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arXiv:1109.5480 · Physical Review A

Quantum crystals in a trapped Rydberg-dressed Bose-Einstein condensate

C.-H. Hsueh, Tai‐Chia Lin, Tzyy‐Leng Horng, W. C. Wu

Published Jul 16, 2012• 38 citations
arXivHTMLPDF

Abstract

Based on a mean-field approach, spontaneously crystalline ground states, called quantum crystals, of a trapped Rydberg-dressed Bose-Einstein condensate are numerically investigated. In a quasi-two-dimensional geometry, a hexagonal lattice of condensate droplets manifests when dressed coupling is above a critical value. The onset of the crystallized state is characterized by a drastic drop of the nonclassical rotational inertia fraction (NCRIF). Nevertheless, the NCRIF remains a large value for a large span of dressed coupling, which indicates that the long-range phase coherence of a superfluid is preserved in the crystallized state. By relaxing the confinement against the two-dimensional geometry and by introducing an anisotropic interaction, an $AB$ stacking bilayer lattice and a nearly square lattice, respectively, are also available in the system. A quasi-one-dimensional lattice is also shown.

DOI
10.1103/physreva.86.013619

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Based on a mean-field approach, spontaneously crystalline ground states, called quantum crystals, of a trapped Rydberg-dressed Bose-Einstein condensate are numerically investigated. In a quasi-two-dimensional geometry, a hexagonal lattice of condensate droplets manifests when dressed coupling is above a critical value. The onset of the crystallized state is characterized by a drastic drop of the nonclassical rotational inertia fraction (NCRIF). Nevertheless, the NCRIF remains a large value for a large span of dressed coupling, which indicates that the long-range phase coherence of a superfluid is preserved in the crystallized state. By relaxing the confinement against the two-dimensional geometry and by introducing an anisotropic interaction, an ABABAB stacking bilayer lattice and a nearly square lattice, respectively, are also available in the system. A quasi-one-dimensional lattice is also shown.
We numerically investigate the quantum crystallographic phases of a Rydberg-dressed Bose gas loaded on a square lattice by using the mean-field Gross-Pitaevskii model. For a relatively weak lattice confinement, the phases of ground state undergo amorphism, polycrystal, and polymorphism following the increase of the blockade radius, and if the confinement is stronger, a single crystal with a specific filling factor will be formed. In order to distinctively characterize these phases, the structure function is also studied. In such an anisotropic system, we show that the superfluid-fraction tensor should be a measurable quantity, and an anisotropy parameter can be defined. In addition, for such crystallographic phases, the interaction potential can manifest where the grain boundaries appear.
We study rotating quasi-two-dimensional Bose-Einstein condensates, in which atoms are dressed to a highly excited Rydberg state. This leads to weak effective interactions that induce a transition to a mesoscopic supersolid state. Considering slow rotation, we determine its superfluidity using quantum Monte Carlo simulations as well as mean field calculations. For rapid rotation, the latter reveal an interesting competition between the supersolid crystal structure and the rotation-induced vortex lattice that gives rise to new phases, including arrays of mesoscopic vortex crystals.
We numerically investigate the vortex structures in a fast rotating two-dimensional Rydberg-dressed Bose-Einstein condensate (BEC) taking into account the Lee-Huang-Yang (LHY) quantum correction. In a rotating BEC of reduced dimensionality, it is shown that there is room to tune the LHY coupling against the short- and long-range couplings. In the absence of the LHY effect, hexagonal, square, striped, and honeycomb lattices can exhibit upon increasing the long-range interaction, which can be realized in the context of superfluid (SF)-supersolid (SS) transition. In the presence of the LHY effect, competition between LHY and long-range terms results in rich lattice structures. In particular, clustering of multiple vortices can occur due to the trapping effect of the SS triangles or grids. Estimates of number of vortices in the clustering are provided.
