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arXiv:1207.6748 · Reviews of Modern Physics

Colloquium: Coherent diffusion of polaritons in atomic media

Ofer Firstenberg, M. Shuker, A. Ron, Nir Davidson

Published Jul 8, 2013• 45 citations
arXivHTMLPDF

Abstract

Coherent diffusion pertains to the motion of atomic dipoles experiencing frequent collisions in vapor while maintaining their coherence. Recent theoretical and experimental studies on the effect of coherent diffusion on key Raman processes, namely, Raman spectroscopy, slow polariton propagation, and stored light, are reviewed in this Colloquium.

DOI
10.1103/revmodphys.85.941

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Coherent diffusion pertains to the motion of atomic dipoles experiencing frequent collisions in vapor while maintaining their coherence. Recent theoretical and experimental studies on the effect of coherent diffusion on key Raman processes, namely, Raman spectroscopy, slow polariton propagation, and stored light, are reviewed in this Colloquium.
Coherent interactions of laser light with atomic ensembles allow one to modify dispersive properties of a medium and lead to new optical phenomena. Studies of the controlled light propagation and storing in such media have recently become a dynamically developing field of research motivated both by the fundamental character of the processes and by potential applications. This article briefly reviews basic theoretical approach to the dynamics of the propagation of laser pulses in optically modified media. The method and the physical processes are discussed that allow one to slow down the group velocity of laser pulse to zero (stopping of light), to transfer the state of a light pulse to atomic coherences and to restore the pulse. The interpretation of these phenomena in the formalism of dark-state polaritons is presented. Examples of possible coherent manipulations on a stored light are also discussed.
A combined experimental and theoretical investigation of time- and alignment-dependent propagation of light in an ultracold atomic gas of atomic 85Rb^{85}\mathrm{Rb}85Rb is reported. Coherences among the scattering amplitudes for light scattering off excited hyperfine levels produce strong variations of the light polarization in the vicinity of atomic resonance. Measurements are in excellent agreement with Monte Carlo simulations of the multiple scattering process.
Modern optical techniques allow one to accurately control light using atoms and to manipulate atoms using light. In this Colloquium the author reviews several ideas indicating how such techniques can be used for accurate manipulation of quantum states of atomic ensembles and photons. First a technique is discussed that allows one to transfer quantum states between light fields and metastable states of matter. The technique is based on trapping quantum states of photons in coherently driven atomic media, in which the group velocity is adiabatically reduced to zero. Next, possible mechanisms are outlined for manipulating quantum states of atomic ensembles. Specifically, a ``dipole blockade'' technique is considered in which optical excitation of mesoscopic samples into Rydberg states can be used to control the state of ensembles at the level of individual quanta. It is also noted that even simple processes involving atom-photon correlations can be used to effectively manipulate the ensemble states. Potentially these techniques can be used for implementation of important concepts from quantum information science.
We show that coherent multiple light scattering, or diffuse light propagation, in a disordered atomic media prepared at ultralow temperatures can be effectively delayed in the presence of a strong control field initiating a stimulated Raman process. On a relatively short time scale, when the atomic system can preserve its configuration and effects of atomic motion can be ignored, the scattered signal pulse, diffusely propagating via multiple coherent scattering through the media, can be stored in the spin subsystem through its stimulated Raman-type conversion into spin coherence. We demonstrate how this mechanism, potentially interesting for developing quantum memories, would work for the example of a coherent light pulse propagating through an alkali-metal atomic vapor under typical conditions attainable in experiments with ultracold atoms.