Spontaneous symmetry breaking can lead to the formation of time crystals, as well as spatial crystals. Here we propose a space-time crystal of trapped ions and a method to realize it experimentally by confining ions in a ring-shaped trapping potential with a static magnetic field. The ions spontaneously form a spatial ring crystal due to Coulomb repulsion. This ion crystal can rotate persistently at the lowest quantum energy state in magnetic fields with fractional fluxes. The persistent rotation of trapped ions produces the temporal order, leading to the formation of a space-time crystal. We show that these space-time crystals are robust for direct experimental observation. We also study the effects of finite temperatures on the persistent rotation. The proposed space-time crystals of trapped ions provide a new dimension for exploring many-body physics and emerging properties of matter.
Spontaneous symmetry breaking can lead to the formation of time crystals, as well as spatial crystals. Here we propose a space-time crystal of trapped ions and a method to realize it experimentally by confining ions in a ring-shaped trapping potential with a static magnetic field. The ions spontaneously form a spatial ring crystal due to Coulomb repulsion. This ion crystal can rotate persistently at the lowest quantum energy state in magnetic fields with fractional fluxes. The persistent rotation of trapped ions produces the temporal order, leading to the formation of a space-time crystal. We show that these space-time crystals are robust for direct experimental observation. We also study the effects of finite temperatures on the persistent rotation. The proposed space-time crystals of trapped ions provide a new dimension for exploring many-body physics and emerging properties of matter.
A constructive theoretical platform for the description of quantum space-time crystals uncovers for N interacting and ring-confined rotating particles the existence of low-lying states with proper space-time crystal behavior. The construction of the corresponding many-body trial wave functions proceeds first via symmetry breaking at the mean-field level followed by symmetry restoration using projection techniques. The ensuing correlated many-body wave functions are stationary states and preserve the rotational symmetries, and at the same time they reflect the point-group symmetries of the mean-field crystals. This behavior results in the emergence of sequences of select magic angular momenta Lm. For angular-momenta away from the magic values, the trial functions vanish. Symmetry breaking beyond the mean-field level can be induced by superpositions of such good-Lm many-body stationary states. We show that superposing a pair of adjacent magic angular momenta states leads to formation of special broken-symmetry states exhibiting quantum space-time-crystal behavior. In particular, the corresponding particle densities rotate around the ring, showing undamped and nondispersed periodic crystalline evolution in both space and time. The experimental synthesis of such quantum space-time-crystal wave packets is predicted to be favored in the vicinity of ground-state energy crossings of the Aharonov-Bohm-type spectra accessed via an externally applied, natural or synthetic, magnetic field. These results are illustrated here for Coulomb-repelling fermionic ions and for a lump of contact-interaction attracting bosons.
Ion Coulomb crystals are ordered structures formed by laser-cooled ions in traps that are characterized by interparticle distances of several micrometers and energy scales on the order of μeV. Their crystalline structure emerges from the interplay between Coulomb repulsion and the external confining potential, which can be readily tuned. Moreover, individual ions can be precisely manipulated with lasers and imaged via resonance fluorescence. These unusual and unique properties make ion crystals a powerful platform for studying phases of matter in the strongly correlated regime and at low temperatures where their dynamics is manifestly quantum mechanical. This review examines the theoretical framework and experimental characterization of ion Coulomb crystals from a condensed-matter perspective. We discuss their dynamical and thermodynamic properties in one, two, and three dimensions, and review recent investigations into their out-of-equilibrium behavior. We provide outlooks on future directions for exploring novel condensed matter phenomena with trapped ion crystals, as well as for exploiting these features for scientific and technical applications.
We investigate the structural properties and melting behaviors of two-dimensional ion crystals in an RF trap, focusing on the effects of ion temperature and trap potential symmetry. We identify distinct crystal structures that form under varying trapping conditions and temperatures through experimental observations and theoretical analyses. As the temperature increases or the trap potential becomes more symmetric, we observe a transition from a lattice arrangement to elongated ring-like formations aligned along the trap axes. Our experimental and theoretical efforts enhance our understanding of phase transitions in low-dimensional, confined systems, offering insights into the controlled formation of quantum crystals for applications in quantum simulations and many-body physics.
