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arXiv:1103.4123 · Physical Review Letters

Kaleidoscope of Exotic Quantum Phases in a Frustrated XY Model

Christopher N. Varney, Kai Sun, Victor M. Galitski, Marcos Rigol

Published Aug 8, 2011• 73 citations
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Abstract

The existence of quantum spin liquids was first conjectured by Pomeranchuk some 70 years ago, who argued that frustration in simple antiferromagnetic theories could result in a Fermi-liquid-like state for spinon excitations. Here we show that a simple quantum spin model on a honeycomb lattice hosts the long sought for Bose metal with a clearly identifiable Bose surface. The complete phase diagram of the model is determined via exact diagonalization and is shown to include four distinct phases separated by three quantum phase transitions.

DOI
10.1103/physrevlett.107.077201

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The existence of quantum spin liquids was first conjectured by Pomeranchuk some 70 years ago, who argued that frustration in simple antiferromagnetic theories could result in a Fermi-liquid-like state for spinon excitations. Here we show that a simple quantum spin model on a honeycomb lattice hosts the long sought for Bose metal with a clearly identifiable Bose surface. The complete phase diagram of the model is determined via exact diagonalization and is shown to include four distinct phases separated by three quantum phase transitions.
The frustrated XY model on the honeycomb lattice has drawn lots of attention because of the potential emergence of chiral spin liquid (CSL) with the increasing of frustrations or competing interactions. In this paper, we study the extended spin-12\frac{1}{2}21​ XY model with nearest-neighbor (J1)({J}_{1})(J1​), and next-nearest-neighbor (J2)({J}_{2})(J2​) interactions in the presence of a three-spins chiral $({J}_{\ensuremath{\chi}})$ term using density matrix renormalization group methods. We obtain a quantum phase diagram with both conventionally ordered and topologically ordered phases. In particular, the long-sought Kalmeyer-Laughlin CSL is shown to emerge under a small ${J}_{\ensuremath{\chi}}$ perturbation due to the interplay of the magnetic frustration and chiral interactions. The CSL, which is a nonmagnetic phase, is identified by the scalar chiral order, the finite spin gap on a torus, and the chiral entanglement spectrum described by chiral SU(2)1SU{(2)}_{1}SU(2)1​ conformal field theory.
Searching for spin-liquid states has long been attracting both experimentalists and theorists. In this paper, we review recent density matrix renormalization group studies of the spin-½ XY model on the honeycomb lattice, with first-neighbor (J1 = 1) and frustrating second-neighbor (J2 > 0) interactions. For the intermediate frustration regime 0.22 ≲ J2 ≲ 0.36, there exists a surprising antiferromagnetic Ising phase, with ordered moments pointing along the z-axis, despite the absence of any SzSz interactions in the Hamiltonian. Surrounding this phase as a function of J2 are antiferromagnetic phases with the moments pointing in the xy-plane for small J2 and a close competition between an xy-plane magnetic collinear phase and a dimer phase for large values of J2. No spin-liquid phases was found in the XY model even with the third-neighbor (J3 > 0) interactions.
We study the spin-1/2 Heisenberg antiferromagnet on a bilayer honeycomb lattice including interlayer frustration. Using a set of complementary approaches, namely, Schwinger bosons, dimer series expansion, bond operators, and exact diagonalization, we map out the quantum phase diagram. Analyzing ground-state energies and elementary excitation spectra, we find four distinct phases, corresponding to three collinear magnetic long-range ordered states, and one quantum disordered interlayer dimer phase. We detail that the latter phase is adiabatically connected to an exact singlet product ground state of the bilayer, which exists along a line of maximum interlayer frustration. The order within the remaining three phases will be clarified.
We have investigated the spin-1/2 XY frustrated antiferromagnetic Heisenberg honeycomb model, which features an intermediate region in its ground state phase diagram that is not well understood. The two dominant phases in the diagram are the quantum spin-liquid (QSL) and the antiferromagnetic Ising order. Quantum correlations suggest that the QSL phase is likely to exhibit entanglement. To explore this possibility, we utilized numerical Lanczos and density matrix renormalization group (DMRG) methods to calculate concurrence, quantum discord (QD), and entanglement entropy. The results of our study indicate the existence of quantum entanglement within the intermediate region, implying a greater probability for the dominance of the quantum spin-liquid (QSL) phase over the antiferromagnetic Ising order. This discovery underscores the importance of considering quantum correlations in comprehending the model's behavior and provides insight into the complex nature of quantum systems.
An emergent SU(4) symmetry discovered in the microscopic model for d1 honeycomb materials [M. G. Yamada, M. Oshikawa, and G. Jackeli, ] has enabled us to tailor exotic SU(4) models in real materials. In the honeycomb structure, the emergent SU(4) Heisenberg model would potentially have a quantum spin-orbital liquid ground state due to the , and we can also expect similar spin-orbital liquids in three-dimensional versions of the honeycomb lattice. In such quantum spin-orbital liquids, both the spin and orbital degrees of freedom become fractionalized and entangled together due to the strong frustrated interactions between them. Similarly to spinons in pure quantum spin liquids, quantum spin-orbital liquids can host not only spinon excitations, but also fermionic excitations at low temperature.
The strong interest in strongly correlated systems in condensed matter physics has continued unabated for the past few decades. In recent years, the number of novel, exotic quantum phases found in theoretical studies has seen a phenomenal rise. Among those interesting quantum states are bose liquids and spin liquids, where strong quantum fluctuations have prevented the systems from developing a long range order. Our work in this thesis seeks to further the understanding of frustrated systems. In the study of a hard-core boson model with ring-only exchange interactions on a square lattice, we obtain concrete numerical realization of the unconventional Exciton Bose Liquid (EBL) phase, which possesses interesting properties such as a "Bose surface" which resembles the Fermi surface in a metal, as well as unusual thermodynamic properties such as a T Log T dependence for specific heat. An equally important result from this work is the demonstration that the widely used Gutzwiller projection on slave-particle wave functions may generally fail to capture the correct long wavelength physics in the respective systems. For the Heisenberg antiferromagnet on the kagome lattice, which is a promising candidate for realizing a spin-disordered ground state, our variational study shows that the projected Schwinger boson wave function is energetically better than the Dirac spin liquid wave function when a small antiferromagnetic second-neighbor spin coupling is added to the nearest-neighbor model. We also study the anisotropic triangular Heisenberg antiferromagnetic in magnetic field, and find simple, yet accurate wave functions for various regions of the surprisingly rich phase diagram, thus providing insights into the energetics of the competing phases in this interesting model. Finally, our work also highlights permanent-type wave functions as potentially useful constructions in variational studies of systems with short-ranged correlations, e.g., a Mott insulator and a gapped spin liquid.