings model, whereas systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to the coupling of other exciton lines to the cavity and interference of different propagation paths toward the detector of the fields emitted by the quantum dot. In contrast, quantitative information about the system can readily be extracted from the dynamical measurements. In the case of photonic crystal cavities, we observe an anti-crossing in the spectra when detuning a single quantum dot through resonance, which is the spectral signature of a strong coupling. However, time-resolved measurements reveal that the actual coupling strength is significantly smaller than anticipated from the spectral measurements and that the quantum dot is rather weakly coupled to the cavity. We suggest that the observed Rabi splitting is due to cavity feeding by other quantum dots and/or multi-exciton complexes giving rise to collective emission effects.

•Jan 1, 2013•23 citations

Observation of Non-Markovian Dynamics of a Single Quantum Dot in a Micropillar Cavity

Kristian Høeg Madsen, Serkan Ateş, Toke Lund-Hansen +4 more

We measure the detuning-dependent dynamics of a quasiresonantly excited single quantum dot coupled to a micropillar cavity. The system is modeled with the dissipative Jaynes-Cummings model where all experimental parameters are determined by explicit measurements. We observe non-Markovian dynamics when the quantum dot is tuned into resonance with the cavity leading to a nonexponential decay in time. Excellent agreement between experiment and theory is observed with no free parameters providing the first quantitative description of an all-solid-state cavity QED system based on quantum dot emitters.

arXiv:1012.0740•Physical Review Letters•Jun 6, 2011•147 citations

The role of optical excitation power on the emission spectra of a strongly coupled quantum dot-micropillar system

S. Münch, Stephan Reitzenstein, P. Franeck +5 more

A strongly coupled quantum dot-micropillar cavity system is studied under variation of the excitation power. The characteristic double peak spectral shape of the emission with a vacuum Rabi splitting of 85 microeV at low excitation transforms gradually into a single broad emission peak when the excitation power is increased. Modelling the experimental data by a recently published formalism [Laussy et al., Phys. Rev. Lett. 101, 083601 (2008)] yields a transition from strong coupling towards weak coupling which is mainly attributed to an excitation power driven decrease of the exciton-photon coupling constant.

Optics Express•Jul 13, 2009•54 citations

Emission characteristics of a highly correlated system of a quantum dot coupled to two distinct micropillar cavity modes

Stefanie Weiler, Ata Ulhaq, Sven M. Ulrich +4 more

The emission characteristics of a system of one quantum dot (QD) nonresonantly coupled to two distinct detuned modes of a surrounding microcavity have been investigated, revealing strong interconnection in terms of photon anti-correlation in QD-mode and mode-mode cross correlations. Temperature-dependent lifetime measurements demonstrate that the QD emission dynamics is transferred to the mode channels through the process of nonresonant coupling, whereas the short coherence time of mode emission stays unperturbed by the QD-mode detuning. Power-dependent studies under pure-resonant QD excitation have traced the strong emitter-mode coupling to both an excited and the fundamental micropillar mode with spectral detunings of up to 3.7 meV.

Physical Review B•Nov 19, 2010•6 citations

Cavity quantum electrodynamics

Prasanta Kumar Basu, Bratati Mukhopadhyay, Rikmantra Basu

Abstract Inhibition and enhancement of spontaneous emission rate, first proposed by Purcell, is discussed in terms of altered density-of-modes in various types of solid-state cavities and the Purcell factor is derived for two-level atomic system. The conditions for observing Purcell factor and experimental findings in micropillars embedded with Quantum Dots (QD)s are discussed. The strong interaction between photons and matter in the form of QD excitons, dispersion relations for ground and excited states separated by Rabi splitting are discussed. Experimental photoluminescence spectra showing anticrossing of exciton lines and cavity lines by temperature and other tuning methods are used to illustrate the strong light-matter interaction. The Jayness–Cummins model based on second quantization is presented to point out Rabi oscillation, Purcell effect, and other novel features. Microcavity structures for observing cavity quantum electrodynamics effects are mentioned. Microcavity lasers predicting thresholdless operation for unity spontaneous emission coupling factors are discussed.

•Apr 5, 2022•0 citations

Interference effects in the emission spectra of quantum dots in high-quality cavities

Leonid V. Keldysh, V. D. Kulakovskiĭ, Stephan Reitzenstein +2 more

We have investigated theoretically and experimentally the emission of (quantum dot-cavity) systems for different coupling strength and a wide range of exciton-photon mode detunings controlled by temperature variation in the range 10–45 K. Under close to resonance conditions, the radiation spectrum from the cavity emission becomes essentially dependent on the primary excitation path, which can be either via resonant quantum-dot exciton or via cavity mode. Particularly, in the case of nonresonant cavity mode excitation, the emission line becomes split into two asymmetric lines already in the weak coupling regime.

