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arXiv:1712.08385 · Physical Review X

Optical Trapping of Ion Coulomb Crystals

Julian Schmidt, Alexander Lambrecht, Pascal Weckesser, Markus Debatin, Leon Karpa, Tobias Schaetz

Published May 1, 2018• 46 citations
arXivHTMLPDF

Abstract

The electronic and motional degrees of freedom of trapped ions can be controlled and coherently coupled on the level of individual quanta.Assembling complex quantum systems ion by ion while keeping this unique level of control remains a challenging task.For many applications, linear chains of ions in conventional traps are ideally suited to address this problem.However, driven motion due to the magnetic or radio-frequency electric trapping fields sometimes limits the performance in one dimension and severely affects the extension to higher-dimensional systems.Here, we report on the trapping of multiple barium ions in a single-beam optical dipole trap without radio-frequency or additional magnetic fields.We study the persistence of order in ensembles of up to six ions within the optical trap, measure their temperature, and conclude that the ions form a linear chain, commonly called a one-dimensional Coulomb crystal.As a proof-of-concept demonstration, we access the collective motion and perform spectrometry of the normal modes in the optical trap.Our system provides a platform that is free of driven motion and combines advantages of optical trapping, such as state-dependent confinement and nanoscale potentials, with the desirable properties of crystals of trapped ions, such as long-range interactions featuring collective motion.Starting with small numbers of ions, it has been proposed that these properties would allow the experimental study of many-body physics and the onset of structural quantum phase transitions between one-and two-dimensional crystals.

