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arXiv:1108.3510 · Physical Review A

s -wave-scattering resonances induced by dipolar interactions of polar molecules

Zhe-Yu Shi, Ran Qi, Hui Zhai

Published Feb 27, 2012• 16 citations
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Abstract

We show that the $s$-wave-scattering resonances induced by dipolar interactions in polar molecular gases have a universal large and positive effective range, which is very different from Feshbach resonances previously realized in cold atoms before, where the effective range is either negligible or negative. Such a difference has important consequences in many-body physics. At a high-temperature regime, a positive effective range gives rise to a stronger repulsive interaction energy for positive scattering length, and a weaker attractive interaction energy for negative scattering length. At low temperatures, we study a polaron problem formed by a single-impurity molecule, and we find that the polaron binding energy increases at the BEC side and decreases at the BCS side. All these effects are opposite to narrow Feshbach resonances, where the effective range is negative.

DOI
10.1103/physreva.85.020702

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We show that the sss-wave-scattering resonances induced by dipolar interactions in polar molecular gases have a universal large and positive effective range, which is very different from Feshbach resonances previously realized in cold atoms before, where the effective range is either negligible or negative. Such a difference has important consequences in many-body physics. At a high-temperature regime, a positive effective range gives rise to a stronger repulsive interaction energy for positive scattering length, and a weaker attractive interaction energy for negative scattering length. At low temperatures, we study a polaron problem formed by a single-impurity molecule, and we find that the polaron binding energy increases at the BEC side and decreases at the BCS side. All these effects are opposite to narrow Feshbach resonances, where the effective range is negative.
Based on the recently developed interaction renormalization for the one-dimensional ppp-wave interaction, we study the problem of a single impurity immersed in a highly polarized Fermi sea. They interact through a narrow ppp-wave Feshbach resonance, so the effective range r0{r}_{0}r0​ naturally appears in the system. We use the variational approach limited to single-particle--hole excitations on top of the unperturbed Fermi sea. The polaron exhibits two branches of solutions, namely, the attractive and repulsive branches, with varying scattering length across the resonance. We calculate the energy spectrum, residue, and effective mass for each of the branches. We compare the polaronic energy with the energy of the dressed molecule and find that the molecular state is energetically favored when increasing the interaction strength. The critical interaction strength for the polaron-to-molecule transition will shift to the BCS side of the ppp-wave resonance as the effective range increases.
We investigate Feshbach resonances in collisions of high-spin atoms such as Er and Dy with closed-shell atoms such as Sr and Yb, using coupled-channel scattering and bound-state calculations.We consider both low-anisotropy and high-anisotropy limits.In both regimes, we find many resonances with a wide variety of widths.The wider resonances are suitable for tuning interatomic interactions, while some of the narrower resonances are highly suitable for magnetoassociation to form high-spin molecules.These molecules might be transferred to short-range states, where they would have large magnetic moments and electric dipole moments that can be induced with very low electric fields.The results offer the opportunity to study mixed quantum gases where one species is dipolar and the other is not and open up important prospects for a new field of ultracold high-spin polar molecules.
Abstract. Ultra-cold atomic systems provide a new setting where to investigate the role of longrange interactions. In this paper we will review the basics features of those physical systems, in particular focusing on the case of Chromium atoms. On the experimental side, we report on the observation of dipolar effects in the expansion dynamics of a Chromium Bose-Einstein condensate. By using a Feshbach resonance, the scattering length characterising the contact interaction can be strongly reduced, thus increasing the relative effect of the dipole-dipole interaction. Such experiments make Chromium atoms the strongest candidates at present for the achievement of the strong dipolar regime. On the theoretical side, we investigate the behaviour of ultra-cold dipolar systems in the presence of a periodic potential. We discuss how to realise this situation experimentally and we characterise the system in terms of its quantum phases and metastable states, discussing in detail the differences with respect to the case of zero-range interactions.