The electronic and motional degrees of freedom of trapped ions can be controlled and coherently coupled on the level of individual quanta.Assembling complex quantum systems ion by ion while keeping this unique level of control remains a challenging task.For many applications, linear chains of ions in conventional traps are ideally suited to address this problem.However, driven motion due to the magnetic or radio-frequency electric trapping fields sometimes limits the performance in one dimension and severely affects the extension to higher-dimensional systems.Here, we report on the trapping of multiple barium ions in a single-beam optical dipole trap without radio-frequency or additional magnetic fields.We study the persistence of order in ensembles of up to six ions within the optical trap, measure their temperature, and conclude that the ions form a linear chain, commonly called a one-dimensional Coulomb crystal.As a proof-of-concept demonstration, we access the collective motion and perform spectrometry of the normal modes in the optical trap.Our system provides a platform that is free of driven motion and combines advantages of optical trapping, such as state-dependent confinement and nanoscale potentials, with the desirable properties of crystals of trapped ions, such as long-range interactions featuring collective motion.Starting with small numbers of ions, it has been proposed that these properties would allow the experimental study of many-body physics and the onset of structural quantum phase transitions between one-and two-dimensional crystals.
Recently, Wilczek proposed a fascinating new concept of time crystals, which spontaneously break the continuous time translation symmetry, in analogy with ordinary crystals which break the continuous spatial translation symmetry. Li et al. soon followed with a concrete proposal for an experimental realization and observation of a (space-)time crystal using trapped ions in a ring threaded by an Aharonov-Bohm flux. However, the very existence, even as a matter of principle, of time crystals is rather controversial. Bruno proved a no-go theorem for time crystals for a specific class of Hamiltonians, which covers the original proposal. A similar observation was made for a charge density wave in a superconducting ring by Nozieres. However, since these arguments were not fully general, several new realizations of time crystals, which avoid these no-go arguments, were proposed. In fact, a part of the confusion can be attributed to the lack of a precise mathematical definition of time crystals. Here, we first propose a definition of time crystals in the equilibrium, which is a natural generalization of that of ordinary crystals and can be formulated precisely also for time crystals. We then prove generally the absence of time crystals defined as such, in the ground state of an arbitrary Hamiltonian which consists only of short-range interactions. While the nature of the time crystal is less understood, it is natural to expect that time crystals would be most easily realized, if at all, at zero temperature, as in the case of ordinary crystals. Thus, we focus on the question whether time crystals can exist as the ground state, as in Wilczek’s original proposal. Naively, time crystals would be defined in terms of the ground-state expectation value of an observable O(t). If it exhibits a periodic time dependence, the system may be regarded as a time crystal. However, the very definition of the ground state Ĥ|0〉 = E0|0〉 immediately implies that the expectation value of any Heisenberg operator O(t) ≡ eiĤtO(0)e−iĤt is time-independent. Yet it is too early to reject the idea of time crystals just from this observation, since a similar argument would preclude ordinary (spatial) crystals. One might naively define crystals from a spatially modulating expectation value of the density operator ρ(~x) = e−i ~ P ·~xρ(~0)ei ~ P ·~x. The unique ground state of the Hamiltonian in a finite box is nevertheless symmetric and hence ~ P |0〉 = 0, implying that 〈0|ρ(~x)|0〉 is constant over space.
Ion Coulomb crystals of laser-cooled Ca+ ions have been observed in a cryogenic linear octupole rf ion trap for the first time. Due to the almost field-free central region, large ion crystals containing over 104 ions of millimeter size were successfully produced. The shapes of the crystals can be manipulated by changing the static voltages applied to the octupole rods and the endcap electrodes. Quasi-two-dimensional Coulomb crystals consisting of a small number of ions were also observed with single-ion sensitivity. When a large number of ions is crystallized in the octupole trap, a new kind crystal image with a dip along the axial direction was obtained. The results show that a linear octupole trap and multipole traps are available for producing large, cold, and novel ion Coulomb crystals. The planar ring-type crystal which has not been observed before may lead to future interesting applications.