DOI
10.1103/physrevx.8.021028

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The electronic and motional degrees of freedom of trapped ions can be controlled and coherently coupled on the level of individual quanta.Assembling complex quantum systems ion by ion while keeping this unique level of control remains a challenging task.For many applications, linear chains of ions in conventional traps are ideally suited to address this problem.However, driven motion due to the magnetic or radio-frequency electric trapping fields sometimes limits the performance in one dimension and severely affects the extension to higher-dimensional systems.Here, we report on the trapping of multiple barium ions in a single-beam optical dipole trap without radio-frequency or additional magnetic fields.We study the persistence of order in ensembles of up to six ions within the optical trap, measure their temperature, and conclude that the ions form a linear chain, commonly called a one-dimensional Coulomb crystal.As a proof-of-concept demonstration, we access the collective motion and perform spectrometry of the normal modes in the optical trap.Our system provides a platform that is free of driven motion and combines advantages of optical trapping, such as state-dependent confinement and nanoscale potentials, with the desirable properties of crystals of trapped ions, such as long-range interactions featuring collective motion.Starting with small numbers of ions, it has been proposed that these properties would allow the experimental study of many-body physics and the onset of structural quantum phase transitions between one-and two-dimensional crystals.
Abstract Isolating neutral and charged particles from the environment is essential in precision experiments. For decades, this has been achieved by trapping ions with radio-frequency (RF) fields and neutral particles with optical fields. Recently, the trapping of ions by interaction with light has been demonstrated. This might permit the advantages of optical trapping and ions to be combined. For example, we would benefit from superimposing optical traps to investigate ensembles of ions and atoms in the absence of any RF fields and from the versatile and scalable trapping geometries featured by optical lattices. In particular, ions provide individual addressability, and electronic and motional degrees of freedom that can be coherently controlled and detected via high-fidelity, state-dependent operations. Their long-range Coulomb interaction is significantly larger compared to those of neutral atoms and molecules. This enables ultra-cold interaction and the chemistry of trapped ions and atoms to be studied, as well as providing a novel platform for higher-dimensional experimental quantum simulations. The aim of this topical review is to present the current state of the art and to discuss the current challenges and prospects of the emerging field.
Laser cooled ions in a Penning trap can be isolated from the environment by placing them in vacuum and only interacting with them through optical and RF fields. The number of trapped particles can be varied from a single ion up to thousands. Confinement is provided by a static homogeneous magnetic field and a quadrupole electric potential. In the natural frame of the ions, this appears as a 3D simple harmonic potential. Therefore three dimensional structures can be formed in the absence of any additional RF field which may lead to heating as is the case with RF traps. There are 3N different motional modes for N particles. I present an analysis of the motion of a single particle showing that the energy levels for all three modes are equally spaced. I also describe the interaction between a trapped two level atom and an optical field. During my time in the lab the laser and computer control of the experiment has been significantly improved. In addition, an existing trap was modified to provide greater optical access and fluorescence collection. This allowed the vibrational levels superimposed on the internal states of a single 40Ca+ ion to be resolved via a narrow linewidth, electric quadrupole transition. This is the first observation of magnetron and modified cyclotron sidebands on an optical transition. When more than one calcium ion is laser cooled, and their temperature reduced below 5mK, they form a Coulomb crystal. The locations of the ions minimise the total potential energy which is comprised of the Coulomb repulsion and trap potential. The fluorescence collection optics have been arranged to resolve individual ions in these crystals. Information about the motion of the ions is deduced by comparing photos from the experiment to numerical simulations. Previously, only two ions have ever been aligned along the magnetic field in a Penning trap. I present strings of up to 29 particles and suggest the only limitation, apart from the electrode structure, is the overlap of the laser beams with the ions.
Leading quantum platforms are largely limited to one or two dimensions, whereas three-dimensional Coulomb crystals of trapped ions self-assemble into dense qubit arrays with no rearrangement overhead. Coherent optical control of such crystals has nonetheless been out of reach, because the optical transition couples to nearly all 3N3N3N collective modes, i.e., a thermally occupied quasi-continuum bath. Here we cool about 3,600 modes of a crystal of over 1,200 ions below single-phonon occupation, using a continuous cooling band that spans more than five octaves in vibrational spectrum, from about 50 kHz to 2.1 MHz. The crystal then serves as a register of optical qubits, allowing global initialization, coherent manipulation and collective detection. We demonstrate ensemble optical coherence of 21.6 milliseconds and reduce the optical-transition frequency uncertainty from 389 Hz for a single ion to 12 Hz for over a thousand ions, approaching the expected projection-noise scaling. Our approach could be extended to even larger crystals with phonon-mediated many-body couplings, opening a route towards entanglement-enhanced precision metrology and three-dimensional quantum simulation, particularly with spatial-shaped illumination for region-resolved collective control.
For conventional ion traps, the trapping potential is close to independent of the electronic state, providing confinement for ions dependent primarily on their charge-to-mass ratio Q/mQ/mQ/m. In contrast, storing ions within an optical dipole trap results in state-dependent confinement. Here we experimentally study optical dipole potentials for 138Ba+^{138}\mathrm{Ba}^{+}138Ba+ ions stored within two distinctive traps operating at 532 and 1064 nm. We prepare the ions in either the electronic ground (6S1/26{S}_{1/2}6S1/2​) or one of the metastable excited states (5D3/25{D}_{3/2}5D3/2​ or 5D5/25{D}_{5/2}5D5/2​) and probe the relative strength and polarity of the potential. On the one hand, we apply our findings to selectively remove ions from a Coulomb crystal, despite all ions sharing the same Q/mQ/mQ/m. On the other hand, we deterministically purify the trapping volume from parasitic ions in higher-energy orbits, resulting in reliable isolation of Coulomb crystals down to a single ion within a radio-frequency trap.
Controlled quantum mechanical motion of trapped atomic ions can be used to simulate and explore collective quantum phenomena and to process quantum information. Groups of cold atomic ions in an externally applied trapping potential self-organize into "Coulomb crystals" due to their mutual electrostatic repulsion. The motion of the ions in these crystals is strongly coupled, and the eigenmodes of motion all involve multiple ions. While this enables studies of many-body physics, it limits the flexibility and tunability of the system as a quantum platform. Here, we demonstrate an array of trapped ions in individual trapping sites whose motional modes can be controllably coupled and decoupled by tuning the local applied confining potential for each ion. We show that a single motional quantum, or phonon, can be coherently shared among two or three ions confined at the vertices of an equilateral triangle 30 μμμm on a side. We can adiabatically tune the ion participation in the motional modes around a closed contour in configuration space, observing that the single-phonon wavefunction acquires a topological Berry phase if the contour encircles a conical intersection of motional eigenvalue surfaces. We observe this phase by single-phonon interference and study its breakdown as the motional mode tuning becomes non-adiabiatic. Our results show that precise, individual quantum control of ion motion in a two-dimensional array can provide unique access to quantum multi-body effects.
Coulomb crystals of cold trapped ions are a leading platform for the realization of quantum processors and quantum simulations and, in quantum metrology, for the construction of optical atomic clocks and for fundamental tests of the standard model.For these applications, it is not only essential to cool the ion crystal in all its degrees of freedom down to the quantum ground state but also to be able to determine its temperature with a high accuracy.However, when a large ground-state cooled crystal is interrogated for thermometry, complex many-body interactions take place, making it challenging to accurately estimate the temperature with established techniques.In this work, we present a new thermometry method tailored for ion crystals.The method is applicable to all normal modes of motion and does not suffer from a computational bottleneck when applied to large ion crystals.We test the temperature estimate with two experiments, namely with a one-dimensional linear chain of four ions and a two-dimensional crystal of 19 ions and verify the results, where possible, using other methods.The results show that the new method is an accurate and efficient tool for thermometry of ion crystals.