We study ultracold gases of alkali-metal atoms in the quantum degenerate regime. The interatomic interactions in these type of systems can be tuned using resonances induced by magnetic or electric fields. The tunability of the interactions, together with the possibility of confining the atoms with several kinds of external potentials, allows for a completely novel approach to study basic problems in many-body physics, and moreover, allows to enter regimes which have never been accessible in condensed matter or nuclear physics. For example, this has led to the experimental demonstration of an intimate relation between two types of superfluidity: the crossover from Bose-Einstein condensation of tightly bound molecules to the superfluid behavior related to weakly bound BCS-like pairs. Another experimental landmark was reached when the existence of universal Efimov three-body bound states was proven in experiments with ultracold bosonic cesium atoms. In this thesis, we study several aspects of these strongly interacting and ultracold atomic gases. We develop an analytical model that encapsulates all of the relevant scattering physics in atomic systems where open-channel shape resonances and closedchannel Feshbach resonances give rise to complicated and non-trivial scattering properties. This model provides lots of physical insight and is shown to describe important quantities, such as the molecular energies and scattering phase shifts, with a high level of accuracy. The model is compared to full numerical coupled-channel calculations in two atomic systems: rubidium and lithium. We study the BCS-BEC crossover using a many-body description of the ultracold gas that includes the non-trivial energy dependence of the scattering model. We show that it gives rise to superfluid behavior associated with the formation of BCS-like pairs while the low-energy interactions are repulsive in character. The energy dependence of the interactions is crucial, as it gives rise to attractive interactions at the Fermi energy, necessary for the formation of Cooper pairs. We demonstrate new ways of controlling the interatomic interactions using a combination of magnetic and electric fields. This leads to experimental control of, for instance, the three-body parameter in the context of Efimov physics and of non-universal behavior in the BCS-BEC crossover in fermionic gases. Using a four-body method based on first principles, we solve the molecule-molecule scattering problem to calculate several important properties of bosonic and fermionic Summary 145 molecules that consist of light and heavy atoms. These type of molecules are of current experimental interest, and we predict several exciting relations between three- and four-body observables in these type of systems.
In this thesis, we investigated the physics of two- and three-dimensional ultra cold Bose gases in the strongly interacting regime at zero temperature. This regime can be experimentally accessed using a Feshbach resonance. We applied a self-consistent diagrammatic approach to determine the chemical potential of three-dimensional Bose gases for a wide range of interaction values. We showed that such strongly interacting Bose gases become unstable towards the formation of molecules at a finite positive scattering length. In fact, the interaction between atoms becomes effectively attractive and the system looses its metastability before reaching the unitary limit. We also found that such systems are nearly fermionized close to the instability point. Near this critical point, the chemical potential reaches a maximum and the contribution to the system energy due to three-body forces is estimated to be only a few percent. We also studied the same system using a self-consistent renormalization group method. This approach confirms the existence of an instability point towards the formation of molecules as well as fermionization. We showed that the instability and accompanying maximum are precursors of the sign change of the effective two-body interaction strength from repulsive to attractive near resonance. In addition, we examined the physics of two-dimensional Bose gases near resonance using a similar self-consistent diagrammatic approach as the one introduced for three-dimensional Bose gases. We demonstrated that a competition between three-body attractive interactions and two-body repulsive forces results in the chemical potential of two-dimensional Bose gases to exhibit a maximum at a critical scattering length beyond which these quantum gases possess a negative compressibility. For larger scattering lengths, the increasingly prominent role played by three-body attractive interactions leads to an onset instability at a second critical value. The three-body effects studied for these systems are universal, fully characterized by the effective two-dimensional scattering length and are, in comparison to the three-dimensional case, independent of three-body ultraviolet physics.
When an impurity is immersed in a Bose-Einstein condensate, impurity-boson interactions are expected to dress the impurity into a quasiparticle, the Bose polaron. We superimpose an ultracold atomic gas of ^{87}Rb with a much lower density gas of fermionic ^{40}K impurities. Through the use of a Feshbach resonance and radio-frequency spectroscopy, we characterize the energy, spectral width, and lifetime of the resultant polaron on both the attractive and the repulsive branches in the strongly interacting regime. The width of the polaron in the attractive branch is narrow compared to its binding energy, even as the two-body scattering length diverges.