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arXiv:1207.2842 · Physical Review A

Spin damping in an rf atomic magnetometer

Orang Alem, Karen L. Sauer, M. V. Romalis

Published Jan 16, 2013• 19 citations
arXivHTMLPDF

Abstract

Under negative feedback, the quality factor $Q$ of a radio-frequency atomic magnetometer can be decreased by more than two orders of magnitude, so that any initial perturbation of the polarized spin system can be rapidly damped, preparing the magnetometer for detection of the desired signal. We find that noise is also suppressed under such spin damping, with a characteristic spectral response corresponding to the type of noise; therefore magnetic, photon shot, and spin-projection noise can be measured distinctly. While the suppression of resonant photon shot noise implies the closed-loop production of polarization-squeezed light, the suppression of resonant spin-projection noise does not imply spin squeezing, rather simply the broadening of the noise spectrum with $Q$. Furthermore, the application of spin damping during phase-sensitive detection suppresses both signal and noise in such a way as to increase the sensitivity bandwidth. We demonstrate a threefold increase in the magnetometer's bandwidth while maintaining 0.3 fT/$\sqrt{\mathrm{Hz}}$ sensitivity.

DOI
10.1103/physreva.87.013413

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Under negative feedback, the quality factor QQQ of a radio-frequency atomic magnetometer can be decreased by more than two orders of magnitude, so that any initial perturbation of the polarized spin system can be rapidly damped, preparing the magnetometer for detection of the desired signal. We find that noise is also suppressed under such spin damping, with a characteristic spectral response corresponding to the type of noise; therefore magnetic, photon shot, and spin-projection noise can be measured distinctly. While the suppression of resonant photon shot noise implies the closed-loop production of polarization-squeezed light, the suppression of resonant spin-projection noise does not imply spin squeezing, rather simply the broadening of the noise spectrum with QQQ. Furthermore, the application of spin damping during phase-sensitive detection suppresses both signal and noise in such a way as to increase the sensitivity bandwidth. We demonstrate a threefold increase in the magnetometer's bandwidth while maintaining 0.3 fT/Hz\sqrt{\mathrm{Hz}}Hz​ sensitivity.
Optically pumped radio frequency (RF) atomic magnetometers have been shown to have an improved sensitivity over standard tuned coils for frequencies less than 50 MHz, making these RF magnetometers attractive for the detection of nuclear quadrupole resonance (NQR) and low-field nuclear magnetic resonance (NMR) signals. In an atomic magnetometer a linearly polarized probe beam measures, through Faraday rotation, the transverse atomic magnetization induced by the resonant RF signal. The resonance, or Larmor, frequency of the magnetometer is easily tuned with a small magnetic field. We construct an atomic magnetometer based on a potassium vapor cell with a measured sensitivity of 0.22 ± 0.02 fT/ √ Hz and a detection bandwidth of 334 ± 11 Hz when tuned to 423 kHz, giving a Q of over 1200. While high Q magnetometers are sensitive to weak magnetic fields, they are also sensitive to magnetic transients, such as those associated with the excitation pulses needed for magnetic resonance. The ringing created by such transients can obscure the signal of interest. This is particularly detrimental for magnetic resonance signals that decay faster than the transverse relaxation rate. We demonstrate that by feeding back part of the optical signal to orthogonal electromagnetic coils, this unwanted ringing can be quickly damped out leaving the magnetometer ready for the detection of the signal. This negative feedback as applied to the K spins is called spin-damping and can be used to relax the K atoms faster by more than two orders of magnitude. Using spin-damping we reduce the dead-time before data acquisition from 0.8 to 0.2 ms in the detection of NQR signals from ammonium nitrate, one of the so-called fertilizer bomb explosives with an NQR frequency of 423 kHz. Furthermore, we discover that spin-damping can not only be used to suppress signals, it can also be used to suppress noise. We show that it can be used to suppress both environmental noise and more fundamental quantum noise, such as photon shot and spin projection noise. The latter suppression opens the door for its use in quantum control to initialize spin systems before measurements. For phase-sensitive detection, as is often used in magnetic resonance, spin-damping suppresses signal and noise in such a way as to increase the sensitivity bandwidth of the magnetometer. We prove, both theoretically and experimentally, that it is possible to increase the magnetometer detection bandwidth by a factor of 3 or more without significant loss in sensitivity. Such gains in bandwidth for a high Q magnetometer translate into savings in detection time, particularly for substance detection where the frequency of the signal of interest may not be completely known.
