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arXiv:1204.0553 · Physical Review A

Entanglement in atomic systems interacting with single-photon pulses in free space

Jader P. Santos, F. L. Semião

Published Nov 21, 2012• 1 citation
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Abstract

New technologies providing tightly focusing lenses and mirrors with large numerical apertures and electro-optic modulation of single photons are now available for the investigation of photon-atom interactions without a cavity. From the theoretical side, new models must be developed which take into account the intrinsic open system aspect of the problem as well as details about atomic relative positions and temporal (spectral) features of the pulses. In this paper, we investigate the generation of nonclassical correlations between two atoms in free space interacting with a quantized pulse containing just one single photon. For this purpose, we develop a general theoretical approach which allows us to find the equations of motion for single- and two-body atomic operators from which we obtained the system density operator. We show that one single photon is capable of promoting substantial entanglement between two initially ground-state atoms, and we analyze the dependence of these correlations on atomic relative positions (vacuum effects) and spectral features of the single-photon pulse.

DOI
10.1103/physreva.86.053825

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New technologies providing tightly focusing lenses and mirrors with large numerical apertures and electro-optic modulation of single photons are now available for the investigation of photon-atom interactions without a cavity. From the theoretical side, new models must be developed which take into account the intrinsic open system aspect of the problem as well as details about atomic relative positions and temporal (spectral) features of the pulses. In this paper, we investigate the generation of nonclassical correlations between two atoms in free space interacting with a quantized pulse containing just one single photon. For this purpose, we develop a general theoretical approach which allows us to find the equations of motion for single- and two-body atomic operators from which we obtained the system density operator. We show that one single photon is capable of promoting substantial entanglement between two initially ground-state atoms, and we analyze the dependence of these correlations on atomic relative positions (vacuum effects) and spectral features of the single-photon pulse.
New technologies providing tight focusing lens and mirrors with large numerical apertures and electro-optic modulation of single photons are now available for the investigation of photon-atom interactions without a cavity. From the theoretical side, new models must be developed which take into account the intrinsic open system aspect of the problem as well as details about atomic relative positions and temporal (spectral) features of the pulses. In this paper, we investigate the generation of nonclassical correlations between two atoms in response to their interaction with a quantized pulse containing just one single photon. For this purpose, we develop a general theoretical approach which allows us to find the equations of motion for single- and two-body atomic operators from which we obtained the system density operator. We show that one single photon is capable of generating substantial entanglement between the atoms, and we analyze the dependence of these correlations on atomic relative positions and spectral features of the pulse.
We describe the interaction of two two-level atoms in free space with propagating modes of the quantized electromagnetic field, using the time-dependent Heisenberg-Langevin method. For single- photon pulses, we consider the effect of the pulse's spatial and temporal profiles on the atomic excitation. In particular, we find the ideal shape for a pulse to put exactly one excitation in any desired state of the bi-atomic system. Furthermore, we analyze the differences in the atomic dynamics between the cases of Fock state pulses and coherent state pulses.
This research program investigated the dynamics of open quantum systems in manifestly quantum or nonclassical domains. The research program exploited recently discovered possibilities in the microscopic realm of quantum mechanics to accomplish tasks that would otherwise be impossible by traditional classical means, including new capabilities for precision measurement and for the processing and distribution of information. Within this setting, the particular investigations related to strong coupling in optical physics whereby nonlinear interactions require only single atoms and photons. The research achieved capabilities beyond traditional nonlinear optics and laser physics and moved into a new regime with dynamical processes involving atoms and photons taken one by one. The research program addressed fundamental issues related to quantum metrology, to quantum communications, and to the general development of quantum information sciences. The most important accomplishments of this work have been the following: (1) The first demonstration of a laser that operates with a single atom; (2) The first realization of a deterministic source for single photons that generates single photons "on demand" from one atom trapped in a cavity; (3) The development of a protocol for the real-time determination of the number of trapped atoms inside an optical cavity in a regime of strong coupling, with N = 0,1,2,3...atoms; and (4) The first experiment to achieve manifestly quantum or nonclassical photon correlations suitable for the implementation of scalable quantum communications networks.
