Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1110.0962 · Physical Review B

Spontaneous dimerization in the spin-1 bilinear-biquadratic Heisenberg model on a honeycomb lattice

Yu-Wen Lee, Min-Fong Yang

Published Mar 6, 2012• 12 citations
arXivHTMLPDF

Abstract

Within the linear flavor-wave theory, we show that due to the quantum order-by-disorder mechanism, the spin-1 bilinear-biquadratic Heisenberg model on a honeycomb lattice can spontaneously develop a columnar dimer order with a non-bipartite structure. The low-lying excitations above this novel ground state form several flat bands separated by nonzero energy gaps. Our results suggest that the quantum phase transition separating this dimerized phase with the nearby N\'eel-order phase may be of first order.

DOI
10.1103/physrevb.85.100402

Related papers

Plaquette order and deconfined quantum critical point in the spin-1 bilinear-biquadratic Heisenberg model on the honeycomb lattice

Hui‐Hai Zhao, Cenke Xu, Qiaoni Chen +4 more

We have precisely determined the ground state phase diagram of the quantum spin-1 bilinear-biquadratic Heisenberg model on the honeycomb lattice using the tensor renormalization group method. We find that the ferromagnetic, ferroquadrupolar, and a large part of the antiferromagnetic phases are stable against quantum fluctuations. However, around the phase where the ground state is antiferroquadrupolar ordered in the classical limit, quantum fluctuations suppress completely all magnetic orders, leading to a plaquette order phase which breaks the lattice symmetry but preserves the spin SU(2) symmetry. On the evidence of our numerical results, the quantum phase transition between the antiferromagnetic phase and the plaquette phase is found to be either a direct second order or a very weak first order transition.

arXiv:1105.2716•Physical Review B•Apr 9, 2012•69 citations

Quantum phases in the frustrated Heisenberg model on the bilayer honeycomb lattice

Hao Zhang, Marcelo Arlego, Carlos Alberto Lamas

We use a combination of analytical and numerical techniques to study the phase diagram of the frustrated Heisenberg model on the bilayer honeycomb lattice. Using the Schwinger-boson description of the spin operators followed by a mean-field decoupling, the magnetic phase diagram is studied as a function of the frustration coupling ${J}_{2}$ and the interlayer coupling ${J}_{\ensuremath{\perp}}$. The presence of both magnetically ordered and disordered phases is investigated by means of the evaluation of ground-state energy, spin gap, local magnetization, and spin-spin correlations. We observe a phase with a spin gap and short-range N\'eel correlations that survives for nonzero next-nearest-neighbor interaction and interlayer coupling. Furthermore, we detect signatures of a reentrant behavior in the melting of the N\'eel phase and symmetry restoring when the system undergoes a transition from an on-layer nematic valence-bond crystal phase to an interlayer valence-bond crystal phase. We complement our work with exact diagonalization on small clusters and dimer-series expansion calculations, together with a linear spin-wave approach to study the phase diagram as a function of the spin $S$, the frustration, and the interlayer couplings.

arXiv:1312.6324•Physical Review B•Jan 6, 2014•31 citations

Dimerized Phase and Transitions in a Spatially Anisotropic Square Lattice Antiferromagnet

Oleg A. Starykh, Leon Balents

We investigate the spatially anisotropic square lattice quantum antiferromagnet. The model describes isotropic spin-1/2 Heisenberg chains (exchange constant J) coupled antiferromagnetically in the transverse (J( perpendicular )) and diagonal (J(x)), with respect to the chain, directions. Classically, the model admits two ordered ground states-with antiferromagnetic and ferromagnetic interchain spin correlations-separated by a first-order phase transition at J( perpendicular )=2J(x). We show that in the quantum model this transition splits into two, revealing an intermediate quantum-disordered columnar dimer phase, both in two dimensions and in a simpler two-leg ladder version. We describe quantum-critical points separating this spontaneously dimerized phase from classical ones.

arXiv:cond-mat/0402055•Physical Review Letters•Sep 15, 2004•128 citations

Spontaneous dimer order, excitation spectrum and quantum-phase transitions in the J 1 - J 2 Heisenberg model

Jaan Oitmaa Valeri N. Kotov

We overview some recent work and present new results on the ground-state properties and the spectrum of excitations of the two-dimensional frustrated Heisenberg antiferromagnet. Spontaneous dimer order is present in the quantum disordered phase of this model. We study the stability and analyse the structure of the spectrum, including the two-particle singlet excitation branch throughout the disordered phase, as well as in the vicinity of the Neel critical point. The variation in the dimer order parameter is also given, and it is argued that near the critical point it reflects the presence of the low-energy singlet bound state.