Rydberg-dressed ground state atoms are atoms with an electron off-resonantly excited to a very high energy state, i.e., a state of high principal quantum number n ≫ 1. This thesis investigates the quantum dynamics of interacting Rydberg-dressed ground state atoms trapped in several multi-well potential traps. Rydberg atoms are atoms with exaggerated properties. One of their most interesting properties is that they exhibit a strong and long-ranged interaction that can be tuned leading to a variety of different quantum behaviours. My work focuses on studying the effects of these interacting atoms when loaded in multi-well potential traps. Generally, multi-well systems are considered as the simplest example of a finite optical lattice structure. For this reason, this thesis covers three research topics that examine the effects of long-range interaction on Rydberg-dressed atoms trapped in several potential confinements. I begin, in the introduction, by discussing the theoretical background of relevance to this work. It starts with presenting the physics of Bose-Einstein condensate. Then, the fundamentals of the interaction between two-level atom and light are analytically studied. This study has the purpose of understanding both; the dressed interacting atoms and optical lattices. The definition, characteristics, and the nature of the interaction between Rydberg atoms are analysed afterwards. The second chapter examines the dynamics of an ensemble of interacting Rydberg- dressed atoms trapped in static, i.e., time-independent, multi-well potentials using a mean-field theoretical approach. I choose one-dimensional double- and triple-well in addition to a two-dimensional quadruple-well potentials. The time-dependent non-linear Gross-Pitaevskii equation is used to numerically explore the ensemble’s quantum dynamics. Solving the dynamical differential equations along with tuning the strength of the applied long-range interaction shows that the behaviour of non-interacting Rydberg-dressed atoms does not differ conceptually according to the geometry of the trapping potential. However, this changes when the interactions are switched on where the shape of the confinement leads to interesting outcomes especially in the non-linear interacting limit, such as macroscopic quantum self-trapping. After investigating an ensemble of interacting Rydberg-dressed atoms in static multi-well potential traps, the second research topic examines the dynamical evolution of these atoms when loaded in a finite optical lattice using the extended Bose-Hubbard model. In this chapter, the atoms ensemble is assumed to be in a superfluid state where I investigate both, the order parameter when the Rydberg excitation laser is applied and the interference pattern of the condensates in different dimensions. The study shows the emerging long-range interactions lead to a rapid collapse of the superfluid order parameter and in general allow only for partial revivals. In addition, the interference experiments can directly reveal the interaction between Rydberg-dressed atoms. In the fourth chapter, the dynamics of Rydberg-dressed atoms trapped in a dynamical, i.e., time-dependent, potential confinement is presented. The dynamical trap is constructed such that it begins as a harmonic oscillator and ends as a double- well potential. The analysis investigates an ensemble of contact-interacting atoms via the time-dependent non-linear GP equation.
Abstract The experimental realization of Rydberg dressing technology in ultracold atomic systems provides another superior platform for studying novel states of matter and macroscopic quantum phenomena. In this work, based on the mean-field theory, we have investigated the ground-state phases of a two-component Bose–Einstein condensate with Rydberg interaction and confined in a toroidal trap. The effects of the Rydberg interaction and external potential, especially the Rydberg blockade radius, on the ground-state structure of such a system have been investigated in full parameter space. Our results show that the Rydberg blockade radius, which can be regarded as another controllable parameter, can be used to obtain a variety of ground-state phases. More interestingly, it is found that for weak Rydberg interactions, the Rydberg blockade radius breaks the spontaneous rotational symmetry of the system, leading to the formation of a discrete unit cell structure. For strongly interacting cases, it can be used to realize different orders of discrete rotational symmetry breaking.
We investigate the ground-state properties and excitations of Rydberg-dressed bosons in both three and two dimensions, using the hypernetted-chain Euler-Lagrange approximation, which accounts for correlations and thus goes beyond the mean-field approximation. The short-range behavior of the pair distribution function signals the instability of the homogeneous system with respect to the formation of droplet crystals at strong couplings and large soft-core radius. This tendency to spatial density modulation coexists with off-diagonal long-range order. The contribution of the correlation energy to the ground-state energy is significant at large coupling strengths and intermediate values of the soft-core radius while for a larger soft-core radius the ground-state energy is dominated by the mean-field (Hartree) energy. We have also performed path integral Monte Carlo simulations at selected system parameters to verify the performance of our hypernetted-chain Euler-Lagrange results in three dimensions. In the homogeneous phase, the two approaches are in very good agreement. Moreover, Monte Carlo simulations predict a first-order quantum phase transition from a homogeneous superfluid phase to the quantum droplet phase with face-centered cubic symmetry for Rydberg-dressed bosons in three dimensions.