State mapping between atoms and photons, and photon-photon interactions play an important role in scalable quantum information processing. We consider the interaction of a two-level atom with a quantized propagating pulse in free space and study the probability Pe(t){P}_{e}(t)Pe​(t) of finding the atom in the excited state at any time ttt. This probability is expected to depend on (i) the quantum state of the pulse field and (ii) the overlap between the pulse and the dipole pattern of the atomic spontaneous emission. We show that the second effect is captured by a single parameter $\ensuremath{\Lambda}\ensuremath{\in}[0,8\ensuremath{\pi}/3]$, obtained by weighting the dipole pattern with the numerical aperture. Then, Pe(t){P}_{e}(t)Pe​(t) can be obtained by solving time-dependent Heisenberg-Langevin equations. We provide detailed solutions for both single-photon Fock state and coherent states and for various temporal shapes of the pulses.
In this thesis the entanglement properties of atom-atom, atom-photon, and photon-photon are investigated. The recent developments of quantum computation as well as quantum information and communication have attracted much interest in the generation of these entanglements in the laboratory. To generate atom-photon entanglement, I discuss a model system in the cavity QED setup. By using a four-level atom and two resonant cavity modes, we can generate atom-photon entanglement almost deterministically. An extension of the above model to a six-level atom and again two resonant cavity modes can generate entangled photon pairs by appropriately adjusting system parameters. I then investigate the atom-atom entanglement in a 1D harmonic trap. I show the dependence of the pair entanglement on the scattering length and temperature, as well as the particle symmetry requirement (bosons or fermions). Among many peculiar properties in a 1D system, we briefly discuss the Fermi-Bose duality". While the entanglement properties of a single-channel model have recently been obtained for 1D and 3D systems, I thus study the entanglement of a multi-channel process in a cylindrical harmonic trap. I discuss the dependence of entanglement on the trap geometry. Finally I present detailed studies of the spin mixing between two Rb87 atoms in a single lattice site. The topic is emphasized on various motional state approximations and dipolar effect. Various motional state approximations can cause up to 20% error to experimental data. I also find that the dipolar interaction can lead to an experimentally observable frequency shift in a cylindrical harmonic trap with very large aspect ratio. The spin mixing of spin-2 manifold has also been discussed.
Rapid advances in quantum technology have made possible the control of quantum states of elementary material quantum systems, such as atoms or molecules, and of the electromagnetic radiation field resulting from spontaneous photon emission of their unstable excited states to such a level of precision that subtle quantum electrodynamical phenomena have become observable experimentally. Recent developments in the area of quantum information processing demonstrate that characteristic quantum electrodynamical effects can even be exploited for practical purposes provided the relevant electromagnetic field modes are controlled by appropriate cavities. A central problem in this context is the realization of an ideal transfer of quantum information between a state of a material quantum system and a quantum state of the electromagnetic radiation field which contains a small number or even a single photon only. Despite much recent work in cavity quantum electrodynamics, which has explored this problem successfully in cases in which the number of accessible electromagnetic field modes is strongly restricted by a cavity, currently still much less is known about ideal quantum state transfer between matter and few-photon quantum states of the electromagnetic field in the extreme opposite case of free space. In this contribution we review recent work which explores characteristic quantum electrodynamical phenomena governing the interaction of a material quantum system with the electromagnetic field in extreme many-mode cases which are close to cavity-free situations. For this purpose the simplest possible quantum electrodynamical situation, namely the interaction of a single material two-level system with the wave packet of a single optical photon, is investigated in free space and in situations in which a large cavity modifies the mode structure of the electromagnetic field modes. It is demonstrated that perfect excitation of an atom by a properly shaped single-photon wave packet is possible even in free space. In particular, it is demonstrated that perfect excitation of an atom can be achieved by a single optical photon which is prepared initially in an appropriate superposition of plane-wave modes, provided this photon is focused subsequently onto the absorbing atom by a parabolic cavity.