Journal of Experimental and Theoretical Physics Letters•Jan 1, 2007•10 citations
We present detuning-dependent spectral and decay-rate measurements to study the difference between the spectral and dynamical properties of single quantum dots embedded in micropillar and photonic crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes–Cummings model, whereas systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to the coupling of other exciton lines to the cavity and interference of different propagation paths toward the detector of the fields emitted by the quantum dot. In contrast, quantitative information about the system can readily be extracted from the dynamical measurements. In the case of photonic crystal cavities, we observe an anti-crossing in the spectra when detuning a single quantum dot through resonance, which is the spectral signature of a strong coupling. However, time-resolved measurements reveal that the actual coupling strength is significantly smaller than anticipated from the spectral measurements and that the quantum dot is rather weakly coupled to the cavity. We suggest that the observed Rabi splitting is due to cavity feeding by other quantum dots and/or multi-exciton complexes giving rise to collective emission effects.
We present detuning-dependent spectral and decay-rate measurements to study the difference between the spectral and dynamical properties of single quantum dots embedded in micropillar and photonic crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes–Cummings model, whereas systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to the coupling of other exciton lines to the cavity and interference of different propagation paths toward the detector of the fields emitted by the quantum dot. In contrast, quantitative information about the system can readily be extracted from the dynamical measurements. In the case of photonic crystal cavities, we observe an anti-crossing in the spectra when detuning a single quantum dot through resonance, which is the spectral signature of a strong coupling. However, time-resolved measurements reveal that the actual coupling strength is significantly smaller than anticipated from the spectral measurements and that the quantum dot is rather weakly coupled to the cavity. We suggest that the observed Rabi splitting is due to cavity feeding by other quantum dots and/or multi-exciton complexes giving rise to collective emission effects.
We measure the detuning-dependent dynamics of a quasiresonantly excited single quantum dot coupled to a micropillar cavity. The system is modeled with the dissipative Jaynes-Cummings model where all experimental parameters are determined by explicit measurements. We observe non-Markovian dynamics when the quantum dot is tuned into resonance with the cavity leading to a nonexponential decay in time. Excellent agreement between experiment and theory is observed with no free parameters providing the first quantitative description of an all-solid-state cavity QED system based on quantum dot emitters.
A strongly coupled quantum dot-micropillar cavity system is studied under variation of the excitation power. The characteristic double peak spectral shape of the emission with a vacuum Rabi splitting of 85 microeV at low excitation transforms gradually into a single broad emission peak when the excitation power is increased. Modelling the experimental data by a recently published formalism [Laussy et al., Phys. Rev. Lett. 101, 083601 (2008)] yields a transition from strong coupling towards weak coupling which is mainly attributed to an excitation power driven decrease of the exciton-photon coupling constant.
The emission characteristics of a system of one quantum dot (QD) nonresonantly coupled to two distinct detuned modes of a surrounding microcavity have been investigated, revealing strong interconnection in terms of photon anti-correlation in QD-mode and mode-mode cross correlations. Temperature-dependent lifetime measurements demonstrate that the QD emission dynamics is transferred to the mode channels through the process of nonresonant coupling, whereas the short coherence time of mode emission stays unperturbed by the QD-mode detuning. Power-dependent studies under pure-resonant QD excitation have traced the strong emitter-mode coupling to both an excited and the fundamental micropillar mode with spectral detunings of up to 3.7 meV.
Abstract Inhibition and enhancement of spontaneous emission rate, first proposed by Purcell, is discussed in terms of altered density-of-modes in various types of solid-state cavities and the Purcell factor is derived for two-level atomic system. The conditions for observing Purcell factor and experimental findings in micropillars embedded with Quantum Dots (QD)s are discussed. The strong interaction between photons and matter in the form of QD excitons, dispersion relations for ground and excited states separated by Rabi splitting are discussed. Experimental photoluminescence spectra showing anticrossing of exciton lines and cavity lines by temperature and other tuning methods are used to illustrate the strong light-matter interaction. The Jayness–Cummins model based on second quantization is presented to point out Rabi oscillation, Purcell effect, and other novel features. Microcavity structures for observing cavity quantum electrodynamics effects are mentioned. Microcavity lasers predicting thresholdless operation for unity spontaneous emission coupling factors are discussed.
We have investigated theoretically and experimentally the emission of (quantum dot-cavity) systems for different coupling strength and a wide range of exciton-photon mode detunings controlled by temperature variation in the range 10–45 K. Under close to resonance conditions, the radiation spectrum from the cavity emission becomes essentially dependent on the primary excitation path, which can be either via resonant quantum-dot exciton or via cavity mode. Particularly, in the case of nonresonant cavity mode excitation, the emission line becomes split into two asymmetric lines already in the weak coupling regime.