We study the effect of optical squeezing on the performance of a sensitive, quantum-noise-limited optically-pumped magnetometer. We use Bell-Bloom optical pumping to excite a 87^{87}87Rb vapor and Faraday rotation to detect spin precession. The sub-pT/Hz\mathrm{pT}/\sqrt{\mathrm{Hz}}pT/Hz​ sensitivity is limited by spin projection noise (photon shot noise) at low (high) frequencies. Probe polarization squeezing both improves high-frequency sensitivity and increases signal bandwidth. The accompanying polarization anti-squeezing perturbs only an unmeasured spin component, so there is no loss of sensitivity at any frequency. The method is compatible with high-density and multi-pass techniques that reach extreme sensitivity.
We study the effect of optical polarization squeezing on the performance of a sensitive, quantum-noise-limited optically pumped magnetometer. We use Bell-Bloom (BB) optical pumping to excite a ^{87}Rb vapor containing 8.2×10^{12} atoms/cm^{3} and Faraday rotation to detect spin precession. The sub-pT/sqrt[Hz] sensitivity is limited by spin projection noise (photon shot noise) at low (high) frequencies. Probe polarization squeezing both improves high-frequency sensitivity and increases measurement bandwidth, with no loss of sensitivity at any frequency, a direct demonstration of the evasion of measurement backaction noise. We provide a model for the quantum noise dynamics of the BB magnetometer, including spin projection noise, probe polarization noise, and measurement backaction effects. The theory shows how polarization squeezing reduces optical noise, while measurement backaction due to the accompanying ellipticity antisqueezing is shunted into the unmeasured spin component. The method is compatible with high-density and multipass techniques that reach extreme sensitivity.
We study quantum enhancement of sensitivity using squeezed light in a multiparameter quantum sensor, the hybrid dc and rf optically pumped magnetometer (hOPM) [M. Lipka , Multiparameter quantum sensing and magnetic communication with a hybrid dc and rf optically pumped magnetometer, , 034054 (2024)]. Using a single spin ensemble, the hOPM acquires both the dc field strength (scalar magnetometry) and resonantly detects one quadrature of the ac magnetic field at a chosen frequency (rf magnetometry). In contrast to the Bell-Bloom scalar magnetometer [C. Troullinou , Squeezed-light enhancement and backaction evasion in a high sensitivity optically pumped magnetometer, , 193601 (2021)], the backaction evasion in the hOPM is incomplete, leading to a nontrivial interplay of the three quantum noise sources in this system: photon shot noise, spin projection noise, and measurement backaction noise. We observe these interactions using squeezed light as a tool to control the distribution of optical quantum noise between S 2 and S 3 polarization Stokes components, and the resulting effect on readout quantum noise and measurement backaction. These results demonstrate quantum-enhanced sensitivity in a continuously operating multiparameter sensor and reveal fundamental trade-offs between sensitivity, backaction, and bandwidth.
We propose and demonstrate a radio-frequency (rf) atomic magnetometer based on parametric resonances. Previously, most rf atomic magnetometers are based on magnetic resonances and their sensitivities are often limited by spin-exchange relaxation. Here, we introduce a novel scheme for an rf magnetometer where the rf magnetic field is measured by exciting the parametric resonances instead of magnetic resonances using parametric modulation fields. In this way, the spin-exchange relaxation is almost eliminated. Benefiting from the low spin relaxation rate, the parametric resonance scheme exhibits a narrower linewidth and stronger signal, which results in a higher sensitivity. With a 6×6×3 mm^{3} Rb atomic vapor cell, we developed an rf atomic magnetometer with a noise floor of 2 fT/Hz^{1/2}, which is about one order of magnitude higher than the sensitivity achieved in the magnetic-resonance-based scheme. The presented rf detection scheme holds promise in advancing rf atomic magnetometers and brings new insight into their various applications.
We study the effect of optical polarization squeezing on the performance of a sensitive, quantum-noise-limited optically pumped magnetometer. We use Bell-Bloom (BB) optical pumping to excite a Rb87 vapor containing 8.2×1012 atoms/cm3 and Faraday rotation to detect spin precession. The sub-pT/Hz sensitivity is limited by spin projection noise (photon shot noise) at low (high) frequencies. Probe polarization squeezing both improves high-frequency sensitivity and increases measurement bandwidth, with no loss of sensitivity at any frequency, a direct demonstration of the evasion of measurement backaction noise. We provide a model for the quantum noise dynamics of the BB magnetometer, including spin projection noise, probe polarization noise, and measurement backaction effects. The theory shows how polarization squeezing reduces optical noise, while measurement backaction due to the accompanying ellipticity antisqueezing is shunted into the unmeasured spin component. The method is compatible with high-density and multipass techniques that reach extreme sensitivity.