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arXiv:1107.5904

Correlation and recombination heating in an ultracold plasma. Analitic estimations

A. P. Gavrilyuk

Published Jul 29, 2011• 0 citations
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Abstract

In the article an ultracold electron-ion plasma created by photoionization of cooled atoms is investigated. We obtained analitical expressions for non-ideality parameters which establish due to correlation heating. In the work the nearest neighbour and the Wigner-Seitz cell approximations were used, the recombination heating of electrons was taken into account. We have got a good agreement with the experiment results. The possibility of creation of strongly non-ideal electron subsystem has been shown and conditions of this process have been determined.

DOI
10.48550/arxiv.1107.5904

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In the recent work Fletcher et al. [Phys. Rev. Lett., v.99, p.145001 (2007)] reported on the novel experimental technique, enabling to measure the temperature of the expanding ultracold plasmas over a considerable time interval (up to 60-70 μs). It was unexpectedly found that the electron temperature dropped with time as T_e(t) ~ t^{-α} with α= 1.2 +/- 0.1 \approx 1 instead of α= 2, which would be expected for the adiabatic cooling of electrons in the cloud expanding linearly in time. The above-cited authors supposed that 'the difference is likely due to the significant heating effects from 3-body recombination' (i.e. the inelastic processes), but they did not provide sufficient quantitative estimates supporting such a conclusion. The aim of the present comment is to mention that the experimentally revealed t^{-1}-dependence can be explained under quite general assumptions by the purely elastic processes in the ultracold plasma, as it was done a few years ago in our work [Yu.V. Dumin, J. Low Temp. Phys., v.119, p.377 (2000)]. Therefore, t^{-1}-dependence revealed in the above-cited experiment should be primarily a manifestation of "virialization" of the electron velocities in the regime of strong electron-ion correlations, while the heat release by inelastic processes should be of secondary importance (it might be responsible, particularly, for changing the exponent from -1 to -1.2). This is confirmed also by our ab initio molecular-dynamic simulations taking into account the strong electron-ion correlations (i.e. not based on the PIC method, Vlasov approximation for electrons, etc., which are applicable only to small-angular scattering).

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This work describes the evolution of an ultracold neutral plasma as it expands freely in vacuum. It presents a comprehensive study of the electron temperature evolution under different initial conditions. Ultracold neutral plasmas are created by photoionizing laser-cooled neutral atoms in ultrahigh vacuum. The ions are typically at a temperature of ∼ 1K while the electron temperature can be set from 1--1000 K. After photoionization, some of the highly energetic electrons escape from the cloud, leaving a net positive charge in the cloud. This creates a Coulomb well which traps the rest of the electrons, and a plasma is formed. Since the electrons have a lot of kinetic energy, they tend to leave the cloud, however, the Coulomb force from the ion pulls the electrons back into the cloud. This exerts a recoil force on the ions, and the whole plasma starts expanding radially outwards. Since the expansion is caused by the thermal pressure of the electrons, a study of the plasma expansion unravels the complicated electron temperature evolution, under different initial conditions. Many collisional processes become significant as a plasma expands. These physical processes tend to heat or cool the ions and electrons, leading to very different kinds of evolution depending on the initial conditions of the plasma. This work demonstrates three different regions of parameter space where the degree of significance of these physical processes is different during the ultracold neutral plasma evolution. The experimental results are verified by theoretical simulations, performed by Thomas Pohl, which untangle the complicated electron temperature evolution.

