We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.
We investigate the low temperature phase of a vector spin glass in the limit of large component numbers
m of the spins, where this model is expected to be replica symmetric. On a Bethe lattice, a random graph with fixed and finite connectivity, we employ a self-consistent effective-field approach to the cavity method to describe equilibrium states of the system in terms of the configuration of cavity fields, which are reduced mean fields onto each spin. We make use of an iterative algorithm to find such equilibrium states for finite system sizes
N and observe a phase transition, which is indicated by an order parameter describing the preferred direction each spin points into in terms of the configuration of cavity, resp. mean local fields. On single realizations of Bethe lattices the transition is sharp and accompanied by the Generalized-Bose-Einstein condensation, in which the cavity, resp. local fields of the spins condense into a subspace of the available
m-dimensional space for large
m. The dimension of this subspace,
meff(T) depends on the temperature. Is either one or two right at the critical temperature and increases below. Furthermore, for fixed temperature it is expected to scale with the system size
N with an exponent
μm which depends on the connectivity. Averaging over many realizations of disorder we find
meff(Tc)=2 and
meff(T)∼Nμm. Even more, the cavity fields are subject to rotations in the low temperature phase, i.e. there is no freezing in time as generally expected. In case of
meff(Tc)=2 the whole configuration rotates at the critical temperature about the same angle and the same axis of rotation corresponding to a single droplet. In addition, we find replica symmetry breaking below the large-
m limit, i.e. for
meff(T)>m. These results are supported by results of parallel tempering Monte Carlo simulations. Replica symmetry breaking is further investigated by an analytical method in the large connectivity limit, where we compare the free energy in terms of spin-spin-correlations of different replicas calculated with a replica symmetric and a one-step broken replica symmetry ansatz. In the large-
m limit, we find that both solutions coexist for finite connectivities and that replica symmetry holds for full connectivity up to corrections in second order around the saddle point for
m→∞. In the last chapter we calculate the sample-to-sample fluctuations of the free energy of the SK model of the large-
m limit. We derive an exact connection between these fluctuations and bond chaos. Making use of a replica calculation for the {\it large deviations} and a scaling ansatz for the {\it small deviations}, we quantify bond chaos, i.e. calculate the probability of finding a given link overlap for two systems with possibly different sets of bonds. With this, we find the sample-to-sample fluctuations to scale with the number of spins,
N, with an exponent
μ in between
1/5 and
3/10.
Using a renormalization group approach, we solve the time evolution of random Ising spin chains with generic interactions starting from initial states of arbitrary energy. As a function of the Hamiltonian parameters, the system is tuned through a dynamical transition, similar to the ground-state critical point, at which the local spin correlations establish true long-range temporal order. In the state with a dominant transverse field, a spin that starts in an up state loses its orientation with time, while in the ``ordered'' state it never does. As in ground-state quantum phase transitions, the dynamical transition has unique signatures in the entanglement properties of the system. When the system is initialized in a product state, the entanglement entropy grows as
log(t) in the two ``phases,'' while at the critical point it grows as ${\mathrm{log}}^{\ensuremath{\alpha}}(t)$, with $\ensuremath{\alpha}$ a universal number. This universal entanglement growth requires generic (``integrability breaking'') interactions to be added to the pure transverse field Ising model.
Ultracold atomic gases loaded into optical cavities constitute one of the most versatile platforms for the study of out-of-equilibrium dynamics and quantum simulation of many- body systems. In this thesis, we explore these two possibilities, motivated by current state-of-the-art atom-cavity experiments, uncovering novel phenomena and opening up new theoretical and experimental avenues into the intriguing world of quantum many- body physics. First, we study a gas of ultracold atoms coupled to three optical resonators. We show that the inherent Z2 symmetries, associated with each atom-cavity coupling, can be combined into a global SO(3) rotational symmetry which can be spontaneously broken. We determine the phase diagram of the system, which shows the emergence and breaking of the continuous symmetries and displays first- and second-order phase transitions. We argue that by coupling the atoms equally to n different modes, it will in general be possible to generate a global SO(n) symmetry. Second, we investigate the dynamics of a spinor BEC inside an optical cavity. We focus on a two-component Dicke model with complex light-matter couplings, accounting for photon losses. We compute the steady-state phase diagram and find dynamical in- stabilities in the form of limit cycles, heralded by the presence of exceptional points and level attraction. We show that the instabilities are induced by dissipative processes that generate nonreciprocal couplings between the two collective spins. Lastly, we explore the dynamics of a BEC inside an optical cavity in the presence of an optical lattice. We derive an effective master equation by adiabatically eliminating the cavity field. In the bad-cavity regime, we find an infinite-temperature steady state, but with relaxation dynamics that can be highly nontrivial. For small hopping, the interplay between dissipation and strong interactions leads to an algebraic relaxation of the system, whereas for large hopping, the approach to the steady state is exponential. In the good- cavity regime, we show that the system allows for optical pumping between momentum modes, enabling cavity cooling.
Finite-size quantum spin systems can be magnetized by the application of a symmetry-breaking field, but in general their symmetry is expected to be restored once the field is turned off adiabatically. Recently (F. Caleca et al., arXiv:2412.15493) we have shown that systems of half-integer spins with an odd number of sites and a parity-preserving Hamiltonian can retain a finite magnetization, hence exhibiting spontaneous symmetry breaking (SSB) at finite size. Here we generalize this phenomenon to spin chains whose low-energy physics (in zero field) realizes a Luttinger-liquid phase. We observe that odd-sized chains can exhibit a phenomenon of finite-size quasi-SSB, in which a net sub-extensive magnetization,
M∼N1−1/(4K) is retained, where
N is the number of sites and
K the Luttinger exponent. Interestingly, the states prepared by turning off the symmetry-breaking field quasi-adiabatically display scalable spin squeezing -- namely stronger the bigger the system -- regardless of the parity of
N. The scaling of the squeezing parameter is dictated again by the Luttinger exponent,
ξR2∼N−1+1/(2K). This result shows that scalable quantum correlations with metrological significance, associated typically with high-dimensional systems, can be found as well in gapless one-dimensional ones; and they are a direct consequence of the critical nature of Luttinger liquids.
Spontaneous symmetry breaking (SSB) occurs when a many-body system governed by a symmetric Hamiltonian, and prepared in a symmetry-broken state by the application of a field coupling to its order parameter O, retains a finite O value even after the field is switched off. SSB is generally thought to occur only in the thermodynamic limit N→∞ (for N degrees of freedom). In this limit, the time to restore the symmetry once the field is turned off, either via thermal or quantum fluctuations, is expected to diverge. Here, we show that SSB can also be observed in finite-size quantum spin systems, provided that the spin is half-integer and three conditions are met: (1) the ground state of the system has long-range correlations, (2) the Hamiltonian conserves the (spin) parity of the order parameter, and (3) N is odd. Using a combination of analytical arguments and numerical results (based on time-dependent variational Monte Carlo and rotor + spin-wave theory), we show that SSB on finite-size systems can be achieved via a quasiadiabatic preparation of the ground state-which, in U(1)-symmetric systems, is shown to require a symmetry-breaking field vanishing over timescales τ∼O(N). In these systems, the symmetry-broken state exhibits spin squeezing with Heisenberg scaling.