Philosophical Magazine B•Jul 11, 2000•10 citations

Spontaneous dimer order, excitation spectrum and quantum-phase transitions in the J1-J2 Heisenberg model

Valeri N. Kotov, J. Oitmaa, Oleg P. Sushkov +1 more

We overview some recent work and present new results on the ground-state properties and the spectrum of excitations of the two-dimensional frustrated Heisenberg antiferromagnet. Spontaneous dimer order is present in the quantum disordered phase of this model. We study the stability and analyse the structure of the spectrum, including the two-particle singlet excitation branch throughout the disordered phase, as well as in the vicinity of the Neel critical point. The variation in the dimer order parameter is also given, and it is argued that near the critical point it reflects the presence of the low-energy singlet bound state.

arXiv:cond-mat/9912228•Philosophical Magazine B•Aug 1, 2000•34 citations

Quantum paramagnetic ground states on the honeycomb lattice and field-induced Néel order

R. Ganesh, D. N. Sheng, Young‐June Kim +1 more

Bi${}_{3}$Mn${}_{4}$O${}_{12}$(NO${}_{3}$) is a recently synthesized spin-3/2 bilayer honeycomb antiferromagnet which behaves as a spin liquid down to very low temperatures. Beyond a magnetic field of about 5 T, it develops long-range N\'eel order. Motivated by this observation, we have studied spin-$S$ Heisenberg models with next neighbor frustrating interactions as well as bilayer couplings on the honeycomb lattice. For a model with frustrating second-neighbor exchange, ${J}_{2}$, we use a Lindemann-like criterion within spin-wave theory to show that N\'eel order melts beyond a critical ${J}_{2}$. The critical ${J}_{2}$ is found to increase in the presence of a magnetic field, implying the existence of a field-induced paramagnet-N\'eel transition over a range of parameters. For the bilayer model, we use a spin-$S$ generalization of bond operator mean-field theory to show that there is a N\'eel-dimer transition for various spin values with increasing bilayer coupling and that the resulting interlayer dimer state undergoes a field-induced transition into a state with transverse N\'eel order. Motivated by a broader interest in such paramagnets, we have also studied a spin-3/2 model which interpolates between the nearest-neighbor Heisenberg model and the Affleck-Kennedy-Lieb-Tasaki (AKLT) parent Hamiltonian. Using exact diagonalization, we have found that there is a single N\'eel-AKLT quantum phase transition in this model. Computing the fidelity susceptibility and assuming a transition in the O(3) universality class, we have located the critical point of this model. In addition, we have obtained the spin gap of the AKLT parent Hamiltonian. Our numerics indicate that the AKLT state also undergoes a field-induced N\'eel ordering transition. We discuss implications of some of our results for experiments on Bi${}_{3}$Mn${}_{4}$O${}_{12}$(NO${}_{3}$) and for numerics on the honeycomb lattice Hubbard model.

