Atoms can scatter light and they can also amplify it by stimulated emission. From this simple starting point, we examine the possibility of realizing a random laser in a cloud of laser-cooled atoms. The answer is not obvious as both processes (elastic scattering and stimulated emission) seem to exclude one another: pumping atoms to make them behave as amplifier reduces drastically their scattering cross-section. However, we show that even the simplest atom model allows the efficient combination of gain and scattering. Moreover, supplementary degrees of freedom that atoms offer allow the use of several gain mechanisms, depending on the pumping scheme. We thus first study these different gain mechanisms and show experimentally that they can induce (standard) lasing. We then present how the constraint of combining scattering and gain can be quantified, which leads to an evaluation of the random laser threshold. The results are promising and we draw some prospects for a practical realization of a random laser with cold atoms.
We address the problem of achieving an optical random laser with a cloud of cold atoms, in which gain and scattering are provided by the same atoms. The lasing threshold can be defined using the on-resonance optical thickness b0 as a single critical parameter. We predict the threshold quantitatively, as well as power and frequency of the emitted light, using two different light transport models and the atomic polarizability of a strongly pumped two-level atom. We find a critical b0 on the order of 300, which is within reach of state-of-the-art cold-atom experiments. Interestingly, we find that random lasing can already occur in a regime of relatively low scattering.
In the first part of this thesis, a detailed analysis of lasing in random multiple-light-scattering media with gain is presented. Random laser emission is analyzed using a time-dependent diffusion model for light propagating in the medium containing active atoms. We demonstrate the effects of scatterers to narrow the emission spectral linewidth and to shorten the emitted pulse duration at a specific threshold pump intensity. This threshold pump intensity decreases with scatterer density and excitation spot diameter, in excellent agreement with experimental results. The coherence properties of the random laser are studied using a generalized master equation. The random laser medium is treated as a collection of low quality-factor cavities, coupled by random photon diffusion. Laser-like coherence, on average, is demonstrated above a specific pumping threshold. We demonstrate that with stronger scattering, the pumping threshold for the transition from chaotic to isotropic coherent light emission decreases and enhanced optical coherence for the emitted light is achieved above threshold. The second part of this thesis presents a study of lasing in photonic crystals (PCs). The emission from an incoherently pumped atomic system in interaction with the electro-magnetic reservoir of a PC is analyzed using a set of generalized semiclassical Maxwell-Bloch equations. We demonstrate that the photonic band edge facilitates the enhancement of stimulated emission and the reduction of internal losses, leading to an important lowering of the laser threshold. In addition, an increase of the laser output at a photonic band edge is demonstrated. We next develop a detailed quantum theory of a coherently pumped two-level atom in a photonic band gap material, coupled to both a multi-mode wave-guide channel and a high-quality micro-cavity embedded within the PC. The cavity field characteristics are highly distinct from that of a corresponding high-Q cavity in ordinary vacuum. We demonstrate enhanced, inversionless, and nearly coherent light generation when the photon density of states (DOS) jump between the Mollow spectral components of atomic resonance fluorescence is large. In the case of a vanishing photon DOS on the lower Mollow sideband and no dipolar dephasing, the emitted photon statistics is Poissonian and the cavity field exhibits quadrature coherence.
"We propose to study the random laser problem. As a lasing system one considers an active gain medium interacting with a light field where the damping of the latter is treated in the spirit of open systems theory, considering a multimode case with the spectral overlap of the modes in the losses term [11]. We approach the problem by using the density matrix formalism, deriving the master equation for the light field in order to find out the detailed description of the laser like emission. The specific character of the field damping and gain effects essentially modifies the master equation in comparison to that of the ordinary laser and thus contributes to the properties of the resulting laser emission. The derivation of the density operator for the field is the main ingredient for describing the quantum statistical properties of the lasing and such a progress represents a great interest for the study of random laser systems."
We investigate the properties of the cooperative decay modes of a cold atomic cloud, characterized by a Gaussian distribution in three dimensions, initially excited by a laser in the linear regime. We study the properties of the decay rate matrix
S, whose dimension coincides with the number of atoms in the cloud, in order to get a deeper insight into properties of cooperative photon emission. Since the atomic positions are random,
S is a Euclidean random matrix whose entries are a function of the atom distances. We show that in the limit of a large number of atoms in the cloud, the eigenvalue distribution of
S depends on a single parameter
b0, called the cooperativeness parameter, which can be viewed as a quantifier of the number of atoms that are coherently involved in an emission process. For very small values of
b0, we find that the limit eigenvalue density is approximately triangular. We also study the nearest-neighbor spacing distribution and the eigenvector statistics, finding that although the decay rate matrices are Euclidean, the bulk of their spectra mostly behaves according to the expectations of classical random matrix theory. In particular, in the bulk, there is level repulsion and the eigenvectors are delocalized, therefore exhibiting the universal behavior of chaotic quantum systems.