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arXiv:1103.2283 · Physical Review Letters

Extended Coherence Time on the Clock Transition of Optically Trapped Rubidium

G. Kleine Büning, J. Will, Wolfgang A. Ertmer, Ernst Maria Rasel, J. Arlt, Carsten Klempt, F. Ramírez-Martínez, Frédéric Piéchon, P. Rosenbusch

Published Jun 16, 2011• 54 citations
arXivHTMLPDF

Abstract

Optically trapped ensembles are of crucial importance for frequency measurements and quantum memories but generally suffer from strong dephasing due to inhomogeneous density and light shifts. We demonstrate a drastic increase of the coherence time to 21 s on the magnetic field insensitive clock transition of (87)Rb by applying the recently discovered spin self-rephasing [C. Deutsch et al., Phys. Rev. Lett. 105, 020401 (2010)]. This result confirms the general nature of this new mechanism and thus shows its applicability in atom clocks and quantum memories. A systematic investigation of all relevant frequency shifts and noise contributions yields a stability of 2.4×10(-11)τ(-1/2), where τ is the integration time in seconds. Based on a set of technical improvements, the presented frequency standard is predicted to rival the stability of microwave fountain clocks in a potentially much more compact setup.

DOI
10.1103/physrevlett.106.240801

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•Apr 28, 2017•0 citations
Optically trapped ensembles are of crucial importance for frequency measurements and quantum memories but generally suffer from strong dephasing due to inhomogeneous density and light shifts. We demonstrate a drastic increase of the coherence time to 21 s on the magnetic field insensitive clock transition of (87)Rb by applying the recently discovered spin self-rephasing [C. Deutsch et al., Phys. Rev. Lett. 105, 020401 (2010)]. This result confirms the general nature of this new mechanism and thus shows its applicability in atom clocks and quantum memories. A systematic investigation of all relevant frequency shifts and noise contributions yields a stability of 2.4×10(-11)τ(-1/2), where τ is the integration time in seconds. Based on a set of technical improvements, the presented frequency standard is predicted to rival the stability of microwave fountain clocks in a potentially much more compact setup.
We present a compact atomic clock interrogating ultracold 87Rb magnetically trapped on an atom chip. Very long coherence times sustained by spin self-rephasing allow us to interrogate the atomic transition with 85% contrast at 5 s Ramsey time. The clock exhibits a fractional frequency stability of 5.8×10−135.8\times 10^{-13}5.8×10−13 at 1 s and is likely to integrate into the 1×10−151\times10^{-15}1×10−15 range in less than a day. A detailed analysis of 7 noise sources explains the measured frequency stability. Fluctuations in the atom temperature (0.4 nK shot-to-shot) and in the offset magnetic field (5×10−65\times10^{-6}5×10−6 relative fluctuations shot-to-shot) are the main noise sources together with the local oscillator, which is degraded by the 30% duty cycle. The analysis suggests technical improvements to be implemented in a future second generation set-up. The results demonstrate the remarkable degree of technical control that can be reached in an atom chip experiment.
We investigate the collective spin dynamics of a self-rephasing bosonic ensemble of 87Rb^{87}\mathrm{Rb}87Rb trapped in a one-dimensional vertical optical lattice. We show that the combination of the frequency shifts induced by atomic interactions and inhomogeneous dephasing, together with the spin self-rephasing mechanism, leads to the existence of a ``magic density'': i.e., a singular operating point where the clock transition is first-order insensitive to density fluctuations. This feature is very appealing for improving the stability of quantum sensors based on trapped pseudo-spin-1/2 ensembles. Ramsey spectroscopy of the $|5s{\phantom{\rule{3.33333pt}{0ex}}}^{2}{S}_{1/2},F=1,{m}_{F}=0\ensuremath{\rangle}\ensuremath{\rightarrow}|5s{\phantom{\rule{3.33333pt}{0ex}}}^{2}{S}_{1/2},F=2,{m}_{F}=0\ensuremath{\rangle}$ hyperfine transition is in qualitative agreement with a numerical model based on coupled Bloch equations of motion for energy-dependent spin vectors.
