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arXiv:1102.2610

The Valididy of the Langevin Equation

J. Frenkel, Jason Taylor

Published Feb 13, 2011• 0 citations
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Abstract

The validity of the Langevin equation (both classical and quantum) is studied in cases when not all the equations of motion are linear. In particular, a model is studied in which the interaction is bilinear in the environment variables. We conclude that the equation is valid only for frequencies close to the frequency of the system alone. If the equation of motion of the system alone is nonlinear, we are unable to find a condition for the validity of the Langevin equation.

DOI
10.48550/arxiv.1102.2610

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The validity of the Langevin equation (both classical and quantum) is studied in cases when not all the equations of motion are linear. In particular, a model is studied in which the interaction is bilinear in the environment variables. We conclude that the equation is valid only for frequencies close to the frequency of the system alone. If the equation of motion of the system alone is nonlinear, we are unable to find a condition for the validity of the Langevin equation.
From microscopic models, a Langevin equation can, in general, be derived only as an approximation. Two possible conditions to validate this approximation are studied. One is, for a linear Langevin equation, that the frequency of the Fourier transform should be close to the natural frequency of the system. The other is by the assumption of "slow" variables. We test this method by comparison with an exactly soluble model and point out its limitations. We base our discussion on two approaches. The first is a direct, elementary treatment of Senitzky. The second is via a generalized Langevin equation as an intermediate step.
Building upon the work of Hu, Paz, and Zhang [1,2] on open quantum systems we consider the quantum Brownian motion (QBM) model with one oscillator (position variable xxx) as the system, {\it nonlinearly} coupled to an environment of NNN harmonic oscillators (with mass mnm_nmn​, natural frequency ωnω_nωn​, position qnq_nqn​ and momentum pnp_npn​ variables) in the form ∑n(vn1(x)qnk+vn2(x)pnl)\sum_{n}\left(v_{n1}(x)q_{n}^{k}+v_{n2}(x)p_{n}^{l}\right)∑n​(vn1​(x)qnk​+vn2​(x)pnl​) where k,lk, lk,l are integers (the present work only considers the k=l=2k=l=2k=l=2 cases). The vertex functions $v_{n1}, v_{n2} $ are of the form vn1=λCn1f(x),vn2(x)=−λ Cn2mn−2ωn−2f(x)v_{n1}=λC_{n1} f(x), v_{n2}(x)=-λ\,C_{n2}m_{n}^{-2}ω_{n}^{-2}f(x)vn1​=λCn1​f(x),vn2​(x)=−λCn2​mn−2​ωn−2​f(x) where Cn1,2C_{n1,2}Cn1,2​ are the coupling constants with the nnnth oscillator, f(x)f(x)f(x) is any arbitrary function of xxx, and λλλ is a dimensionless constant. Employing the closed-time-path formalism the influence action SIFS_{IF}SIF​ is calculated using a perturbative expansion in λλλ. It is possible to identify the terms in SIFS_{IF}SIF​ quadratic or higher in Δ(s)≡f(x+(s))−f(x−(s))Δ(s)\equiv f(x_{+}(s))-f(x_{-}(s))Δ(s)≡f(x+​(s))−f(x−​(s)) to constitute the noise kernel, while terms linear in ΔΔΔ to that of the dissipation kernel. The non-Gaussian noise kernel gives rise to non-zero three-point correlation function of the corresponding stochastic force. The pathway presented here should be useful for the exploration of \textit{non-Gaussian properties of systems nonlinearly coupled with their environments}; examples in early universe cosmology and in quantum optomechanics (QOM) are mentioned. A modified fluctuation-dissipation relation (FDR) is also established, which ensures the consistency of the model and the accuracy of results even at higher perturbative orders. Another result of significance is the derivation of a nonlinear Langevin equation which is expected to be useful for many open quantum system applications.
It has long been recognized that the dynamics of linear quantum systems is classical in the Wigner representation. Yet many conceptually important linear problems are typically analyzed using such generally applicable techniques as influence functionals and Bogoliubov transformations. In this Letter we point out that the classical equations of motion provide a simpler and more intuitive formalism for linear quantum systems. We examine the important problem of Brownian motion in the independent oscillator model, and show that the quantum dynamics is described directly and completely by a c-number Langevin equation. We are also able to apply recent insights into quantum Brownian motion to show that the classical Fokker-Planck equation is always local in time, regardless of the spectral density of the environment.
The generalized Langevin equation and its attendant fluctuation–dissipation relation (FDR) for both classical and quantum systems is explictly derived for a large class of system-bath interaction potentials. We demonstrate for this class of potentials that the classical FDR involving only the temperature of the bath is satisfied, and that in general the decay times of the dissipative processes and of the system are temperature dependent. We also demonstrate that the quantum FDR depends in detail on the nature of the bath and on the specific system-bath interaction. Thus we conclude that while the classical Langevin equation is phenomenologically useful, its quantum counterpart is much more limited.