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arXiv:1206.7091 · Physical Review Letters

Magic Radio-Frequency Dressing of Nuclear Spins in High-Accuracy Optical Clocks

T. Zanon-Willette, Emeric de Clercq, E. Arimondo

Published Nov 30, 2012• 18 citations
arXivHTMLPDF

Abstract

A Zeeman-insensitive optical clock atomic transition is engineered when nuclear spins are dressed by a nonresonant radio-frequency field. For fermionic species as (87)Sr, (171)Yb, and (199)Hg, particular ratios between the radio-frequency driving amplitude and frequency lead to "magic" magnetic values where a net cancelation of the Zeeman clock shift and a complete reduction of first-order magnetic variations are produced within a relative uncertainty below the 10(-18) level. An Autler-Townes continued fraction describing a semiclassical radio-frequency dressed spin is numerically computed and compared to an analytical quantum description including higher-order magnetic field corrections to the dressed energies.

DOI
10.1103/physrevlett.109.223003

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A Zeeman-insensitive optical clock atomic transition is engineered when nuclear spins are dressed by a nonresonant radio-frequency field. For fermionic species as (87)Sr, (171)Yb, and (199)Hg, particular ratios between the radio-frequency driving amplitude and frequency lead to "magic" magnetic values where a net cancelation of the Zeeman clock shift and a complete reduction of first-order magnetic variations are produced within a relative uncertainty below the 10(-18) level. An Autler-Townes continued fraction describing a semiclassical radio-frequency dressed spin is numerically computed and compared to an analytical quantum description including higher-order magnetic field corrections to the dressed energies.
It has been proposed to use magnetically trapped atomic ensembles to enhance the interrogation time in microwave clocks. To mitigate the perturbing effects of the magnetic trap, near-magic-field configurations are employed, where the involved clock transition becomes independent of the atom's potential energy to first order. Still, higher order effects are a dominating source for dephasing, limiting the performance of this approach. Here we propose a simple method to cancel the energy dependence to both first and second order, using weak radio-frequency dressing. We give values for dressing frequencies, amplitudes, and trapping fields for 87Rb{}^{87}\mathrm{Rb}87Rb atoms and investigate quantitatively the robustness of these second-order-magic conditions to variations of the system parameters. We conclude that radio-frequency dressing can suppress field-induced dephasing by at least one order of magnitude for typical experimental parameters.
We demonstrate control of the differential Zeeman shift between clock states of ultracold rubidium atoms by means of nonresonant microwave dressing. Using the dc field dependence of the microwave detuning, we suppress the first- and second-order differential Zeeman shift in magnetically trapped 87Rb^{87}\mathrm{Rb}87Rb atoms. By dressing the state pair 5S1/25{S}_{1/2}5S1/2​ F=1F=1F=1, ${m}_{F}=\ensuremath{-}1$ and F=2F=2F=2, mF=1{m}_{F}=1mF​=1, a residual frequency spread of <0.1<0.1<0.1 Hz in a range of 100 mG around a chosen magnetic offset field can be achieved. This is one order of magnitude smaller than the shift of the bare states at the magic field of the Breit-Rabi parabola. We further identify double magic points, around which the clock frequency is insensitive to fluctuations both in the magnetic field and in the dressing Rabi frequency. The technique is compatible with chip-based cold-atom systems and allows the creation of clock and qubit states with reduced sensitivity to magnetic-field noise.
We study the spectral signatures and coherence properties of radio-frequency-dressed hyperfine Zeeman sublevels of 87Rb^{87}\mathrm{Rb}87Rb. Experimentally, we engineer combinations of static and RF magnetic fields to modify the response of the atomic spin states to environmental magnetic field noise. We demonstrate analytically and experimentally the existence of ``magic'' dressing conditions where decoherence due to electromagnetic field noise is strongly suppressed. Building on this result, we propose a bichromatic dressing configuration that reduces the global sensitivity of the atomic ground states to low-frequency noise, and enables the simultaneous protection of multiple transitions between the two ground hyperfine manifolds of atomic alkali species. Our methods produce protected transitions between any pair of hyperfine sublevels at arbitrary (low) DC-magnetic fields.
We study the spectral signatures and coherence properties of radio-frequency-dressed hyperfine Zeeman sublevels of Rb87. Experimentally, we engineer combinations of static and RF magnetic fields to modify the response of the atomic spin states to environmental magnetic field noise. We demonstrate analytically and experimentally the existence of "magic"dressing conditions where decoherence due to electromagnetic field noise is strongly suppressed. Building on this result, we propose a bichromatic dressing configuration that reduces the global sensitivity of the atomic ground states to low-frequency noise, and enables the simultaneous protection of multiple transitions between the two ground hyperfine manifolds of atomic alkali species. Our methods produce protected transitions between any pair of hyperfine sublevels at arbitrary (low) DC-magnetic fields.
A form of quantum control is proposed by applying twisted light, also known as optical vortex beams, to drive ultranarrow atomic transitions in neutral Ca, Mg, Yb, Sr, Hg, and Cd bosonic isotopes. This innovative all-optical spectroscopic method introduces spatially tailored electric and magnetic fields to fully rewrite atomic selection rules, reducing simultaneously probe-induced frequency shifts and additional action of external ac and dc field distortions. A twisted-light focused probe beam produces strong longitudinal electric and magnetic fields along the laser propagation axis, which opens the $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{0}$ doubly forbidden clock transition with a high E1M1E1M1E1M1 two-photon excitation rate. This long-lived clock transition is thus immune to nonscalar electromagnetic perturbations. Zeeman components of the M2M2M2 magnetic quadrupole $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{2}$ transition considered for quantum computation and simulation are now selectively driven by transverse or longitudinal field gradients with vanishing electric fields. These field gradients are manipulated by the mutual action of orbital and spin angular momentum of the light beam and are used in presence of tunable vector and tensor polarizabilities. A combination of these two different twisted-light induced clock transitions within a single quantum system, at the same magic wavelength and in presence of a common thermal environment, significantly reduces systematic uncertainties. Furthermore, it generates an optical synthetic frequency which efficiently limits the blackbody radiation shift and its variations at room temperature. Engineering light-matter interaction by optical vortices merged with composite pulses will ultimately benefit experimental atomic and molecular platforms targeting an optimal coherent control of quantum states, reliant quantum simulation, novel approaches to atomic interferometry, and precision tests of fundamental theories in physics and high-accuracy optical metrology.
Radio-frequency quantum engineering of spins is based on the dressing by a nonresonant electromagnetic field. Radio-frequency dressing occurs also for the motion of particles, electrons, or ultracold atoms, within a periodic spatial potential. The dressing, producing a renormalization and also a freeze of the system energy, is described by different approaches: dressed atom, magnetic resonance semiclassical treatment, and continued-fraction solution of the Schr\"odinger equation. A comparison between these solutions points out that the semiclassical treatment, to be denoted as the SSS solution, represents the most convenient tool to evaluate the tunneling renormalization of ultracold atoms.