•Jan 1, 2007•2 citations
In the article an ultracold electron-ion plasma created by photoionization of cooled atoms is investigated. We obtained analitical expressions for non-ideality parameters which establish due to correlation heating. In the work the nearest neighbour and the Wigner-Seitz cell approximations were used, the recombination heating of electrons was taken into account. We have got a good agreement with the experiment results. The possibility of creation of strongly non-ideal electron subsystem has been shown and conditions of this process have been determined.
In recent experiments ultracold plasmas were produced by photoionizing small clouds of laser cooled atoms. This paper presents the results of molecular dynamic simulations for the early time evolution of such plasmas. Contrary to earlier speculation, no evidence of strong electron–electron correlations is observed in the simulations even if the initial value of the coupling parameter (Γe=e2/akTe) is much larger than unity. As electron–electron correlations begin to develop, the correlation energy is released to heat the electrons, raising the electron temperature to the point where Γe∼1 and limiting further development of correlation. Further heating of the electrons occurs as a by-product of three-body recombination. When a model of laser cooling is added to the simulation, the formation of strong ion–ion correlation is observed. Contrary to earlier suggestion, the rate of three-body recombination is observed to be in reasonable agreement with the traditional formula, R=3.9×10−9 s−1[n(cm−3)]2[Te(K)]−9/2, but care must be taken to use the correct temporally evolving temperature, Te. The simulations are challenging because it is necessary to follow three-body recombination into weakly bound (high n quasiclassical) Rydberg states, and the time scale for such states is short compared to that for the plasma dynamics. This kind of problem was faced earlier in computational astrophysics when studying binary star formation in globular clusters and the simulation method used here is adapted from such studies.
We present a theoretical interpretation of the recently revealed features of temperature evolution in the ultracold plasma clouds released from a magneto-optical trap, namely: (a) its independence at the sufficiently large times on the initial plasma parameters and (b) the asymptotics close to t^{-1} instead of t^{-2}, expected for a rarefied ideal gas. It is shown that both these properties can be well explained by the model of virialization of the charged particle velocities in the regime of strong electron-ion correlations, while heating due to inelastic processes (e.g. three-body recombination) should be of secondary importance. These conclusions are confirmed also by the results of ab initio computer simulations.
Ultracold plasmas are a promising candidate for the creation of strongly coupled Coulomb systems. Unfortunately, the values of the coupling parameter Γe actually achieved after photoionization of the neutral atoms remain relatively small because of the considerable intrinsic heating of the electrons. A conceivable way to get around this obstacle might be to utilize a spontaneous ionization of the ultracold Rydberg gas, where the initial kinetic energies could be much less. However, the spontaneous avalanche ionization will result in a very inhomogeneous distribution (clusterization) of the ions, which can change the efficiency of the electron relaxation in the vicinity of such clusters substantially. In the present work, this hypothesis is tested by an extensive set of numerical simulations. As a result, it is found that despite a less initial kinetic energy, the subsequent relaxation of the electron velocities in the clusterized plasmas proceeds much more violently than in the case of the statistically uniform ionic distribution. The electron temperature, first, experiences a sharp initial jump (presumably, caused by the “virialization” of energies of the charged particles) and, second, exhibits a gradual subsequent increase (presumably, associated with a multi-particle recombination of the electrons at the ionic clusters). As a possible tool to reduce the anomalous temperature increase, we also considered a two-step plasma formation, involving the blockaded Rydberg states. This leads to a suppression of the clusterization due to a quasi-regular distribution of ions. In such a case, according to the numerical simulations, the subsequent evolution of the electron temperature proceeds more gently, approximately with the same rate as in the statistically uniform ionic distribution.
Rydberg atom formation is a source of heating in plasmas. The rate of three-body recombination in an ultracold neutral plasma was measured and electron temperature was derived from it using standard equilibrium recombination rates. With large-scale Monte Carlo and particle-in-cell simulations, we have calculated ab initio the rate of excitation, de-excitation, ionization (and recombination) in electron-Rydberg atom collision and investigated the short-time dynamics of three-body recombination in an ultracold neutral plasma. Comparison with observed rates is quite good. Particular attention is paid to the low-frequency microfield effect on Rydberg state cut-off in the plasma.
In the recent work Fletcher et al. [Phys. Rev. Lett., v.99, p.145001 (2007)] reported on the novel experimental technique, enabling to measure the temperature of the expanding ultracold plasmas over a considerable time interval (up to 60-70 μs). It was unexpectedly found that the electron temperature dropped with time as T_e(t) ~ t^{-α} with α= 1.2 +/- 0.1 \approx 1 instead of α= 2, which would be expected for the adiabatic cooling of electrons in the cloud expanding linearly in time. The above-cited authors supposed that 'the difference is likely due to the significant heating effects from 3-body recombination' (i.e. the inelastic processes), but they did not provide sufficient quantitative estimates supporting such a conclusion. The aim of the present comment is to mention that the experimentally revealed t^{-1}-dependence can be explained under quite general assumptions by the purely elastic processes in the ultracold plasma, as it was done a few years ago in our work [Yu.V. Dumin, J. Low Temp. Phys., v.119, p.377 (2000)]. Therefore, t^{-1}-dependence revealed in the above-cited experiment should be primarily a manifestation of "virialization" of the electron velocities in the regime of strong electron-ion correlations, while the heat release by inelastic processes should be of secondary importance (it might be responsible, particularly, for changing the exponent from -1 to -1.2). This is confirmed also by our ab initio molecular-dynamic simulations taking into account the strong electron-ion correlations (i.e. not based on the PIC method, Vlasov approximation for electrons, etc., which are applicable only to small-angular scattering).
This work describes the evolution of an ultracold neutral plasma as it expands freely in vacuum. It presents a comprehensive study of the electron temperature evolution under different initial conditions. Ultracold neutral plasmas are created by photoionizing laser-cooled neutral atoms in ultrahigh vacuum. The ions are typically at a temperature of ∼ 1K while the electron temperature can be set from 1--1000 K. After photoionization, some of the highly energetic electrons escape from the cloud, leaving a net positive charge in the cloud. This creates a Coulomb well which traps the rest of the electrons, and a plasma is formed. Since the electrons have a lot of kinetic energy, they tend to leave the cloud, however, the Coulomb force from the ion pulls the electrons back into the cloud. This exerts a recoil force on the ions, and the whole plasma starts expanding radially outwards. Since the expansion is caused by the thermal pressure of the electrons, a study of the plasma expansion unravels the complicated electron temperature evolution, under different initial conditions. Many collisional processes become significant as a plasma expands. These physical processes tend to heat or cool the ions and electrons, leading to very different kinds of evolution depending on the initial conditions of the plasma. This work demonstrates three different regions of parameter space where the degree of significance of these physical processes is different during the ultracold neutral plasma evolution. The experimental results are verified by theoretical simulations, performed by Thomas Pohl, which untangle the complicated electron temperature evolution.