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arXiv:0803.3963 · Physical Review Letters

Quantum Fluctuations, Temperature, and Detuning Effects in Solid-Light Systems

Markus Aichhorn, Martin Hohenadler, Charles Tahan, P. B. Littlewood

Published May 29, 2008• 84 citations
arXivHTMLPDF

Abstract

The superfluid to Mott insulator transition in cavity polariton arrays is analyzed using the variational cluster approach, taking into account quantum fluctuations exactly on finite length scales. Phase diagrams in one and two dimensions exhibit important non-mean-field features. Single-particle excitation spectra in the Mott phase are dominated by particle and hole bands separated by a Mott gap. In contrast to Bose-Hubbard models, detuning allows for changing the nature of the bosonic particles from quasilocalized excitons to polaritons to weakly interacting photons. The Mott state with density one exists up to temperatures T/g > or = 0.03, implying experimentally accessible temperatures for realistic cavity couplings g.

DOI
10.1103/physrevlett.100.216401

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•Jan 1, 2013•8 citations
The superfluid to Mott insulator transition in cavity polariton arrays is analyzed using the variational cluster approach, taking into account quantum fluctuations exactly on finite length scales. Phase diagrams in one and two dimensions exhibit important non-mean-field features. Single-particle excitation spectra in the Mott phase are dominated by particle and hole bands separated by a Mott gap. In contrast to Bose-Hubbard models, detuning allows for changing the nature of the bosonic particles from quasilocalized excitons to polaritons to weakly interacting photons. The Mott state with density one exists up to temperatures T/g > or = 0.03, implying experimentally accessible temperatures for realistic cavity couplings g.
Spectral properties of the Bose-Hubbard model and a recently proposed coupled-cavity model are studied by means of quantum Monte Carlo simulations in one dimension. Both models exhibit a quantum phase transition from a Mott insulator to a superfluid phase. The dynamic structure factor $S(k,\ensuremath{\omega})$ and the single-particle spectrum $A(k,\ensuremath{\omega})$ are calculated, focusing on the parameter region around the phase transition from the Mott insulator with density one to the superfluid phase, where correlations are important. The strongly interacting nature of the superfluid phase manifests itself in terms of additional gapped modes in the spectra. Comparison is made to recent analytical work on the Bose-Hubbard model. Despite some subtle differences due to the polaritonic particles in the cavity model, the gross features are found to be very similar to the Bose-Hubbard case. For the polariton model, emergent particle-hole symmetry near the Mott lobe tip is demonstrated and temperature and detuning effects are analyzed. A scaling analysis for the generic transition suggests mean-field exponents, in accordance with field-theory results.
Recent experiments on strongly coupled cavity quantum electrodynamics present new directions in ``matter-light'' systems. Following on from our previous work [Phys. Rev. Lett. 102, 135301 (2009)] we investigate Bose-Hubbard models coupled to a cavity light field. We discuss the emergence of photoexcitations or ``polaritons'' within the Mott phase, and obtain the complete variational phase diagram. Exploiting connections to the super-radiance transition in the Dicke model we discuss the nature of polariton condensation within this novel state. Incorporating the effects of carrier superfluidity, we identify a first-order transition between the super-radiant Mott phase and the single component atomic superfluid. The overall predictions of mean field theory are in excellent agreement with exact diagonalization and we provide details of superfluid fractions, density fluctuations, and finite size effects. We highlight connections to recent work on coupled cavity arrays.
We discuss the Jaynes–Cummings–Hubbard model describing the superfluid–Mott insulator transition of polaritons (i.e., dressed photon–qubit states) in coupled qubit–cavity arrays in the crossover from strong to weak correlations. In the strongly correlated regime the phase diagram and the elementary excitations of lattice polaritons near the Mott lobes are calculated analytically using a slave-boson theory (SBT). The opposite regime of weakly interacting polariton superfluids is described by a weak-coupling mean-field theory for a generalized multi-mode Dicke model. We show that a remarkable relation between the two theories exists in the limit of large photon bandwidth and large negative detuning, i.e., when the nature of polariton quasiparticles becomes qubit-like. In this regime, the weak-coupling theory predicts the existence of a single Mott lobe with a change of the universality class of the phase transition at the tip of the lobe, in perfect agreement with the SBT. Moreover, the spectra of low energy excitations, i.e., the sound velocity of the Goldstone mode and the gap of the amplitude mode match exactly as calculated from both theories.
We propose a scheme which can realize an extended two-component Bose-Hubbard model using polaritons confined in an array of optical cavities. In addition to the density-dependent interactions, this model also contains nonlinear coupling terms between the two components of the polariton. Using a mean-field calculation, we obtain the phase diagram which shows how these terms affect the transition between the Mott insulator and the superfluid phase. In addition, we employ both a perturbation approach and an exact diagonalization method to gain more insights into the phase diagram.
In this work, we study the exciton-polariton condensate phase transition in a microcavity matter-light system in which electron-hole Coulomb interaction and matter-light coupling effects are treated on an equal footing. In the framework of the unrestricted Hartree-Fock approximation applying the two-dimensional exciton-polariton model, we derive the self-consistent equations determining simultaneously the excitonic and the photonic condenstate order parameters. In the thermal-equilibrium limit, we find a condensed state of the exciton-polariton systems and phase diagrams are then constructed. At a given low temperature, the condensate by its nature shows a crossover from an excitonic to a polaritonic and finally photonic condensed state as the excitation density increases at large detuning. Without the detuning, the excitonic condensed state disappears whereas the polaritonic or photonic phases dominate. The crossover is also found by lowering the Coulomb interaction at a finite matter-light coupling. Lowering the Coulomb interaction or increasing the temperature, the excitonic Mott transition occurs, at which the exciton-polariton condensates dissociate to free electron-hole/photon. Depending on temperature and excitation density, the phase transition of the exciton-polariton condensates is also addressed in signatures of photoluminescence mapping to the photonic momentum distribution.
Ultracold atoms uniformly filling an optical lattice can be treated like an artificial crystal. An implementation including the atomic occupation of a single excited atomic state can be represented by a two-component Bose-Hubbard model. Its phase diagram exhibits a quantum phase transition from a superfluid to a Mott insulator phase. The dynamics of electronic excitations governed by electrostatic dipole-dipole interactions in the ordered regime can be well described by wave-like collective excitations called excitons. Here we present an extensive study of such excitons for a wide range of geometries and dimensionality. Their lifetimes can vary over many orders of magnitude from metastable propagation to superradiant decay. Particularly strong effects occur in one dimensional atomic chains coupled to tapered optical fibers. For an optical lattice within a cavity the excitons are coupled to cavity photons and the resulting collective cavity QED model can be efficiently formulated in terms of polaritons. Their properties are explicitly calculated for different lattices and they constitute a non-destructive monitoring tool for important system properties. Even the formation of molecules in optical lattices manifests itself in modified polariton properties as e.g. an anisotropic optical spectrum. Partial dissipation of the exciton energy in the lattice leads to heating, which can be microscopically understood through a mechanism transferring atoms into higher Bloch bands via a resonant excitation transfer among neighboring lattice sites. The presence of lattice defects like vacancies in the Mott insulator induces a characteristic scattering of polaritons, which can be optically observed to monitor the lattice integrity. Our models can be applied to simulate and understand corresponding collective phenomena in solid crystals, where many effects are often masked by noise and disorder.