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arXiv:1202.0737 · New Journal of Physics

Equilibrium and disorder-induced behavior in quantum light–matter systems

Eduardo Mascarenhas, Libby Heaney, M C O Aguiar, Marcelo França Santos

Published Apr 25, 2012• 11 citations
arXivHTMLPDF

Abstract

We analyze equilibrium properties of coupled-doped cavities described by the Jaynes–Cummings–Hubbard Hamiltonian. In particular, we characterize the entanglement of the system in relation to the insulating–superfluid phase transition. We point out the existence of a crossover inside the superfluid phase of the system when the excitations change from polaritonic to purely photonic. Using an ensemble statistical approach for small systems and stochastic mean-field theory for large systems, we analyze static disorder of the characteristic parameters of the system and explore the ground state-induced statistics. We report on a variety of glassy phases deriving from the hybrid statistics of the system. On-site strong disorder induces insulating behavior through two different mechanisms. For disorder in the light–matter detuning, low-energy cavities dominate the statistics, allowing the excitations to localize and bunch in such cavities. In the case of disorder in the light–matter coupling, sites with strong coupling between light and matter become very significant, which enhances the Mott-like insulating behavior. Inter-site (hopping) disorder induces fluidity and the dominant sites are strongly coupled to each other.

DOI
10.1088/1367-2630/14/4/043033

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We analyze equilibrium properties of coupled-doped cavities described by the Jaynes–Cummings–Hubbard Hamiltonian. In particular, we characterize the entanglement of the system in relation to the insulating–superfluid phase transition. We point out the existence of a crossover inside the superfluid phase of the system when the excitations change from polaritonic to purely photonic. Using an ensemble statistical approach for small systems and stochastic mean-field theory for large systems, we analyze static disorder of the characteristic parameters of the system and explore the ground state-induced statistics. We report on a variety of glassy phases deriving from the hybrid statistics of the system. On-site strong disorder induces insulating behavior through two different mechanisms. For disorder in the light–matter detuning, low-energy cavities dominate the statistics, allowing the excitations to localize and bunch in such cavities. In the case of disorder in the light–matter coupling, sites with strong coupling between light and matter become very significant, which enhances the Mott-like insulating behavior. Inter-site (hopping) disorder induces fluidity and the dominant sites are strongly coupled to each other.
We discuss the Jaynes–Cummings–Hubbard model describing the superfluid–Mott insulator transition of polaritons (i.e., dressed photon–qubit states) in coupled qubit–cavity arrays in the crossover from strong to weak correlations. In the strongly correlated regime the phase diagram and the elementary excitations of lattice polaritons near the Mott lobes are calculated analytically using a slave-boson theory (SBT). The opposite regime of weakly interacting polariton superfluids is described by a weak-coupling mean-field theory for a generalized multi-mode Dicke model. We show that a remarkable relation between the two theories exists in the limit of large photon bandwidth and large negative detuning, i.e., when the nature of polariton quasiparticles becomes qubit-like. In this regime, the weak-coupling theory predicts the existence of a single Mott lobe with a change of the universality class of the phase transition at the tip of the lobe, in perfect agreement with the SBT. Moreover, the spectra of low energy excitations, i.e., the sound velocity of the Goldstone mode and the gap of the amplitude mode match exactly as calculated from both theories.
We study the interplay of disorder with pumping and decay in coupled qubit-cavity arrays, the Jaynes-Cummings-Hubbard model. We find that relatively weak disorder can wash out the bistability present in the clean pumped system and that moreover the combination of disorder in on-site energies and decay can lead to effective phase disorder. To explore these questions, we present a nonequilibrium generalization of stochastic mean-field theory, providing a simple tool to address such questions. This technique is developed for rather general forms of light-matter coupling, driving, dissipation, and on-site disorder, making it applicable to a wide range of systems.
An empirical framework for studying the way vacuum fluctuations in a Fabry–Perot cavity produce collective light–matter hybrid states (polariton states) is reported. The reason that the Tavis–Cummings model, where a single mode of the radiation field couples to all the molecules, succeeds is discussed in terms of the strong phase correlation of the vacuum fluctuations in the cavity, which produces a single effective cavity mode (ECM). The model is used to study the onset of the collective state, or “superradiant phase”, for ensembles of molecules with significant disorder in their transition energies, as a function of cavity strength factor, from low Q cavities to high Q cavities. A key result is the quantification of the coherence of the ensemble of the lowest energy eigenstate. This is assessed, primarily, using an entropy distance measure. The statistical model provides a physical intuition for the formation of coherence of polariton states when the collective coupling is strong enough that they dominate over the tail of the dark-state density-of-states.
The superfluid to Mott insulator transition in cavity polariton arrays is analyzed using the variational cluster approach, taking into account quantum fluctuations exactly on finite length scales. Phase diagrams in one and two dimensions exhibit important non-mean-field features. Single-particle excitation spectra in the Mott phase are dominated by particle and hole bands separated by a Mott gap. In contrast to Bose-Hubbard models, detuning allows for changing the nature of the bosonic particles from quasilocalized excitons to polaritons to weakly interacting photons. The Mott state with density one exists up to temperatures T/g > or = 0.03, implying experimentally accessible temperatures for realistic cavity couplings g.
The nature of the ground states for a system composed of two coupled cavities with each containing a pair of dipole-coupled two-level atoms are studied over a wide range of detunings and dipole coupling strengths. The cases for three limits of exact resonance, large positive and negative detunings are discussed, and four types of the ground states are revealed. Then the phase diagrams of the ground state are plotted by choosing three different "order parameters". We find that the phase space, determined by the combinative action of detuning and the dipole coupling strength, is divided into four regions. This is different from the general Bose-Hubbard model and more richer physics are presented in the two-site coupled cavities system. That is, the insulator region may be polaritonic or atomic and the superfluid region may be polaritonic or photonic in nature.
Regular arrays of electromagnetic resonators, in turn coupled coherently to individual quantum two-level systems, exhibit a quantum phase transition of polaritons from a superfluid phase to a Mott-insulating phase. The critical behavior of such a Jaynes-Cummings lattice thus resembles the physics of the Bose-Hubbard model. We explore this analogy by elaborating on the mean-field theory of the phase transition and by presenting several useful mappings which pinpoint both similarities and differences of the two models. We show that a field-theory approach can be applied to prove the existence of multicritical curves analogous to the multicritical points of the Bose-Hubbard model, and we provide analytical expressions for the position of these curves.