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arXiv:1209.6550 · Physical Review Letters

Electrical Readout for Coherent Phenomena Involving Rydberg Atoms in Thermal Vapor Cells

Daniel Barredo, Harald Kübler, Renate Daschner, R. Löw, Tilman Pfau

Published Mar 21, 2013• 54 citations
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Abstract

We present a very sensitive and scalable method to measure the population of highly excited Rydberg states in a thermal vapor cell of rubidium atoms. We detect the Rydberg ionization current in a 5 mm electrically contacted cell. The measured current is found to be in qualitatively good agreement with a theory for the Rydberg population based on a master equation for the three-level problem, including an ionization channel and the full Doppler distributions at the corresponding temperatures. The signal-to-noise ratio of the current detection is substantially better than that of purely optical techniques.

DOI
10.1103/physrevlett.110.123002

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We present a very sensitive and scalable method to measure the population of highly excited Rydberg states in a thermal vapor cell of rubidium atoms. We detect the Rydberg ionization current in a 5 mm electrically contacted cell. The measured current is found to be in qualitatively good agreement with a theory for the Rydberg population based on a master equation for the three-level problem, including an ionization channel and the full Doppler distributions at the corresponding temperatures. The signal-to-noise ratio of the current detection is substantially better than that of purely optical techniques.
We present experimental results on nondegenerate four-wave mixing in a thermal vapor cell of rubidium atoms via highly excited Rydberg states. We observe sub-Doppler spectral features and a large sensitivity of the mixed light mode to small electric fields due to the large polarizabilities of the involved Rydberg state. We observe a saturation of the optical response due to the nonlinear four-level physics. The strong interaction between Rydberg atoms and the associated Rydberg blockade could potentially increase the nonlinearity dramatically.
We investigate a technique for detecting radio frequency (RF) electric fields in a cesium (Cs) vapor cell at room temperature by collecting charges from ionized Rydberg atoms and compare its performance with the established method of electromagnetically induced transparency (EIT). By applying a known RF field, we measure the response from both the electrical (ionization current-based) and optical (EIT-based) readouts. The ionization current-based method yields a sensitivity of 22 μ V m−1 Hz−1/2, while the EIT-based method achieves 3.7 μ V m−1 Hz−1/2. The sensitivity of the ionization current-based method is limited by the 2.2 k Ω resistance between the collection electrodes, attributed to a thin Cs film on the inner surfaces of the vapor cell. Controlling or eliminating the Cs layer can significantly improve the sensitivity of this ionization approach.
Rydberg atoms have large transition electric dipole moments and high sensitivity to electric fields. We describe a new method for microwave field sensing in a vapor cell consisting of separate excitation, quantum evolution between two Rydberg levels in the dark and state-dependent detection with probe laser transmission. Using microwave pulse techniques we study homogeneous and inhomogeneous relaxation of the coherence between Rydberg levels and demonstrate detection of a 10 GHz signal with electric field sensitivity of 10 nV/cm/Hz1/2^{1/2}1/2.
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With the rapid advancement of terahertz (THz) technology, there is an urgent demand for highly sensitive, broadband THz detectors that can operate at room temperature to support the evolving applications. Due to the high sensitivity of Rydberg atoms to external electric fields, detectors based on Rydberg quantum coherence offer great potential for highperformance THz detection. This paper proposed a ambient temperature electrometry approach for THz detection using probe laser spectroscopy of Rb Rydberg atoms and carry out a comprehensive study of a four-level system involving electromagnetically induced transparency (EIT) and Autler-Townes (AT) splitting in Rb cascades. By solving the Lindblad master equation, the influences of the THz electric field, probe laser, and coupling laser on the populations of the ground and Rydberg states were analyzed. Furthermore, the effects of temperature and vapor cell dimensions on the Rb atomic density are examined, revealing their critical impact on detection sensitivity. The results predict that the proposed quantum coherence based THz detection method can achieve a sensitivity as low as 10−9^{-9}−9V/m/Hz1/2^{1/2}1/2at ambient temperature. This paper provides a solid theoretical foundation for the implementation and optimization of Rydbergatom- based quantum coherence techniques for high-sensitivity, ambient temperature THz wave detection.