arXiv:1012.0316•Physical Review B•Apr 18, 2011•76 citations
Within the linear flavor-wave theory, we show that due to the quantum order-by-disorder mechanism, the spin-1 bilinear-biquadratic Heisenberg model on a honeycomb lattice can spontaneously develop a columnar dimer order with a non-bipartite structure. The low-lying excitations above this novel ground state form several flat bands separated by nonzero energy gaps. Our results suggest that the quantum phase transition separating this dimerized phase with the nearby N'eel-order phase may be of first order.
We have precisely determined the ground state phase diagram of the quantum spin-1 bilinear-biquadratic Heisenberg model on the honeycomb lattice using the tensor renormalization group method. We find that the ferromagnetic, ferroquadrupolar, and a large part of the antiferromagnetic phases are stable against quantum fluctuations. However, around the phase where the ground state is antiferroquadrupolar ordered in the classical limit, quantum fluctuations suppress completely all magnetic orders, leading to a plaquette order phase which breaks the lattice symmetry but preserves the spin SU(2) symmetry. On the evidence of our numerical results, the quantum phase transition between the antiferromagnetic phase and the plaquette phase is found to be either a direct second order or a very weak first order transition.
We use a combination of analytical and numerical techniques to study the phase diagram of the frustrated Heisenberg model on the bilayer honeycomb lattice. Using the Schwinger-boson description of the spin operators followed by a mean-field decoupling, the magnetic phase diagram is studied as a function of the frustration coupling J2{J}_{2}J2​ and the interlayer coupling ${J}_{\ensuremath{\perp}}$. The presence of both magnetically ordered and disordered phases is investigated by means of the evaluation of ground-state energy, spin gap, local magnetization, and spin-spin correlations. We observe a phase with a spin gap and short-range N\'eel correlations that survives for nonzero next-nearest-neighbor interaction and interlayer coupling. Furthermore, we detect signatures of a reentrant behavior in the melting of the N\'eel phase and symmetry restoring when the system undergoes a transition from an on-layer nematic valence-bond crystal phase to an interlayer valence-bond crystal phase. We complement our work with exact diagonalization on small clusters and dimer-series expansion calculations, together with a linear spin-wave approach to study the phase diagram as a function of the spin SSS, the frustration, and the interlayer couplings.
We investigate the spatially anisotropic square lattice quantum antiferromagnet. The model describes isotropic spin-1/2 Heisenberg chains (exchange constant J) coupled antiferromagnetically in the transverse (J( perpendicular )) and diagonal (J(x)), with respect to the chain, directions. Classically, the model admits two ordered ground states-with antiferromagnetic and ferromagnetic interchain spin correlations-separated by a first-order phase transition at J( perpendicular )=2J(x). We show that in the quantum model this transition splits into two, revealing an intermediate quantum-disordered columnar dimer phase, both in two dimensions and in a simpler two-leg ladder version. We describe quantum-critical points separating this spontaneously dimerized phase from classical ones.
We overview some recent work and present new results on the ground-state properties and the spectrum of excitations of the two-dimensional frustrated Heisenberg antiferromagnet. Spontaneous dimer order is present in the quantum disordered phase of this model. We study the stability and analyse the structure of the spectrum, including the two-particle singlet excitation branch throughout the disordered phase, as well as in the vicinity of the Neel critical point. The variation in the dimer order parameter is also given, and it is argued that near the critical point it reflects the presence of the low-energy singlet bound state.
We overview some recent work and present new results on the ground-state properties and the spectrum of excitations of the two-dimensional frustrated Heisenberg antiferromagnet. Spontaneous dimer order is present in the quantum disordered phase of this model. We study the stability and analyse the structure of the spectrum, including the two-particle singlet excitation branch throughout the disordered phase, as well as in the vicinity of the Neel critical point. The variation in the dimer order parameter is also given, and it is argued that near the critical point it reflects the presence of the low-energy singlet bound state.
Bi3{}_{3}3​Mn4{}_{4}4​O12{}_{12}12​(NO3{}_{3}3​) is a recently synthesized spin-3/2 bilayer honeycomb antiferromagnet which behaves as a spin liquid down to very low temperatures. Beyond a magnetic field of about 5 T, it develops long-range N\'eel order. Motivated by this observation, we have studied spin-SSS Heisenberg models with next neighbor frustrating interactions as well as bilayer couplings on the honeycomb lattice. For a model with frustrating second-neighbor exchange, J2{J}_{2}J2​, we use a Lindemann-like criterion within spin-wave theory to show that N\'eel order melts beyond a critical J2{J}_{2}J2​. The critical J2{J}_{2}J2​ is found to increase in the presence of a magnetic field, implying the existence of a field-induced paramagnet-N\'eel transition over a range of parameters. For the bilayer model, we use a spin-SSS generalization of bond operator mean-field theory to show that there is a N\'eel-dimer transition for various spin values with increasing bilayer coupling and that the resulting interlayer dimer state undergoes a field-induced transition into a state with transverse N\'eel order. Motivated by a broader interest in such paramagnets, we have also studied a spin-3/2 model which interpolates between the nearest-neighbor Heisenberg model and the Affleck-Kennedy-Lieb-Tasaki (AKLT) parent Hamiltonian. Using exact diagonalization, we have found that there is a single N\'eel-AKLT quantum phase transition in this model. Computing the fidelity susceptibility and assuming a transition in the O(3) universality class, we have located the critical point of this model. In addition, we have obtained the spin gap of the AKLT parent Hamiltonian. Our numerics indicate that the AKLT state also undergoes a field-induced N\'eel ordering transition. We discuss implications of some of our results for experiments on Bi3{}_{3}3​Mn4{}_{4}4​O12{}_{12}12​(NO3{}_{3}3​) and for numerics on the honeycomb lattice Hubbard model.