In our original paper (Altin et al 2011 New J. Phys. 13 065020), we presented the results from a Ramsey atom interferometer operating with an optically trapped sample of up to 10 6 Bose-condensed 87 Rb atoms in the m F = 0 clock states. We were unable to observe projection noise fluctuations on the interferometer output, which we attribute to the stability of our microwave oscillator and background magnetic field. Numerical simulations of the Gross–Pitaevskii equations for our system show that dephasing due to spatial dynamics driven by interparticle interactions accounts for much of the observed decay in fringe visibility at long interrogation times. The simulations show good agreement with the experimental data when additional technical decoherence is accounted for, and suggest that the clock states are indeed immiscible. With smaller samples of 5 × 10 4 atoms, we observe a coherence time of τ = 1.0 +0.5 −0.3 s.
Abstract We analyze an optical atomic clock using two-photon 5 S 1 / 2 → 4 D J transitions in rubidium. Four one- and two-color excitation schemes to probe the 4 D 3 / 2 and 4 D 5 / 2 fine-structure states are considered in detail. We compare key characteristics of Rb 4 D J and 5 D 5 / 2 two-photon clocks. The 4 D J clock features a high signal-to-noise ratio due to two-photon decay at favorable wavelengths, low dc electric and magnetic susceptibilities, and minimal black-body shifts. Ac Stark shifts from the clock interrogation lasers are compensated by two-color Rabi-frequency matching. We identify a ‘magic’ wavelength near 1060 nm, which allows for in-trap, Doppler-free clock-transition interrogation with lattice-trapped cold atoms. From our analysis of clock statistics and systematics, we project a quantum-noise-limited relative clock stability at the 10 − 13 / τ ( s ) -level, with integration time τ in seconds, and a relative accuracy of ∼ 10 − 13 . We describe a potential architecture for implementing the proposed clock using a single telecom clock laser at 1550 nm, which is conducive to optical communication and long-distance clock comparisons. Our work could be of interest in efforts to realize small and portable Rb clocks and in high-precision measurements of atomic properties of Rb 4 D J -states.
Experiments were carried out to evaluate the performances of a semiconductor laser pumped rubidium (87Rb) atomic clock. Two kinds of Rb gas cells were used and their performances were compared [gas cell A (natural rubidium (87Rb/85Rb =\frac{3}{7}) and buffer gases) and gas cell B (87Rb and buffer gases)]. The highest microwave frequency stabilities were estimated as3.4 \times 10^{-12} \tau^{-1/2}and2.7 \times 10^{-12} \tau^{-1/2}at the optimal gas cell temperatures of 60°C and 48°C for the gas cellsAandB, respectively (τ: integration time). The light shift, i.e., microwave frequency shift induced by laser light, was measured as -0.50 Hz/MHz and -0.11 Hz/MHz for the gas cellsAandBat their optimal operating conditions given above. As an improved experiment by utilizing high temporal coherence of the laser, a novel double resonance spectral line shape with a drastically narrower linewidth was demonstrated. A technique, similar to FM laser spectroscopy, was employed for this purpose by utilizing laser FM sidebands which are induced by microwave frequency modulation and nonlinear susceptibility of three-level87Rb atoms. The minimum linewidth obtained was 20 Hz, which can be used as a sensitive frequency discriminator for an improved87Rb atomic clock.
A review of a cold-atom clock based on coherent population trapping that highlights recent progress will be presented. Improvements in the coherence of the interrogation spectrum have resulted in the generation of dark states in the cold Rb atoms with essentially 100 % transmission – evidence that decoherence in this system is negligible. This improvement in coherence has resulted in improved short-term stability at the level of 1.5E-11 fractional frequency stability for a one second integration period. In combination with improved interrogation schemes, the improved spectrum has also resulted in dramatically smaller light shifts and improved long-term frequency stability – with the clock averaging down to the level of 1E-13 fractional frequency stability on time scales of over 10,000 seconds.